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    Climatic response to anthropogenic sulphate aerosols versus well-mixed greenhouse gases from 1850 to 2000 AD in CLIMBER-2
    (Abingdon : Taylor and Francis Ltd., 2008) Bauer, E.; Petoukhov, V.; Ganopolski, A.; Eliseev, A.V.
    The Earth system model CLIMBER-2 is extended by a scheme for calculating the climatic response to anthropogenic sulphur dioxide emissions. The scheme calculates the direct radiative forcing, the first indirect cloud albedo effect, and the second indirect cloud lifetime effect induced by geographically resolved sulphate aerosol burden. The simulated anthropogenic sulphate aerosol burden in the year 2000 amounts to 0.47 TgS. The best guesses for the radiative forcing due to the direct effect are -0.4 W m-2 and for the decrease in short-wave radiation due to all aerosol effects -0.8 W m-2. The simulated global warming by 1 K from 1850 to 2000 caused by anthropogenic greenhouse gases reduces to 0.6 K when the sulphate aerosol effects are included. The model's hydrological sensitivity of 4%/K is decreased by the second indirect effect to 0.8%/K. The quality of the geographically distributed climatic response to the historic emissions of sulphur dioxide and greenhouse gases makes the extended model relevant to computational efficient investigations of future climate change scenarios.
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    Geoengineering climate by stratospheric sulfur injections: Earth system vulnerability to technological failure
    (Dordrecht [u.a.] : Springer, 2009) Brovkin, V.; Petoukhov, V.; Claussen, M.; Bauer, E.; Archer, D.; Jaeger, C.
    We use a coupled climate-carbon cycle model of intermediate complexity to investigate scenarios of stratospheric sulfur injections as a measure to compensate for CO2-induced global warming. The baseline scenario includes the burning of 5,000 GtC of fossil fuels. A full compensation of CO2-induced warming requires a load of about 13 MtS in the stratosphere at the peak of atmospheric CO2 concentration. Keeping global warming below 2°C reduces this load to 9 MtS. Compensation of CO 2 forcing by stratospheric aerosols leads to a global reduction in precipitation, warmer winters in the high northern latitudes and cooler summers over northern hemisphere landmasses. The average surface ocean pH decreases by 0.7, reducing the calcifying ability of marine organisms. Because of the millennial persistence of the fossil fuel CO2 in the atmosphere, high levels of stratospheric aerosol loading would have to continue for thousands of years until CO2 was removed from the atmosphere. A termination of stratospheric aerosol loading results in abrupt global warming of up to 5°C within several decades, a vulnerability of the Earth system to technological failure. © 2008 The Author(s).
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    Small-scale mixing processes enhancing troposphere-to-stratosphere transport by pyro-cumulonimbus storms
    (Göttingen : Copernicus GmbH, 2007) Luderer, G.; Trentmann, J.; Hungershöfer, K.; Herzog, M.; Fromm, M.; Andreae, M.O.
    Deep convection induced by large forest fires is an efficient mechanism for transport of aerosol particles and trace gases into the upper troposphere and lower stratosphere (UT/LS). For many pyro-cumulonimbus clouds (pyroCbs) as well as other cases of severe convection without fire forcing, radiometric observations of cloud tops in the thermal infrared (IR) reveal characteristic structures, featuring a region of relatively high brightness temperatures (warm center) surrounded by a U-shaped region of low brightness temperatures. We performed a numerical simulation of a specific case study of pyroCb using a non-hydrostatic cloud resolving model with a two-moment cloud microphysics parameterization and a prognostic turbulence scheme. The model is able to reproduce the thermal IR structure as observed from satellite radiometry. Our findings establish a close link between the observed temperature pattern and small-scale mixing processes atop and downwind of the overshooting dome of the pyroCb. Such small-scale mixing processes are strongly enhanced by the formation and breaking of a stationary gravity wave induced by the overshoot. They are found to increase the stratospheric penetration of the smoke by up to almost 30 K and thus are of major significance for irreversible transport of forest fire smoke into the lower stratosphere.