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Phase transition and anomalous low temperature ferromagnetic phase in Pr 0.6Sr 0.4MnO 3 single crystals

2009, Rößler, S., Harikrishnan, S., Naveen Kumar, C.M., Bhat, H.L., Elizabeth, S., Rößler, U.K., Steglich, F., Wirth, S.

We report on the magnetic and electrical properties of Pr 0.6Sr 0.4MnO 3 single crystals. This compound undergoes a continuous paramagnetic-ferromagnetic transition with a Curie temperature T C301 K and a first-order structural transition at T S64 K. At T S, the magnetic susceptibility exhibits an abrupt jump, and a corresponding small hump is seen in the resistivity. The critical behavior of the static magnetization and the temperature dependence of the resistivity are consistent with the behavior expected for a nearly isotropic ferromagnet with short-range exchange belonging to the Heisenberg universality class. The magnetization (M-H) curves below T S are anomalous in that the virgin curve lies outside the subsequent M-H loops. The hysteretic structural transition at T S as well as the irreversible magnetization processes below T S can be explained by phase separation between a high-temperature orthorhombic and a low-temperature monoclinic ferromagnetic phase.

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Magnetic field-induced twin boundary motion in polycrystalline Ni-Mn-Ga fibres

2008, Scheerbaum, N., Heczko, O., Liu, J., Hinz, D., Schultz, L., Gutfleisch, O.

Magnetic field-induced twin boundary motion leading to large magnetic field-induced strain of ~1.0% was established in polycrystalline Ni50.9Mn27.1Ga22.0 (at.%) fibres at room temperature (~60–100 μm in diameter and ~3 mm in length). The fibres' grains are as large as the fibre diameter and of random orientation. At room temperature, a ferromagnetic 5M martensite is found. Magnetic field-induced twin boundary motion was indicated by magnetic measurements and validated by electron backscatter diffraction (EBSD). The application of a magnetic field shifts the equilibrium temperature of martensite and austenite by ~0.4 K T−1, which agrees with calculations using the Clapeyron–Clausius approach.

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Hyper-domains in exchange bias micro-stripe pattern

2008, Theis-Bröhl, K., Westphalen, A., Zabel, H., Rücker, U., McCord, J., Höink, V., Schmalhorst, J., Reiss, G., Weis, T., Engel, D., Ehresmann, A., Toperverg, B.P.

A combination of experimental techniques, e.g. vector-MOKE magnetometry, Kerr microscopy and polarized neutron reflectometry, was applied to study the field induced evolution of the magnetization distribution over a periodic pattern of alternating exchange bias (EB) stripes. The lateral structure is imprinted into a continuous ferromagnetic/antiferromagnetic EB bilayer via laterally selective exposure to He-ion irradiation in an applied field. This creates an alternating frozen-in interfacial EB field competing with the external field in the course of the re-magnetization. It was found that in a magnetic field applied at an angle with respect to the EB axis parallel to the stripes the re-magnetization process proceeds via a variety of different stages. They include coherent rotation of magnetization towards the EB axis, precipitation of small random (ripple) domains, formation of a stripe-like alternation of the magnetization, and development of a state in which the magnetization forms large hyper-domains comprising a number of stripes. Each of those magnetic states is quantitatively characterized via the comprehensive analysis of data on specular and off-specular polarized neutron reflectivity. The results are discussed within a phenomenological model containing a few parameters, which can readily be controlled by designing systems with a desired configuration of magnetic moments of micro- and nano-elements.