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    Advanced fiber in-coupling through nanoprinted axially symmetric structures
    (New York, NY : AIP, 2023) Yermakov, Oleh; Zeisberger, Matthias; Schneidewind, Henrik; Kim, Jisoo; Bogdanov, Andrey; Kivshar, Yuri; Schmidt, Markus A.
    Here, we introduce and demonstrate nanoprinted all-dielectric nanostructures located on fiber end faces as a novel concept for the efficient coupling of light into optical fibers, especially at multiple incidence angles and across large angular intervals. Taking advantage of the unique properties of the nanoprinting technology, such as flexibly varying the width, height, and gap distance of each individual element, we realize different polymeric axial-symmetric structures, such as double-pitch gratings and aperiodic arrays, placed on the facet of commercial step-index fibers. Of particular note is the aperiodic geometry, enabling an unprecedentedly high average coupling efficiency across the entire angular range up to 80°, outperforming regular gratings and especially bare fibers by orders of magnitude. The excellent agreement between simulation and experiment clearly demonstrates the quality of the fabricated structures and the high accuracy of the nanoprinting process. Our approach enables realizing highly integrated and ready-to-use fiber devices, defining a new class of compact, flexible, and practically relevant all-fiber devices beyond the state-of-art. Applications can be found in a variety of cutting-edge fields that require highly efficient light collection over selected angular intervals, such as endoscopy or quantum technologies. Furthermore, fiber functionalization through nanoprinting represents a promising approach for interfacing highly complex functional photonic structures with optical fibers.
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    Perspectives on weak interactions in complex materials at different length scales
    (Cambridge : RSC Publ., 2022) Fiedler, J.; Berland, K.; Borchert, J.W.; Corkery, R. W.; Eisfeld, A.; Gelbwaser-Klimovsky, D.; Greve, M.M.; Holst, B.; Jacobs, K.; Krüger, M.; Parsons, D. F.; Persson, C.; Presselt, M.; Reisinger, T.; Scheel, S.; Stienkemeier, F.; Tømterud, M.; Walter, M.; Weitz, R.T.; Zalieckas, J.
    Nanocomposite materials consist of nanometer-sized quantum objects such as atoms, molecules, voids or nanoparticles embedded in a host material. These quantum objects can be exploited as a super-structure, which can be designed to create material properties targeted for specific applications. For electromagnetism, such targeted properties include field enhancements around the bandgap of a semiconductor used for solar cells, directional decay in topological insulators, high kinetic inductance in superconducting circuits, and many more. Despite very different application areas, all of these properties are united by the common aim of exploiting collective interaction effects between quantum objects. The literature on the topic spreads over very many different disciplines and scientific communities. In this review, we present a cross-disciplinary overview of different approaches for the creation, analysis and theoretical description of nanocomposites with applications related to electromagnetic properties.
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    Porous spherical gold nanoparticles via a laser induced process
    (Cambridge : Royal Society of Chemistry, 2022) Schmidl, Gabriele; Raugust, Marc; Jia, Guobin; Dellith, Andrea; Dellith, Jan; Schmidl, Frank; Plentz, Jonathan
    Nanoparticles consisting of a mixture of several metals and also porous nanoparticles due to their special structure exhibit properties that find applications in spectroscopic detection or catalysis. Different approaches of top down or bottom up technologies exist for the fabrication of such particles. We present a novel combined approach for the fabrication of spherical porous gold nanoparticles on low-cost glass substrates under ambient conditions using a UV-laser induced particle preparation process with subsequent wet chemical selective etching. In this preparation route, nanometer-sized branched structures are formed in spherical particles. The laser process, which is applied to a silver/gold bilayer system with different individual layer thicknesses, generates spherical mixed particles in a nanosecond range and influences the properties of the fabricated nanoparticles, such as the size and the mixture and thus the spectral response. The subsequent etching process is performed by selective wet chemical removal of silver from the nanoparticles with diluted nitric acid. The gold to silver ratio was investigated by energy-dispersive X-ray spectroscopy. The porosity depends on laser parameters and film thickness as well as on etching parameters such as time. After etching, the surface area of the remaining Au nanoparticles increases which makes these particles interesting for catalysis and also as carrier particles for substances. Such substances can be positioned at defined locations or be released in appropriate environments. Absorbance spectra are also analyzed to show how the altered fractured shape of the particles changes localized plasmon resonances of the resultingt particles.