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End date: 2024 × Start date: 2020 × DDC: 333.7 × DDC: 550 × Publisher: London : Springer Nature ×

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    Nucleation of jet engine oil vapours is a large source of aviation-related ultrafine particles
    (London : Springer Nature, 2022) Ungeheuer, Florian; Caudillo, Lucía; Ditas, Florian; Simon, Mario; van Pinxteren, Dominik; Kılıç, Doğuşhan; Rose, Diana; Jacobi, Stefan; Kürten, Andreas; Curtius, Joachim; Vogel, Alexander L.
    Large airports are a major source of ultrafine particles, which spread across densely populated residential areas, affecting air quality and human health. Jet engine lubrication oils are detectable in aviation-related ultrafine particles, however, their role in particle formation and growth remains unclear. Here we show the volatility and new-particle-formation ability of a common synthetic jet oil, and the quantified oil fraction in ambient ultrafine particles downwind of Frankfurt International Airport, Germany. We find that the oil mass fraction is largest in the smallest particles (10-18 nm) with 21% on average. Combining ambient particle-phase concentration and volatility of the jet oil compounds, we determine a lower-limit saturation ratio larger than 1 × 105 for ultra-low volatility organic compounds. This indicates that the oil is an efficient nucleation agent. Our results demonstrate that jet oil nucleation is an important mechanism that can explain the abundant observations of high number concentrations of non-refractory ultrafine particles near airports.
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    Global perturbation of stratospheric water and aerosol burden by Hunga eruption
    (London : Springer Nature, 2022) Khaykin, Sergey; Podglajen, Aurelien; Ploeger, Felix; Grooß, Jens-Uwe; Tence, Florent; Bekki, Slimane; Khlopenkov, Konstantin; Bedka, Kristopher; Rieger, Landon; Baron, Alexandre; Godin-Beekmann, Sophie; Legras, Bernard; Sellitto, Pasquale; Sakai, Tetsu; Barnes, John; Uchino, Osamu; Morino, Isamu; Nagai, Tomohiro; Wing, Robin; Baumgarten, Gerd; Gerding, Michael; Duflot, Valentin; Payen, Guillaume; Jumelet, Julien; Querel, Richard; Liley, Ben; Bourassa, Adam; Clouser, Benjamin; Feofilov, Artem; Hauchecorne, Alain; Ravetta, François
    The eruption of the submarine Hunga volcano in January 2022 was associated with a powerful blast that injected volcanic material to altitudes up to 58 km. From a combination of various types of satellite and ground-based observations supported by transport modeling, we show evidence for an unprecedented increase in the global stratospheric water mass by 13% relative to climatological levels, and a 5-fold increase of stratospheric aerosol load, the highest in the last three decades. Owing to the extreme injection altitude, the volcanic plume circumnavigated the Earth in only 1 week and dispersed nearly pole-to-pole in three months. The unique nature and magnitude of the global stratospheric perturbation by the Hunga eruption ranks it among the most remarkable climatic events in the modern observation era, with a range of potential long-lasting repercussions for stratospheric composition and climate.