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- ItemAnalysis of number size distributions of tropical free tropospheric aerosol particles observed at Pico Espejo (4765 m a.s.l.), Venezuela(München : European Geopyhsical Union, 2011) Schmeissner, T.; Krejci, R.; Ström, J.; Birmili, W.; Wiedensohler, A.; Hochschild, G.; Gross, J.; Hoffmann, P.; Calderon, S.The first long-term measurements of aerosol number and size distributions in South-American tropical free troposphere (FT) were performed from March 2007 until March 2009. The measurements took place at the high altitude Atmospheric Research Station Alexander von Humboldt. The station is located on top of the Sierra Nevada mountain ridge at 4765 m a.s.l. nearby the city of Mérida, Venezuela. Aerosol size distribution and number concentration data was obtained with a custom-built Differential Mobility Particle Sizer (DMPS) system and a Condensational Particle Counter (CPC). The analysis of the annual and diurnal variability of the tropical FT aerosol focused mainly on possible links to the atmospheric general circulation in the tropics. Considerable annual and diurnal cycles of the particle number concentration were observed. Highest total particle number concentrations were measured during the dry season (January–March, 519 ± 613 cm−3), lowest during the wet season (July–September, 318 ± 194 cm−3). The more humid FT (relative humidity (RH) range 50–95 %) contained generally higher aerosol particle number concentrations (573 ± 768 cm−3 during dry season, 320 ± 195 cm−3 during wet season) than the dry FT (RH < 50 %, 454 ± 332 cm−3 during dry season, 275 ± 172 cm−3 during wet season), indicating the importance of convection for aerosol distributions in the tropical FT. The diurnal cycle in the variability of the particle number concentration was mainly driven by local orography.
- ItemClassical nucleation theory of immersion freezing: sensitivity of contact angle schemes to thermodynamic and kinetic parameters(Katlenburg-Lindau : EGU, 2017) Ickes, Luisa; Welti, André; Lohmann, UlrikeHeterogeneous ice formation by immersion freezing in mixed-phase clouds can be parameterized in general circulation models (GCMs) by classical nucleation theory (CNT). CNT parameterization schemes describe immersion freezing as a stochastic process, including the properties of insoluble aerosol particles in the droplets. There are different ways to parameterize the properties of aerosol particles (i.e., contact angle schemes), which are compiled and tested in this paper. The goal of this study is to find a parameterization scheme for GCMs to describe immersion freezing with the ability to shift and adjust the slope of the freezing curve compared to homogeneous freezing to match experimental data. We showed in a previous publication that the resulting freezing curves from CNT are very sensitive to unconstrained kinetic and thermodynamic parameters in the case of homogeneous freezing. Here we investigate how sensitive the outcome of a parameter estimation for contact angle schemes from experimental data is to unconstrained kinetic and thermodynamic parameters. We demonstrate that the parameters describing the contact angle schemes can mask the uncertainty in thermodynamic and kinetic parameters. Different CNT formulations are fitted to an extensive immersion freezing dataset consisting of size-selected measurements as a function of temperature and time for different mineral dust types, namely kaolinite, illite, montmorillonite, microcline (K-feldspar), and Arizona test dust. We investigated how accurate different CNT formulations (with estimated fit parameters for different contact angle schemes) reproduce the measured freezing data, especially the time and particle size dependence of the freezing process. The results are compared to a simplified deterministic freezing scheme. In this context, we evaluated which CNT-based parameterization scheme able to represent particle properties is the best choice to describe immersion freezing in a GCM.
- ItemReduced Complexity Model Intercomparison Project Phase 1: introduction and evaluation of global-mean temperature response(Katlenburg-Lindau : Copernicus, 2020) Nicholls, Zebedee R. J.; Meinshausen, Malte; Lewis, Jared; Gieseke, Robert; Dommenget, Dietmar; Dorheim, Kalyn; Fan, Chen-Shuo; Fuglestvedt, Jan S.; Gasser, Thomas; Golüke, Ulrich; Goodwin, Philip; Hartin, Corinne; Hope, Austin P.; Kriegler, Elmar; Leach, Nicholas J.; Marchegiani, Davide; McBride, Laura A.; Quilcaille, Yann; Rogelj, Joeri; Salawitch, Ross J.; Samset, Bjørn H.; Sandstad, Marit; Shiklomanov, Alexey N.; Skeie, Ragnhild B.; Smith, Christopher J.; Smith, Steve; Tanaka, Katsumasa; Tsutsui, Junichi; Xie, ZhiangReduced-complexity climate models (RCMs) are critical in the policy and decision making space, and are directly used within multiple Intergovernmental Panel on Climate Change (IPCC) reports to complement the results of more comprehensive Earth system models. To date, evaluation of RCMs has been limited to a few independent studies. Here we introduce a systematic evaluation of RCMs in the form of the Reduced Complexity Model Intercomparison Project (RCMIP). We expect RCMIP will extend over multiple phases, with Phase 1 being the first. In Phase 1, we focus on the RCMs' global-mean temperature responses, comparing them to observations, exploring the extent to which they emulate more complex models and considering how the relationship between temperature and cumulative emissions of CO2 varies across the RCMs. Our work uses experiments which mirror those found in the Coupled Model Intercomparison Project (CMIP), which focuses on complex Earth system and atmosphere–ocean general circulation models. Using both scenario-based and idealised experiments, we examine RCMs' global-mean temperature response under a range of forcings. We find that the RCMs can all reproduce the approximately 1 ∘C of warming since pre-industrial times, with varying representations of natural variability, volcanic eruptions and aerosols. We also find that RCMs can emulate the global-mean temperature response of CMIP models to within a root-mean-square error of 0.2 ∘C over a range of experiments. Furthermore, we find that, for the Representative Concentration Pathway (RCP) and Shared Socioeconomic Pathway (SSP)-based scenario pairs that share the same IPCC Fifth Assessment Report (AR5)-consistent stratospheric-adjusted radiative forcing, the RCMs indicate higher effective radiative forcings for the SSP-based scenarios and correspondingly higher temperatures when run with the same climate settings. In our idealised setup of RCMs with a climate sensitivity of 3 ∘C, the difference for the ssp585–rcp85 pair by 2100 is around 0.23∘C(±0.12 ∘C) due to a difference in effective radiative forcings between the two scenarios. Phase 1 demonstrates the utility of RCMIP's open-source infrastructure, paving the way for further phases of RCMIP to build on the research presented here and deepen our understanding of RCMs.
- ItemThree-dimensional parameterizations of the synoptic scale kinetic energy and momentum flux in the Earth's atmosphere(Göttingen : Copernicus GmbH, 2011) Coumou, D.; Petoukhov, V.; Eliseev, A.V.We present a new set of statistical-dynamical equations (SDEs) which can accurately reproduce the three-dimensional atmospheric fields of synoptic scale kinetic energy and momentum flux. The set of equations is closed by finding proper parameterizations for the vertical macro-turbulent diffusion coefficient and ageostrophic terms. The equations have been implemented in a new SD atmosphere model, named Aeolus. We show that the synoptic scale kinetic energy and momentum fluxes generated by the model are in good agreement with empirical data, which were derived from bandpass-filtered ERA-40 data. In addition to present-day climate, the model is tested for substantially colder (last glacial maximum) and warmer (2×CO2) climates, and shown to be in agreement with general circulation model (GCM) results. With the derived equations, one can efficiently study the position and strength of storm tracks under different climate scenarios with calculation time a fraction of those of GCMs. This work prepares ground for the development of a new generation of fast Earth System Models of Intermediate Complexity which are able to perform multi-millennia simulations in a reasonable time frame while appropriately accounting for the climatic effect of storm tracks.
- ItemThe rôle of orographically and thermally forced stationary waves in the causation of the residual circulation(Milton Park : Taylor & Francis, 1999) Becker, E.; Schmitz, G.Several experiments performed with an idealized troposphere–stratosphere GCM are comparedto estimate the impact of orography and prescribed local heat sources on the residual circulationin the northern winter stratosphere. It is found that only the combined action of orographicand thermal wave forcing in northern midlatitudes is capable of inducing a residual circulationreaching continuously from tropical to polar latitudes at stratospheric altitudes. Intensificationsof the residual circulation in response to modified forcing of stationary waves are generallyassociated with, firstly, a reduced polar night jet accompanied by enhanced easterlies inlow and summer hemispheric latitudes and, secondly, substantial warming of the polar nightstratosphere completely compensated by cooling in the tropics and subtropics.