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- ItemGraphene Q-switched Yb:KYW planar waveguide laser(New York, NY : American Inst. of Physics, 2015) Kim, Jun Wan; Young Choi, Sun; Aravazhi, Shanmugam; Pollnau, Markus; Griebner, Uwe; Petrov, Valentin; Bae, Sukang; Jun Ahn, Kwang; Yeom, Dong-Il; Rotermund, FabianA diode-pumped Yb:KYW planar waveguide laser, single-mode Q-switched by evanescent-field interaction with graphene, is demonstrated for the first time. Few-layer graphene grown by chemical vapor deposition is transferred onto the top of a guiding layer, which initiates stable Q-switched operation in a 2.4-cm-long waveguide laser operating near 1027 nm. Average output powers up to 34 mW and pulse durations as short as 349 ns are achieved. The measured output beam profile, clearly exhibiting a single mode, agrees well with the theoretically calculated mode intensity distribution inside the waveguide. As the pump power is increased, the repetition rate and pulse energy increase from 191 to 607 kHz and from 7.4 to 58.6 nJ, respectively, whereas the pulse duration decreases from 2.09 μs to 349 ns.
- ItemInfrared spectroscopy in superfluid helium droplets(Abingdon : Taylor and Francis Ltd., 2019) Verma D.; Tanyag R.M.P.; O’Connell S.M.O.; Vilesov A.F.For more than two decades, encapsulation in superfluid helium nanodroplets has served as a reliable technique for probing the structure and dynamics of molecules and clusters at a low temperature of ≈0.37 K. Due to weak interactions between molecules and the host liquid helium, good spectral resolution can usually be achieved, making helium droplets an ideal matrix for spectroscopy in a wide spectral range from infrared to ultraviolet. Furthermore, rotational structure in the spectra of small molecules provides a unique probe for interactions with the superfluid on an atomic scale. This review presents a summary of results and a discussion of recent experimental developments in helium droplet spectroscopy with the emphasis laid on infrared studies. Initially, studies focused on single molecules and have been expanded to larger species, such as metal-molecular clusters, biomolecules, free radicals, ions, and proteins. © 2018 The Author(s). Published by Informa UK Limited, trading as Taylor & Francis Group.
- ItemExcitation of H2 at large internuclear separation: F1∑+g outer well states and continuum resonances(London : Taylor & Francis, 2019) Trivikram, T.M.; Salumbides, E.J.; Jungen, Ch.; Ubachs, W.Bound and free quantum resonances of molecular hydrogen exhibiting wave-function density at large internuclear separation, (Formula presented.) 4–5 a.u., are excited via multi-step laser spectroscopy. Highly excited vibrational levels of H (Formula presented.) are prepared via two-photon UV-photolysis of H (Formula presented.) S. Subsequent two-photon Doppler-free precision measurements are performed connecting (Formula presented.) levels with (Formula presented.) outer-well levels. Detection and spectroscopic labelling of the quantum states is assisted by further laser excitation into the auto-ionisation continuum employing a third UV-laser. Level energies of high rotational states ((Formula presented.)) in the outer-well state (Formula presented.) are accurately determined. The three-laser study demonstrates a method for probing resonances in the H (Formula presented.) ionisation continuum with wave-function density at large internuclear separation (Formula presented.) 4–5 a.u., large angular momenta J, and energy range 131,100–133,000 cm-1, a hitherto unexplored territory. © 2019, © 2019 The Author(s). Published by Informa UK Limited, trading as Taylor & Francis Group.
- ItemGeneration of millijoule few-cycle pulses at 5 μm by indirect spectral shaping of the idler in an optical parametric chirped pulse amplifier(Washington, DC : Soc., 2018) Bock, Martin; Grafenstein, Lorenz von; Griebner, Uwe; Elsaesser, ThomasSpectral pulse shaping in a high-intensity midwave-infrared (MWIR) optical parametric chirped pulse amplifier (OPCPA) operating at 1 kHz repetition rate is reported. We successfully apply a MWIR spatial light modulator (SLM) for the generation of ultrashort idler pulses at 5 μm wavelength. Only bulk optics and active phase control of the 3.5 μm signal pulses via the SLM are employed for generating compressed idler pulses with a duration of 80 fs. The 80-fs pulse duration corresponds to less than five optical cycles at the central wavelength of 5.0 μm. The pulse energy amounts to 1.0 mJ, which translates into a peak power of 10 GW. The generated pulse parameters represent record values for high-intensity MWIR OPCPAs.
- ItemX-ray emission from stainless steel foils irradiated by femtosecond petawatt laser pulses(Bristol : IOP Publ., 2018) Alkhimova, M.A.; Faenov, A.Ya.; Pikuz, T.A.; Skobelev, I.Yu.; Pikuz, S.A.; Nishiuchi, M.; Sakaki, H.; Pirozhkov, A.S.; Sagisaka, S.; Dover, N.P.; Kondo, Ko.; Ogura, K.; Fukuda, Y.; Kiriyama, H.; Esirkepov, T.; Bulanov, S V.; Andreev, A.; Kando, M.; Zhidkov, A.; Nishitani, K.; Miyahara, T.; Watanabe, Y.; Kodama, R.; Kondo, K.We report about nonlinear growth of x-ray emission intensity emitted from plasma generated by femtosecond petawatt laser pulses irradiating stainless steel foils. X-ray emission intensity increases as ∼ I 4.5 with laser intensity I on a target. High spectrally resolved x-ray emission from front and rear surfaces of 5 μm thickness stainless steel targets were obtained at the wavelength range 1.7-2.1 Å, for the first time in experiments at femtosecond petawatt laser facility J-KAREN-P. Total intensity of front x-ray spectra three times dominates to rear side spectra for maximum laser intensity I ≈ 3.21021 W/cm2. Growth of x-ray emission is mostly determined by contribution of bremsstrahlung radiation that allowed estimating bulk electron plasma temperature for various magnitude of laser intensity on target.
- ItemLooking inside the tunnelling barrier: II. Co- and counter-rotating electrons at the ‘tunnelling exit’(Bristol : IOP Publ., 2018-08-03) Kaushal, Jivesh; Smirnova, OlgaThe initial conditions for electron trajectories at the exit from the tunnelling barrier are often used in strong field models, for example to bridge the first and the second steps of the three-step model celebrated in this issue. Since the analytical R-matrix theory does not rely on the three-step model or the concept of the tunnelling barrier in coordinate space, obtaining the initial conditions for electron trajectories at the barrier exit is, strictly speaking, not necessary to calculate standard observables. Not necessary, but possible—especially when motivated by the occasion of this issue. The opportunity to evaluate such initial conditions emerges as a corollary of analysing sub-barrier kinematics, which includes the interplay of laser and Coulomb fields on the sub-cycle scale (see the companion paper I). We apply our results to discuss the difference in such initial conditions for co- and counter-rotating electrons liberated during strong field ionisation. We derive quantum orbits and classical trajectories describing ionization dynamics of co- and counter-rotating electrons in long-range potentials.
- ItemTerahertz magnetic field enhancement in an asymmetric spiral metamaterial(Bristol : IOP Publ., 2018-10-25) Polley, Debanjan; Hagström, Nanna Zhou; Schmising, Clemens von Korff; Eisebitt, Stefan; Bonetti, StefanoWe use finite element simulations in both the frequency and the time-domain to study the terahertz resonance characteristics of a metamaterial (MM) comprising a spiral connected to a straight arm. The MM acts as a RLC circuit whose resonance frequency can be precisely tuned by varying the characteristic geometrical parameters of the spiral: inner and outer radius, width and number of turns. We provide a simple analytical model that uses these geometrical parameters as input to give accurate estimates of the resonance frequency. Finite element simulations show that linearly polarized terahertz radiation efficiently couples to the MM thanks to the straight arm, inducing a current in the spiral, which in turn induces a resonant magnetic field enhancement at the center of the spiral. We observe a large (approximately 40 times) and uniform (over an area of ∼10 μm2) enhancement of the magnetic field for narrowband terahertz radiation with frequency matching the resonance frequency of the MM. When a broadband, single-cycle terahertz pulse propagates towards the MM, the peak magnetic field of the resulting band-passed waveform still maintains a six-fold enhancement compared to the peak impinging field. Using existing laser-based terahertz sources, our MM design allows to generate magnetic fields of the order of 2 T over a time scale of several picoseconds, enabling the investigation of nonlinear ultrafast spin dynamics in table-top experiments. Furthermore, our MM can be implemented to generate intense near-field narrowband, multi-cycle electromagnetic fields to study generic ultrafast resonant terahertz dynamics in condensed matter.
- ItemPhase- and intensity-resolved measurements of above threshold ionization by few-cycle pulses(Bristol : IOP Publ., 2018-06-11) Kübel, M.; Arbeiter, M.; Burger, C.; Kling, Nora G.; Pischke, T.; Moshammer, R.; Fennel, T.; Kling, M.F.; Bergues, B.We investigate the carrier-envelope phase (CEP) and intensity dependence of the longitudinal momentum distribution of photoelectrons resulting from above threshold ionization of argon by few-cycle laser pulses. The intensity of the pulses with a center wavelength of 750 nm is varied in a range between 0.7 × 1014 and . Our measurements reveal a prominent maximum in the CEP-dependent asymmetry at photoelectron energies of 2 U P (U P being the ponderomotive potential), that is persistent over the entire intensity range. Further local maxima are observed around 0.3 and 0.8 U P. The experimental results are in good agreement with theoretical results obtained by solving the three-dimensional time-dependent Schrödinger equation. We show that for few-cycle pulses, the amplitude of the CEP-dependent asymmetry provides a reliable measure for the peak intensity on target. Moreover, the measured asymmetry amplitude exhibits an intensity-dependent interference structure at low photoelectron energy, which could be used to benchmark model potentials for complex atoms.
- ItemX-ray spectroscopy of super-intense laser-produced plasmas for the study of nonlinear processes. Comparison with PIC simulations(Bristol : IOP Publ., 2017) Dalimier, E.; Ya Faenov, A.; Oks, E.; Angelo, P.; Pikuz, T.A.; Fukuda, Y.; Andreev, A.; Koga, J.; Sakaki, H.; Kotaki, H.; Pirozhkov, A.; Hayashi, Y.; Skobelev, I.Yu.; Pikuz, S.A.; Kawachi, T.; Kando, M.; Kondo, K.; Zhidkov, A.; Tubman, E.; Butler, N.M.H.; Dance, R.J.; Alkhimova, M.A.; Booth, N.; Green, J.; Gregory, C.; McKenna, P.; Woolsey, N.; Kodama, R.We present X-ray spectroscopic diagnostics in femto-second laser-driven experiments revealing nonlinear phenomena caused by the strong coupling of the laser radiation with the created plasma. Among those nonlinear phenomena, we found the signatures of the Two Plasmon Decay (TPD) instability in a laser-driven CO2 cluster-based plasma by analyzing the Langmuir dips in the profile of the O VIII Lyϵ line, caused by the Langmuir waves created at the high laser intensity 3 1018Wcm-2. With similar laser intensities, we reveal also the nonlinear phenomenon of the Second Harmonic Generation (SHG) of the laser frequency by analyzing the nonlinear phenomenon of satellites of Lyman δ and ϵ lines of Ar XVII. In the case of relativistic laser-plasma interaction we discovered the Parametric Decay Instability (PDI)-induced ion acoustic turbulence produced simultaneously with Langmuir waves via irradiation of thin Si foils by laser intensities of 1021Wcm-2.
- ItemEmittance Reduction of RF Photoinjector Generated Electron Beams by Transverse Laser Beam Shaping(Bristol : IOP Publ., 2019) Gross, M.; Qian, H.J.; Boonpornprasert, P.; Chen, Y.; Good, J.D.; Huck, H.; Isaev, I.; Koschitzki, C.; Krasilnikov, M.; Lal, S.; Li, X.; Lishilin, O.; Loisch, G.; Melkumyan, D.; Mohanty, S.K.; Niemczyk, R.; Oppelt, A.; Shaker, H.; Shu, G.; Stephan, F.; Vashchenko, G.; Will, I.Laser pulse shaping is one of the key elements to generate low emittance electron beams with RF photoinjectors. Ultimately high performance can be achieved with ellipsoidal laser pulses, but 3-dimensional shaping is challenging. High beam quality can also be reached by simple transverse pulse shaping, which has demonstrated improved beam emittance compared to a transversely uniform laser in the 'pancake' photoemission regime. In this contribution we present the truncation of a Gaussian laser at a radius of approximately one sigma in the intermediate (electron bunch length directly after emission about the same as radius) photoemission regime with high acceleration gradients (up to 60 MV/m). This type of electron bunch is used e.g. at the European XFEL and FLASH free electron lasers at DESY, Hamburg site and is being investigated in detail at the Photoinjector Test facility at DESY in Zeuthen (PITZ). Here we present ray-tracing simulations and experimental data of a laser beamline upgrade enabling variable transverse truncation. Initial projected emittance measurements taken with help of this setup are shown, as well as supporting beam dynamics simulations. Additional simulations show the potential for substantial reduction of slice emittance at PITZ. © Published under licence by IOP Publishing Ltd.