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- ItemA global analysis of climate-relevant aerosol properties retrieved from the network of Global Atmosphere Watch (GAW) near-surface observatories(Katlenburg-Lindau : Copernicus, 2020) Laj, Paolo; Bigi, Alessandro; Rose, Clémence; Andrews, Elisabeth; Lund Myhre, Cathrine; Collaud Coen, Martine; Lin, Yong; Wiedensohler, Alfred; Schulz, Michael; Ogren, John A.; Fiebig, Markus; Prenni, Anthony; Reisen, Fabienne; Romano, Salvatore; Sellegri, Karine; Sharma, Sangeeta; Schauer, Gerhard; Sheridan, Patrick; Sherman, James Patrick; Schütze, Maik; Schwerin, Andreas; Tuch, Thomas; Sohmer, Ralf; Sorribas, Mar; Steinbacher, Martin; Sun, Junying; Titos, Gloria; Toczko, Barbara; Tulet, Pierre; Tunved, Peter; Vakkari, Ville; Velarde, Fernando; Velasquez, Patricio; Villani, Paolo; Vratolis, Sterios; Wang, Sheng-Hsiang; Weinhold, Kay; Gliß, Jonas; Weller, Rolf; Yela, Margarita; Yus-Diez, Jesus; Zdimal, Vladimir; Zieger, Paul; Zikova, Nadezda; Mortier, Augustin; Pandolfi, Marco; Petäja, Tuukka; Kim, Sang-Woo; Aas, Wenche; Putaud, Jean-Philippe; Mayol-Bracero, Olga; Keywood, Melita; Labrador, Lorenzo; Aalto, Pasi; Ahlberg, Erik; Alados Arboledas, Lucas; Alastuey, Andrés; Andrade, Marcos; Artíñano, Begoña; Ausmeel, Stina; Arsov, Todor; Asmi, Eija; Backman, John; Baltensperger, Urs; Bastian, Susanne; Bath, Olaf; Beukes, Johan Paul; Brem, Benjamin T.; Bukowiecki, Nicolas; Conil, Sébastien; Couret, Cedric; Day, Derek; Dayantolis, Wan; Degorska, Anna; Eleftheriadis, Konstantinos; Fetfatzis, Prodromos; Favez, Olivier; Flentje, Harald; Gini, Maria I.; Gregorič, Asta; Gysel-Beer, Martin; Hallar, A. Gannet; Hand, Jenny; Hoffer, Andras; Hueglin, Christoph; Hooda, Rakesh K.; Hyvärinen, Antti; Kalapov, Ivo; Kalivitis, Nikos; Kasper-Giebl, Anne; Kim, Jeong Eun; Kouvarakis, Giorgos; Kranjc, Irena; Krejci, Radovan; Kulmala, Markku; Labuschagne, Casper; Lee, Hae-Jung; Lihavainen, Heikki; Lin, Neng-Huei; Löschau, Gunter; Luoma, Krista; Marinoni, Angela; Martins Dos Santos, Sebastiao; Meinhardt, Frank; Merkel, Maik; Metzger, Jean-Marc; Mihalopoulos, Nikolaos; Nguyen, Nhat Anh; Ondracek, Jakub; Pérez, Noemi; Perrone, Maria Rita; Petit, Jean-Eudes; Picard, David; Pichon, Jean-Marc; Pont, Veronique; Prats, NataliaAerosol particles are essential constituents of the Earth's atmosphere, impacting the earth radiation balance directly by scattering and absorbing solar radiation, and indirectly by acting as cloud condensation nuclei. In contrast to most greenhouse gases, aerosol particles have short atmospheric residence times, resulting in a highly heterogeneous distribution in space and time. There is a clear need to document this variability at regional scale through observations involving, in particular, the in situ near-surface segment of the atmospheric observation system. This paper will provide the widest effort so far to document variability of climate-relevant in situ aerosol properties (namely wavelength dependent particle light scattering and absorption coefficients, particle number concentration and particle number size distribution) from all sites connected to the Global Atmosphere Watch network. High-quality data from almost 90 stations worldwide have been collected and controlled for quality and are reported for a reference year in 2017, providing a very extended and robust view of the variability of these variables worldwide. The range of variability observed worldwide for light scattering and absorption coefficients, single-scattering albedo, and particle number concentration are presented together with preliminary information on their long-term trends and comparison with model simulation for the different stations. The scope of the present paper is also to provide the necessary suite of information, including data provision procedures, quality control and analysis, data policy, and usage of the ground-based aerosol measurement network. It delivers to users of the World Data Centre on Aerosol, the required confidence in data products in the form of a fully characterized value chain, including uncertainty estimation and requirements for contributing to the global climate monitoring system.
- ItemOn the importance of cascading moisture recycling in South America(München : European Geopyhsical Union, 2014) Zemp, D.C.; Schleussner, C.-F.; Barbosa, H.M.J.; van der Ent, R.J.; Donges, J.F.; Heinke, J.; Sampaio, G.; Rammig, A.Continental moisture recycling is a crucial process of the South American climate system. In particular, evapotranspiration from the Amazon basin contributes substantially to precipitation regionally as well as over other remote regions such as the La Plata basin. Here we present an in-depth analysis of South American moisture recycling mechanisms. In particular, we quantify the importance of cascading moisture recycling (CMR), which describes moisture transport between two locations on the continent that involves re-evaporation cycles along the way. Using an Eulerian atmospheric moisture tracking model forced by a combination of several historical climate data sets, we were able to construct a complex network of moisture recycling for South America. Our results show that CMR contributes about 9–10% to the total precipitation over South America and 17–18% over the La Plata basin. CMR increases the fraction of total precipitation over the La Plata basin that originates from the Amazon basin from 18–23 to 24–29% during the wet season. We also show that the south-western part of the Amazon basin is not only a direct source of rainfall over the La Plata basin, but also a key intermediary region that distributes moisture originating from the entire Amazon basin towards the La Plata basin during the wet season. Our results suggest that land use change in this region might have a stronger impact on downwind rainfall than previously thought. Using complex network analysis techniques, we find the eastern side of the sub-tropical Andes to be a key region where CMR pathways are channeled. This study offers a better understanding of the interactions between the vegetation and the atmosphere on the water cycle, which is needed in a context of land use and climate change in South America.
- ItemCoincidences of climate extremes and anomalous vegetation responses: Comparing tree ring patterns to simulated productivity(München : European Geopyhsical Union, 2015) Rammig, A.; Wiedermann, M.; Donges, J.F.; Babst, F.; von Bloh, W.; Frank, D.; Thonicke, K.; Mahecha, M.D.Climate extremes can trigger exceptional responses in terrestrial ecosystems, for instance by altering growth or mortality rates. Such effects are often manifested in reductions in net primary productivity (NPP). Investigating a Europe-wide network of annual radial tree growth records confirms this pattern: we find that 28% of tree ring width (TRW) indices are below two standard deviations in years in which extremely low precipitation, high temperatures or the combination of both noticeably affect tree growth. Based on these findings, we investigate possibilities for detecting climate-driven patterns in long-term TRW data to evaluate state-of-the-art dynamic vegetation models such as the Lund-Potsdam-Jena dynamic global vegetation model for managed land (LPJmL). The major problem in this context is that LPJmL simulates NPP but not explicitly the radial tree growth, and we need to develop a generic method to allow for a comparison between simulated and observed response patterns. We propose an analysis scheme that quantifies the coincidence rate of climate extremes with some biotic responses (here TRW or simulated NPP). We find a relative reduction of 34% in simulated NPP during precipitation, temperature and combined extremes. This reduction is comparable to the TRW response patterns, but the model responds much more sensitively to drought stress. We identify 10 extreme years during the 20th century during which both model and measurements indicate high coincidence rates across Europe. However, we detect substantial regional differences in simulated and observed responses to climatic extreme events. One explanation for this discrepancy could be the tendency of tree ring data to originate from climatically stressed sites. The difference between model and observed data is amplified by the fact that dynamic vegetation models are designed to simulate mean ecosystem responses on landscape or regional scales. We find that both simulation results and measurements display carry-over effects from climate anomalies during the previous year. We conclude that radial tree growth chronologies provide a suitable basis for generic model benchmarks. The broad application of coincidence analysis in generic model benchmarks along with an increased availability of representative long-term measurements and improved process-based models will refine projections of the long-term carbon balance in terrestrial ecosystems.
- ItemImpact of temperature and precipitation extremes on the flowering dates of four German wildlife shrub species(München : European Geopyhsical Union, 2016) Siegmund, Jonatan F.; Wiedermann, Marc; Donges, Jonathan F.; Donner, Reik V.Ongoing climate change is known to cause an increase in the frequency and amplitude of local temperature and precipitation extremes in many regions of the Earth. While gradual changes in the climatological conditions have already been shown to strongly influence plant flowering dates, the question arises if and how extremes specifically impact the timing of this important phenological phase. Studying this question calls for the application of statistical methods that are tailored to the specific properties of event time series. Here, we employ event coincidence analysis, a novel statistical tool that allows assessing whether or not two types of events exhibit similar sequences of occurrences in order to systematically quantify simultaneities between meteorological extremes and the timing of the flowering of four shrub species across Germany. Our study confirms previous findings of experimental studies by highlighting the impact of early spring temperatures on the flowering of the investigated plants. However, previous studies solely based on correlation analysis do not allow deriving explicit estimates of the strength of such interdependencies without further assumptions, a gap that is closed by our analysis. In addition to direct impacts of extremely warm and cold spring temperatures, our analysis reveals statistically significant indications of an influence of temperature extremes in the autumn preceding the flowering.
- ItemImpacts of enhanced weathering on biomass production for negative emission technologies and soil hydrology(Katlenburg-Lindau [u.a.] : Copernicus, 2020) De Oliveira Garcia, Wagner; Amann, Thorben; Hartmann, Jens; Karstens, Kristine; Popp, Alexander; Boysen, Lena R.; Smith, Pete; Goll, DanielLimiting global mean temperature changes to well below 2 °C likely requires a rapid and large-scale deployment of negative emission technologies (NETs). Assessments so far have shown a high potential of biomass-based terrestrial NETs, but only a few assessments have included effects of the commonly found nutrient-deficient soils on biomass production. Here, we investigate the deployment of enhanced weathering (EW) to supply nutrients to areas of afforestation-reforestation and naturally growing forests (AR) and bioenergy grasses (BG) that are deficient in phosphorus (P), besides the impacts on soil hydrology. Using stoichiometric ratios and biomass estimates from two established vegetation models, we calculated the nutrient demand of AR and BG. Insufficient geogenic P supply limits C storage in biomass. For a mean P demand by AR and a lowgeogenic-P-supply scenario, AR would sequester 119 Gt C in biomass; for a high-geogenic-P-supply and low-AR-Pdemand scenario, 187 Gt C would be sequestered in biomass; and for a low geogenic P supply and high AR P demand, only 92 GtC would be accumulated by biomass. An average amount of ∼ 150 Gt basalt powder applied for EW would be needed to close global P gaps and completely sequester projected amounts of 190 Gt C during the years 2006-2099 for the mean AR P demand scenario (2-362 Gt basalt powder for the low-AR-P-demand and for the high-AR-P-demand scenarios would be necessary, respectively). The average potential of carbon sequestration by EW until 2099 is ∼ 12 GtC (∼ 0:2-∼ 27 Gt C) for the specified scenarios (excluding additional carbon sequestration via alkalinity production). For BG, 8 kg basaltm2 a1 might, on average, replenish the exported potassium (K) and P by harvest. Using pedotransfer functions, we show that the impacts of basalt powder application on soil hydraulic conductivity and plant-Available water, to close predicted P gaps, would depend on basalt and soil texture, but in general the impacts are marginal. We show that EW could potentially close the projected P gaps of an AR scenario and nutrients exported by BG harvest, which would decrease or replace the use of industrial fertilizers. Besides that, EW ameliorates the soil's capacity to retain nutrients and soil pH and replenish soil nutrient pools. Lastly, EW application could improve plant-Available-water capacity depending on deployed amounts of rock powder - adding a new dimension to the coupling of land-based biomass NETs with EW. © 2020 Royal Society of Chemistry. All rights reserved.
- ItemRole of CO2, climate and land use in regulating the seasonal amplitude increase of carbon fluxes in terrestrial ecosystems: A multimodel analysis(München : European Geopyhsical Union, 2016) Zhao, Fang; Zeng, Ning; Asrar, Ghassem; Friedlingstein, Pierre; Ito, Akihiko; Jain, Atul; Kalnay, Eugenia; Kato, Etsushi; Koven, Charles D.; Poulter, Ben; Rafique, Rashid; Sitch, Stephen; Shu, Shijie; Stocker, Beni; Viovy, Nicolas; Wiltshire, Andy; Zaehle, SonkeWe examined the net terrestrial carbon flux to the atmosphere (FTA) simulated by nine models from the TRENDY dynamic global vegetation model project for its seasonal cycle and amplitude trend during 1961–2012. While some models exhibit similar phase and amplitude compared to atmospheric inversions, with spring drawdown and autumn rebound, others tend to rebound early in summer. The model ensemble mean underestimates the magnitude of the seasonal cycle by 40 % compared to atmospheric inversions. Global FTA amplitude increase (19 ± 8 %) and its decadal variability from the model ensemble are generally consistent with constraints from surface atmosphere observations. However, models disagree on attribution of this long-term amplitude increase, with factorial experiments attributing 83 ± 56 %, −3 ± 74 and 20 ± 30 % to rising CO2, climate change and land use/cover change, respectively. Seven out of the nine models suggest that CO2 fertilization is the strongest control – with the notable exception of VEGAS, which attributes approximately equally to the three factors. Generally, all models display an enhanced seasonality over the boreal region in response to high-latitude warming, but a negative climate contribution from part of the Northern Hemisphere temperate region, and the net result is a divergence over climate change effect. Six of the nine models show that land use/cover change amplifies the seasonal cycle of global FTA: some are due to forest regrowth, while others are caused by crop expansion or agricultural intensification, as revealed by their divergent spatial patterns. We also discovered a moderate cross-model correlation between FTA amplitude increase and increase in land carbon sink (R2 = 0.61). Our results suggest that models can show similar results in some benchmarks with different underlying mechanisms; therefore, the spatial traits of CO2 fertilization, climate change and land use/cover changes are crucial in determining the right mechanisms in seasonal carbon cycle change as well as mean sink change.
- ItemThe "dual-spot" Aethalometer: An improved measurement of aerosol black carbon with real-time loading compensation(München : European Geopyhsical Union, 2015) Drinovec, L.; Močnik, G.; Zotter, P.; Prévôt, A.S.H.; Ruckstuhl, C.; Coz, E.; Rupakheti, M.; Sciare, J.; Müller, T.; Wiedensohler, A.; Hansen, A.D.A.Aerosol black carbon is a unique primary tracer for combustion emissions. It affects the optical properties of the atmosphere and is recognized as the second most important anthropogenic forcing agent for climate change. It is the primary tracer for adverse health effects caused by air pollution. For the accurate determination of mass equivalent black carbon concentrations in the air and for source apportionment of the concentrations, optical measurements by filter-based absorption photometers must take into account the "filter loading effect". We present a new real-time loading effect compensation algorithm based on a two parallel spot measurement of optical absorption. This algorithm has been incorporated into the new Aethalometer model AE33. Intercomparison studies show excellent reproducibility of the AE33 measurements and very good agreement with post-processed data obtained using earlier Aethalometer models and other filter-based absorption photometers. The real-time loading effect compensation algorithm provides the high-quality data necessary for real-time source apportionment and for determination of the temporal variation of the compensation parameter k.
- ItemConsecutive extreme flooding and heat wave in Japan: Are they becoming a norm?(Hoboken, NJ : Wiley, 2019) Wang, Simon S.-Y.; Kim, Hyungjun; Coumou, Dim; Yoon, Jin-Ho; Zhao, Lin; Gillies, Robert R.[No abstract available]
- ItemClimate and air quality impacts due to mitigation of non-methane near-term climate forcers(Katlenburg-Lindau : EGU, 2020) Allen, Robert J.; Turnock, Steven; Nabat, Pierre; Neubauer, David; Lohmann, Ulrike; Olivié, Dirk; Oshima, Naga; Michou, Martine; Wu, Tongwen; Zhang, Jie; Takemura, Toshihiko; Schulz, Michael; Tsigaridis, Kostas; Bauer, Susanne E.; Emmons, Louisa; Horowitz, Larry; Naik, Vaishali; van Noije, Twan; Bergman, Tommi; Lamarque, Jean-Francois; Zanis, Prodromos; Tegen, Ina; Westervelt, Daniel M.; Le Sager, Philippe; Good, Peter; Shim, Sungbo; O’Connor, Fiona; Akritidis, Dimitris; Georgoulias, Aristeidis K.; Deushi, Makoto; Sentman, Lori T.; John, Jasmin G.; Fujimori, Shinichiro; Collins, William J.It is important to understand how future environmental policies will impact both climate change and air pollution. Although targeting near-term climate forcers (NTCFs), defined here as aerosols, tropospheric ozone, and precursor gases, should improve air quality, NTCF reductions will also impact climate. Prior assessments of the impact of NTCF mitigation on air quality and climate have been limited. This is related to the idealized nature of some prior studies, simplified treatment of aerosols and chemically reactive gases, as well as a lack of a sufficiently large number of models to quantify model diversity and robust responses. Here, we quantify the 2015-2055 climate and air quality effects of non-methane NTCFs using nine state-of-the-art chemistry-climate model simulations conducted for the Aerosol and Chemistry Model Intercomparison Project (AerChemMIP). Simulations are driven by two future scenarios featuring similar increases in greenhouse gases (GHGs) but with weak (SSP3-7.0) versus strong (SSP3-7.0-lowNTCF) levels of air quality control measures. As SSP3-7.0 lacks climate policy and has the highest levels of NTCFs, our results (e.g., surface warming) represent an upper bound. Unsurprisingly, we find significant improvements in air quality under NTCF mitigation (strong versus weak air quality controls). Surface fine particulate matter (PM2:5) and ozone (O3) decrease by 2:20:32 ugm3 and 4:60:88 ppb, respectively (changes quoted here are for the entire 2015-2055 time period; uncertainty represents the 95% confidence interval), over global land surfaces, with larger reductions in some regions including south and southeast Asia. Non-methane NTCF mitigation, however, leads to additional climate change due to the removal of aerosol which causes a net warming effect, including global mean surface temperature and precipitation increases of 0:250:12K and 0:030:012mmd1, respectively. Similarly, increases in extreme weather indices, including the hottest and wettest days, also occur. Regionally, the largest warming and wetting occurs over Asia, including central and north Asia (0:660:20K and 0:030:02mmd1), south Asia (0:470:16K and 0:170:09mmd1), and east Asia (0:460:20K and 0:150:06mmd1). Relatively large warming and wetting of the Arctic also occur at 0:590:36K and 0:040:02mmd1, respectively. Similar surface warming occurs in model simulations with aerosol-only mitigation, implying weak cooling due to ozone reductions. Our findings suggest that future policies that aggressively target non-methane NTCF reductions will improve air quality but will lead to additional surface warming, particularly in Asia and the Arctic. Policies that address other NTCFs including methane, as well as carbon dioxide emissions, must also be adopted to meet climate mitigation goals. © Author(s) 2020. This work is distributed under the Creative Commons Attribution 4.0 License.
- ItemRecommendations for reporting "black carbon" measurements(München : European Geopyhsical Union, 2013) Petzold, A.; Ogren, J.A.; Fiebig, M.; Laj, P.; Li, S.-M.; Baltensperger, U.; Holzer-Popp, T.; Kinne, S.; Pappalardo, G.; Sugimoto, N.; Wehrli, C.; Wiedensohler, A.; Zhang, X.-Y.Although black carbon (BC) is one of the key atmospheric particulate components driving climate change and air quality, there is no agreement on the terminology that considers all aspects of specific properties, definitions, measurement methods, and related uncertainties. As a result, there is much ambiguity in the scientific literature of measurements and numerical models that refer to BC with different names and based on different properties of the particles, with no clear definition of the terms. The authors present here a recommended terminology to clarify the terms used for BC in atmospheric research, with the goal of establishing unambiguous links between terms, targeted material properties and associated measurement techniques.