192 results
Search Results
Now showing 1 - 10 of 192
- ItemEvaluating arbitrary strain configurations and doping in graphene with Raman spectroscopy(Bristol : IOP Publ., 2017-11-6) Mueller, Niclas S.; Heeg, Sebastian; Peña Alvarez, Miriam; Kusch, Patryk; Wasserroth, Sören; Clark, Nick; Schedin, Fredrik; Parthenios, John; Papagelis, Konstantinos; Galiotis, Costas; Kalbáč, Martin; Vijayaraghavan, Aravind; Huebner, Uwe; Gorbachev, Roman; Frank, Otakar; Reich, StephanieThe properties of graphene depend sensitively on strain and doping affecting its behavior in devices and allowing an advanced tailoring of this material. A knowledge of the strain configuration, i.e. the relative magnitude of the components of the strain tensor, is particularly crucial, because it governs effects like band-gap opening, pseudo-magnetic fields, and induced superconductivity. It also enters critically in the analysis of the doping level. We propose a method for evaluating unknown strain configurations and simultaneous doping in graphene using Raman spectroscopy. In our analysis we first extract the bare peak shift of the G and 2D modes by eliminating their splitting due to shear strain. The shifts from hydrostatic strain and doping are separated by a correlation analysis of the 2D and G frequencies, where we find Delta omega(2D)/Delta omega(G) = 2.21 +/- 0.05 for pure hydrostatic strain. We obtain the local hydrostatic strain, shear strain and doping without any assumption on the strain configuration prior to the analysis, as we demonstrate for two model cases: Graphene under uniaxial stress and graphene suspended on nanostructures that induce strain. Raman scattering with circular corotating polarization is ideal for analyzing frequency shifts, especially for weak strain when the peak splitting by shear strain cannot be resolved.
- ItemAnisotropic solid-liquid interface kinetics in silicon: An atomistically informed phase-field model(Bristol : IOP Publ., 2017) Bergmann, S.; Albe, K.; Flege, E.; Barragan-Yani, D.A.; Wagner, B.We present an atomistically informed parametrization of a phase-field model for describing the anisotropic mobility of liquid–solid interfaces in silicon. The model is derived from a consistent set of atomistic data and thus allows to directly link molecular dynamics and phase field simulations. Expressions for the free energy density, the interfacial energy and the temperature and orientation dependent interface mobility are systematically fitted to data from molecular dynamics simulations based on the Stillinger–Weber interatomic potential. The temperature-dependent interface velocity follows a Vogel–Fulcher type behavior and allows to properly account for the dynamics in the undercooled melt.
- ItemThe effect of oxygen admixture on the properties of microwave generated plasma in Ar-O2: A modelling study(Bristol : IOP Publ., 2021) Baeva, M; Stankov, M; Trautvetter, T; Methling, R; Hempel, F; Loffhagen, D; Foest, RThis work presents results of a self-consistent modelling analysis on microwave plasma generated in Ar-O2 mixtures at a frequency of 2.45 GHz at atmospheric pressure. The study focuses on how the plasma properties are influenced by the increase of the oxygen fraction in the gas mixture. The oxygen admixture is increased from 1% up to 95% in mass for values of the input microwave power of 1 and 1.5 kW. The results show that for a power of 1 kW and gradually increasing the oxygen admixture from 1% to 25% the electron density drops by a factor of more than four due to the energy lost by the electrons due to dissociation of oxygen molecules and the gas heating. An analysis of the number densities of species produced in the Ar-O2 plasma is presented. Oxygen admixtures of above 50% are considered along with an increase of the input microwave power in order to supply the discharge with electron number density values of the order of 1019 m-3. Gas temperatures above 3700 K are obtained in the plasma core along with a strong production of oxygen atoms with a number density of the order of 1023 m-3.
- ItemX-ray emission from stainless steel foils irradiated by femtosecond petawatt laser pulses(Bristol : IOP Publ., 2018) Alkhimova, M.A.; Faenov, A.Ya.; Pikuz, T.A.; Skobelev, I.Yu.; Pikuz, S.A.; Nishiuchi, M.; Sakaki, H.; Pirozhkov, A.S.; Sagisaka, S.; Dover, N.P.; Kondo, Ko.; Ogura, K.; Fukuda, Y.; Kiriyama, H.; Esirkepov, T.; Bulanov, S V.; Andreev, A.; Kando, M.; Zhidkov, A.; Nishitani, K.; Miyahara, T.; Watanabe, Y.; Kodama, R.; Kondo, K.We report about nonlinear growth of x-ray emission intensity emitted from plasma generated by femtosecond petawatt laser pulses irradiating stainless steel foils. X-ray emission intensity increases as ∼ I 4.5 with laser intensity I on a target. High spectrally resolved x-ray emission from front and rear surfaces of 5 μm thickness stainless steel targets were obtained at the wavelength range 1.7-2.1 Å, for the first time in experiments at femtosecond petawatt laser facility J-KAREN-P. Total intensity of front x-ray spectra three times dominates to rear side spectra for maximum laser intensity I ≈ 3.21021 W/cm2. Growth of x-ray emission is mostly determined by contribution of bremsstrahlung radiation that allowed estimating bulk electron plasma temperature for various magnitude of laser intensity on target.
- ItemLooking inside the tunnelling barrier: II. Co- and counter-rotating electrons at the ‘tunnelling exit’(Bristol : IOP Publ., 2018-08-03) Kaushal, Jivesh; Smirnova, OlgaThe initial conditions for electron trajectories at the exit from the tunnelling barrier are often used in strong field models, for example to bridge the first and the second steps of the three-step model celebrated in this issue. Since the analytical R-matrix theory does not rely on the three-step model or the concept of the tunnelling barrier in coordinate space, obtaining the initial conditions for electron trajectories at the barrier exit is, strictly speaking, not necessary to calculate standard observables. Not necessary, but possible—especially when motivated by the occasion of this issue. The opportunity to evaluate such initial conditions emerges as a corollary of analysing sub-barrier kinematics, which includes the interplay of laser and Coulomb fields on the sub-cycle scale (see the companion paper I). We apply our results to discuss the difference in such initial conditions for co- and counter-rotating electrons liberated during strong field ionisation. We derive quantum orbits and classical trajectories describing ionization dynamics of co- and counter-rotating electrons in long-range potentials.
- ItemHausdorff metric BV discontinuity of sweeping processes(Bristol : IOP Publ., 2016) Klein, Olaf; Recupero, VincenzoSweeping processes are a class of evolution differential inclusions arising in elastoplasticity and were introduced by J.J. Moreau in the early seventies. The solution operator of the sweeping processes represents a relevant example of rate independent operator. As a particular case we get the so called play operator, which is a typical example of a hysteresis operator. The continuity properties of these operators were studied in several works. In this note we address the continuity with respect to the strict metric in the space of functions of bounded variation with values in the metric space of closed convex subsets of a Hilbert space. We provide counterexamples showing that for all BV-formulations of the sweeping process the corresponding solution operator is not continuous when its domain is endowed with the strict topology of BV and its codomain is endowed with the L1-topology. This is at variance with the play operator which has a BV-extension that is continuous in this case.
- ItemTerahertz magnetic field enhancement in an asymmetric spiral metamaterial(Bristol : IOP Publ., 2018-10-25) Polley, Debanjan; Hagström, Nanna Zhou; Schmising, Clemens von Korff; Eisebitt, Stefan; Bonetti, StefanoWe use finite element simulations in both the frequency and the time-domain to study the terahertz resonance characteristics of a metamaterial (MM) comprising a spiral connected to a straight arm. The MM acts as a RLC circuit whose resonance frequency can be precisely tuned by varying the characteristic geometrical parameters of the spiral: inner and outer radius, width and number of turns. We provide a simple analytical model that uses these geometrical parameters as input to give accurate estimates of the resonance frequency. Finite element simulations show that linearly polarized terahertz radiation efficiently couples to the MM thanks to the straight arm, inducing a current in the spiral, which in turn induces a resonant magnetic field enhancement at the center of the spiral. We observe a large (approximately 40 times) and uniform (over an area of ∼10 μm2) enhancement of the magnetic field for narrowband terahertz radiation with frequency matching the resonance frequency of the MM. When a broadband, single-cycle terahertz pulse propagates towards the MM, the peak magnetic field of the resulting band-passed waveform still maintains a six-fold enhancement compared to the peak impinging field. Using existing laser-based terahertz sources, our MM design allows to generate magnetic fields of the order of 2 T over a time scale of several picoseconds, enabling the investigation of nonlinear ultrafast spin dynamics in table-top experiments. Furthermore, our MM can be implemented to generate intense near-field narrowband, multi-cycle electromagnetic fields to study generic ultrafast resonant terahertz dynamics in condensed matter.
- ItemPhase- and intensity-resolved measurements of above threshold ionization by few-cycle pulses(Bristol : IOP Publ., 2018-06-11) Kübel, M.; Arbeiter, M.; Burger, C.; Kling, Nora G.; Pischke, T.; Moshammer, R.; Fennel, T.; Kling, M.F.; Bergues, B.We investigate the carrier-envelope phase (CEP) and intensity dependence of the longitudinal momentum distribution of photoelectrons resulting from above threshold ionization of argon by few-cycle laser pulses. The intensity of the pulses with a center wavelength of 750 nm is varied in a range between 0.7 × 1014 and . Our measurements reveal a prominent maximum in the CEP-dependent asymmetry at photoelectron energies of 2 U P (U P being the ponderomotive potential), that is persistent over the entire intensity range. Further local maxima are observed around 0.3 and 0.8 U P. The experimental results are in good agreement with theoretical results obtained by solving the three-dimensional time-dependent Schrödinger equation. We show that for few-cycle pulses, the amplitude of the CEP-dependent asymmetry provides a reliable measure for the peak intensity on target. Moreover, the measured asymmetry amplitude exhibits an intensity-dependent interference structure at low photoelectron energy, which could be used to benchmark model potentials for complex atoms.
- ItemDelayed relaxation of highly excited naphthalene cations(Bristol : IOP Publ., 2020) Reitsma, G.; Hummert, J.; Dura, J.; Loriot, V.; Vrakking, M.J.J.; Lépine, F.; Kornilov, O.The efficiency of energy transfer in ultrafast electronic relaxation of molecules depends strongly on the complex interplay between electronic and nuclear motion. In this study we use wavelength-selected XUV pulses to induce relaxation dynamics of highly excited cationic states of naphthalene. Surprisingly, the observed relaxation lifetimes increase with the cationic excitation energy. We propose that this is a manifestation of a quantum mechanical population trapping that leads to delayed relaxation of molecules in the regions with a high density of excited states. © 2019 Published under licence by IOP Publishing Ltd.
- ItemLaser-induced surface modification of biopolymers - Micro/nanostructuring and functionalization(Bristol : IOP Publ., 2018) Stankova, N.E.; Atanasov, P.A.; Nedyalkov, N.N.; Tatchev, Dr.; Kolev, K.N.; Valova, E.I.; Armyanov, St.A.; Grochowska, K.; Śliwiński, G.; Fukata, N.; Hirsch, D.; Rauschenbach, B.The medical-grade polydimethylsiloxane (PDMS) elastomer is a widely used biomaterial in medicine for preparation of high-tech devices because of its remarkable properties. In this paper, we present experimental results on surface modification of PDMS elastomer by using ultraviolet, visible, and near-infrared ns-laser system and investigation of the chemical composition and the morphological structure inside the treated area in dependence on the processing parameters - wavelength, laser fluence and number of pulses. Remarkable chemical transformations and changes of the morphological structure were observed, resulting in the formation of a highly catalytically active surface, which was successfully functionalized via electroless Ni and Pt deposition by a sensitizing-activation free process. The results obtained are very promising in view of applying the methods of laser-induced micro- and nano-structuring and activation of biopolymers' surface and further electroless metal plating to the preparation of, e.g., multielectrode arrays (MEAs) devices in neural and muscular surface interfacing implantable systems.