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- ItemEstablishment of a Laboratory Scale Set-Up with Controlled Temperature and High Humidity to Investigate Dry Matter Losses of Wood Chips from Poplar during Storage(Basel : MDPI, 2022) Hernandez-Estrada, Albert; Pecenka, Ralf; Dumfort, Sabrina; Ascher-Jenull, Judith; Lenz, Hannes; Idler, Christine; Hoffmann, ThomasThe aim of this work was to improve the understanding of dry matter losses (DML) that occur in wood chips during the initial phase of storage in outdoor piles. For this purpose, a laboratory scale storage chamber was developed and investigated regarding its ability to recreate the conditions that chips undergo during the initial phase of outdoor storage. Three trials with poplar Max-4 (Populus maximowiczii Henry Populus nigra L.) chips were performed for 6–10 weeks in the storage chamber under controlled temperature and assisted humidity. Two different setups were investigated to maintain a high relative humidity (RH) inside the storage chamber; one using water containers, and one assisted with a humidifier. Moisture content (MC) and DML of the chips were measured at different storage times to evaluate their storage behaviour in the chamber. Additionally, microbiological analyses of the culturable fraction of saproxylic microbiota were performed, with a focus on mesophilic fungi, but discriminating also xerophilic fungi, and mesophilic bacteria, with focus on actinobacteria, in two trials, to gain a view on the poplar wood chip-inhabiting microorganisms as a function of storage conditions (moisture, temperature) and time. Results show that DML up to 8.8–13.7% occurred in the chips within 6–10 storage weeks. The maximum DML were reached in the trial using the humidifier, which seemed a suitable technique to keep a high RH in the testing chamber, and thus, to analyse the wood chips in conditions comparable to those in outdoor piles during the initial storage phase.
- ItemCylindrospermopsin is effectively degraded in water by pulsed corona-like and dielectric barrier discharges(Amsterdam [u.a.] : Elsevier Science, 2020) Schneider, Marcel; Rataj, Raphael; Kolb, Juergen F.; Bláha, LuděkCylindrospermopsin (CYN) is an important cyanobacterial toxin posing a major threat to surface waters during cyanobacterial blooms. Hence, methods for cyanotoxin removal are required to confront seasonal or local incidences to sustain the safety of potable water reservoirs. Non-thermal plasmas provide the possibility for an environmentally benign treatment which can be adapted to specific concentrations and environmental conditions without the need of additional chemicals. We therefore investigated the potential of two different non-thermal plasma approaches for CYN degradation, operated either in a water mist, i.e. in air, or submerged in water. A degradation efficacy of 0.03 ± 0.00 g kWh−1 L−1 was found for a dielectric barrier discharge (DBD) operated in air, while a submerged pulsed corona-like discharge resulted in an efficacy of 0.24 ± 0.02 g kWh−1 L−1. CYN degradation followed a pseudo zeroth order or pseudo first order reaction kinetic, respectively. Treatment efficacy of the corona-like discharge submerged in water increased with pH values of the initial solution changing from 5.0 to 7.5. Notably, a pH-depending residual oxidative effect was observed for the submerged discharge, resulting in ongoing CYN degradation, even without further plasma treatment. In this case hydroxyl radicals were identified as the dominant oxidants of CYN at acidic pH values. In comparison, degradation by the DBD could be related primarily to the generation of ozone. © 2020 The AuthorsThe degradation of cylindrospermopsin by a pulsed corona-like discharge in water was more effective compared with a pulsed dielectric barrier discharge in air around a water mist. © 2020 The Authors
- ItemResponsibility Under Uncertainty: Which Climate Decisions Matter Most?(Amsterdam : Baltzer Science Publ., 2023) Botta, Nicola; Brede, Nuria; Crucifix, Michel; Ionescu, Cezar; Jansson, Patrik; Li, Zheng; Martínez, Marina; Richter, TimWe propose a new method for estimating how much decisions under monadic uncertainty matter. The method is generic and suitable for measuring responsibility in finite horizon sequential decision processes. It fulfills “fairness” requirements and three natural conditions for responsibility measures: agency, avoidance and causal relevance. We apply the method to study how much decisions matter in a stylized greenhouse gas emissions process in which a decision maker repeatedly faces two options: start a “green” transition to a decarbonized society or further delay such a transition. We account for the fact that climate decisions are rarely implemented with certainty and that their consequences on the climate and on the global economy are uncertain. We discover that a “moral” approach towards decision making — doing the right thing even though the probability of success becomes increasingly small — is rational over a wide range of uncertainties.