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Generation of terahertz radiation from ionizing two-color laser pulses in Ar filled metallic hollow waveguides
The generation of THz radiation from ionizing two-color femtosecond pulses propagating in metallic hollow waveguides filled with Ar is numerically studied. We observe a strong reshaping of the low-frequency part of the spectrum. Namely, after several millimeters of propagation the spectrum is extended from hundreds of GHz up to 150 THz. For longer propagation distances, nearly single-cycle near-infrared pulses with wavelengths around 4.5 μm are obtained by appropriate spectral filtering, with an efficiency of up to 0.25 %.
Symmetry breaking and strong persistent plasma currents via resonant destabilization of atoms
The ionization rate of an atom in a strong optical field can be resonantly enhanced by the presence of long-living atomic levels (so called Freeman resonances). This process is most prominent in the multiphoton ionization regime meaning that ionization event takes many optical cycles. Nevertheless, here we show that these resonances can lead to fast subcycle-scale plasma buildup at the resonant values of the intensity in the pump pulse. The fast buildup can break the cycletocycle symmetry of the ionization process, resulting in generation of persistent macroscopic plasma currents which remain after the end of the pulse. This, in turn, gives rise to a broadband radiation of unusual spectral structure forming a comb from terahertz (THz) to visible. This radiation contains fingerprints of the attosecond electronic dynamics in Rydberg states during ionization.
Ultrafast spatio-temporal dynamics of terahertz generation by ionizing two-color femtosecond pulses in gases
We present a combined theoretical and experimental study of spatio-temporal propagation effects in terahertz (THz) generation in gases using two-color ionizing laser pulses. The observed strong broadening of the THz spectra with increasing gas pressure reveals the prominent role of spatio-temporal reshaping and of a plasma-induced blue-shift of the pump pulses in the generation process. Results obtained from (3+1)-dimensional simulations are in good agreement with experimental findings and clarify the mechanisms responsible for THz emission.