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    Atmospheric dust modeling from meso to global scales with the online NMMB/BSC-Dust model – Part 2: Experimental campaigns in Northern Africa
    (München : European Geopyhsical Union, 2012) Haustein, K.; Pérez, C.; Baldasano, J.M.; Jorba, O.; Basart, S.; Miller, R.L.; Janjic, Z.; Black, T.; Nickovic, S.; Todd, M.C.; Washington, R.; Müller, D.; Tesche, M.; Weinzierl, B.; Esselborn, M.; Schladitz, A.
    The new NMMB/BSC-Dust model is intended to provide short to medium-range weather and dust forecasts from regional to global scales. It is an online model in which the dust aerosol dynamics and physics are solved at each model time step. The companion paper (Pérez et al., 2011) develops the dust model parameterizations and provides daily to annual evaluations of the model for its global and regional configurations. Modeled aerosol optical depth (AOD) was evaluated against AERONET Sun photometers over Northern Africa, Middle East and Europe with correlations around 0.6–0.7 on average without dust data assimilation. In this paper we analyze in detail the behavior of the model using data from the Saharan Mineral dUst experiment (SAMUM-1) in 2006 and the Bodélé Dust Experiment (BoDEx) in 2005. AOD from satellites and Sun photometers, vertically resolved extinction coefficients from lidars and particle size distributions at the ground and in the troposphere are used, complemented by wind profile data and surface meteorological measurements. All simulations were performed at the regional scale for the Northern African domain at the expected operational horizontal resolution of 25 km. Model results for SAMUM-1 generally show good agreement with satellite data over the most active Saharan dust sources. The model reproduces the AOD from Sun photometers close to sources and after long-range transport, and the dust size spectra at different height levels. At this resolution, the model is not able to reproduce a large haboob that occurred during the campaign. Some deficiencies are found concerning the vertical dust distribution related to the representation of the mixing height in the atmospheric part of the model. For the BoDEx episode, we found the diurnal temperature cycle to be strongly dependant on the soil moisture, which is underestimated in the NCEP analysis used for model initialization. The low level jet (LLJ) and the dust AOD over the Bodélé are well reproduced. The remaining negative AOD bias (due to underestimated surface wind speeds) can be substantially reduced by decreasing the threshold friction velocity in the model.
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    Optimizing CALIPSO Saharan dust retrievals
    (München : European Geopyhsical Union, 2013) Amiridis, V.; Wandinger, U.; Marinou, E.; Giannakaki, E.; Tsekeri, A.; Basart, S.; Kazadzis, S.; Gkikas, A.; Taylor, M.; Baldasano, J.; Ansmann, A.
    We demonstrate improvements in CALIPSO (Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations) dust extinction retrievals over northern Africa and Europe when corrections are applied regarding the Saharan dust lidar ratio assumption, the separation of the dust portion in detected dust mixtures, and the averaging scheme introduced in the Level 3 CALIPSO product. First, a universal, spatially constant lidar ratio of 58 sr instead of 40 sr is applied to individual Level 2 dust-related backscatter products. The resulting aerosol optical depths show an improvement compared with synchronous and collocated AERONET (Aerosol Robotic Network) measurements. An absolute bias of the order of −0.03 has been found, improving on the statistically significant biases of the order of −0.10 reported in the literature for the original CALIPSO product. When compared with the MODIS (Moderate-Resolution Imaging Spectroradiometer) collocated aerosol optical depth (AOD) product, the CALIPSO negative bias is even less for the lidar ratio of 58 sr. After introducing the new lidar ratio for the domain studied, we examine potential improvements to the climatological CALIPSO Level 3 extinction product: (1) by introducing a new methodology for the calculation of pure dust extinction from dust mixtures and (2) by applying an averaging scheme that includes zero extinction values for the nondust aerosol types detected. The scheme is applied at a horizontal spatial resolution of 1° × 1° for ease of comparison with the instantaneous and collocated dust extinction profiles simulated by the BSC-DREAM8b dust model. Comparisons show that the extinction profiles retrieved with the proposed methodology reproduce the well-known model biases per subregion examined. The very good agreement of the proposed CALIPSO extinction product with respect to AERONET, MODIS and the BSC-DREAM8b dust model makes this dataset an ideal candidate for the provision of an accurate and robust multiyear dust climatology over northern Africa and Europe.
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    Satellite retrievals of dust aerosol over the Red Sea and the Persian Gulf (2005-2015)
    (Katlenburg-Lindau : EGU, 2017) Banks, Jamie R.; Brindley, Helen E.; Stenchikov, Georgiy; Schepanski, Kerstin
    The inter-annual variability of the dust aerosol presence over the Red Sea and the Persian Gulf is analysed over the period 2005-2015. Particular attention is paid to the variation in loading across the Red Sea, which has previously been shown to have a strong, seasonally dependent latitudinal gradient. Over the 11 years considered, the July mean 630 nm aerosol optical depth (AOD) derived from the Spinning Enhanced Visible and InfraRed Imager (SEVIRI) varies between 0.48 and 1.45 in the southern half of the Red Sea. In the north, the equivalent variation is between 0.22 and 0.66. The temporal and spatial pattern of variability captured by SEVIRI is also seen in AOD retrievals from the MODerate Imaging Spectroradiometer (MODIS), but there is a systematic offset between the two records. Comparisons of both sets of retrievals with ship-and land-based AERONET measurements show a high degree of correlation with biases of <0.08. However, these comparisons typically only sample relatively low aerosol loadings. When both records are stratified by AOD retrievals from the Multi-angle Imaging SpectroRadiometer (MISR), opposing behaviour is revealed at high MISR AODs (>1), with offsets of C0.19 for MODIS and 0.06 for SEVIRI. Similar behaviour is also seen over the Persian Gulf. Analysis of the scattering angles at which retrievals from the SEVIRI and MODIS measurements are typically performed in these regions suggests that assumptions concerning particle sphericity may be responsible for the differences seen.
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    Measurement report: Balloon-borne in situ profiling of Saharan dust over Cyprus with the UCASS optical particle counter
    (Katlenburg-Lindau : European Geosciences Union, 2021) Kezoudi, Maria; Tesche, Matthias; Smith, Helen; Tsekeri, Alexandra; Baars, Holger; Dollner, Maximilian; Estellés, Víctor; Bühl, Johannes; Weinzierl, Bernadett; Ulanowski, Zbigniew; Müller, Detlef; Amiridis, Vassilis
    This paper presents measurements of mineral dust concentration in the diameter range from 0.4 to 14.0 µm with a novel balloon-borne optical particle counter, the Universal Cloud and Aerosol Sounding System (UCASS). The balloon launches were coordinated with ground-based active and passive remote-sensing observations and airborne in situ measurements with a research aircraft during a Saharan dust outbreak over Cyprus from 20 to 23 April 2017. The aerosol optical depth at 500 nm reached values up to 0.5 during that event over Cyprus, and particle number concentrations were as high as 50 cm−3 for the diameter range between 0.8 and 13.9 µm. Comparisons of the total particle number concentration and the particle size distribution from two cases of balloon-borne measurements with aircraft observations show reasonable agreement in magnitude and shape despite slight mismatches in time and space. While column-integrated size distributions from balloon-borne measurements and ground-based remote sensing show similar coarse-mode peak concentrations and diameters, they illustrate the ambiguity related to the missing vertical information in passive sun photometer observations. Extinction coefficient inferred from the balloon-borne measurements agrees with those derived from coinciding Raman lidar observations at height levels with particle number concentrations smaller than 10 cm−3 for the diameter range from 0.8 to 13.9 µm. An overestimation of the UCASS-derived extinction coefficient of a factor of 2 compared to the lidar measurement was found for layers with particle number concentrations that exceed 25 cm−3, i.e. in the centre of the dust plume where particle concentrations were highest. This is likely the result of a variation in the refractive index and the shape and size dependency of the extinction efficiency of dust particles along the UCASS measurements. In the future, profile measurements of the particle number concentration and particle size distribution with the UCASS could provide a valuable addition to the measurement capabilities generally used in field experiments that are focussed on the observation of coarse aerosols and clouds.
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    Profiling of Saharan dust from the Caribbean to western Africa-Part 1: Layering structures and optical properties from shipborne polarization/Raman lidar observations
    (Katlenburg-Lindau : EGU, 2017) Rittmeister, Franziska; Ansmann, Albert; Engelmann, Ronny; Skupin, Annett; Baars, Holger; Kanitz, Thomas; Kinne, Stefan
    We present final and quality-assured results of multiwavelength polarization/Raman lidar observations of the Saharan air layer (SAL) over the tropical Atlantic. Observations were performed aboard the German research vessel R/V Meteor during the 1-month transatlantic cruise from Guadeloupe to Cabo Verde over 4500 km from 61.5 to 20 W at 14-15 N in April-May 2013. First results of the shipborne lidar measurements, conducted in the framework of SALTRACE (Saharan Aerosol Long-range Transport and Aerosol-Cloud Interaction Experiment), were reported by Kanitz et al. (2014). Here, we present four observational cases representing key stages of the SAL evolution between Africa and the Caribbean in detail in terms of layering structures and optical properties of the mixture of predominantly dust and aged smoke in the SAL. We discuss to what extent the lidar results confirm the validity of the SAL conceptual model which describes the dust long-range transport and removal processes over the tropical Atlantic. Our observations of a clean marine aerosol layer (MAL, layer from the surface to the SAL base) confirm the conceptual model and suggest that the removal of dust from the MAL, below the SAL, is very efficient. However, the removal of dust from the SAL assumed in the conceptual model to be caused by gravitational settling in combination with large-scale subsidence is weaker than expected. To explain the observed homogenous (heightindependent) dust optical properties from the SAL base to the SAL top, from the African coast to the Caribbean, we have to assume that the particle sedimentation strength is reduced and dust vertical mixing and upward transport mechanisms must be active in the SAL. Based on lidar observations on 20 nights at different longitudes in May 2013, we found, on average, MAL and SAL layer mean values (at 532 nm) of the extinction-to-backscatter ratio (lidar ratio) of 17-5 sr (MAL) and 43±8 sr (SAL), of the particle linear depolarization ratio of 0:025±0:015 (MAL) and 0:19±0:09 (SAL), and of the particle extinction coefficient of 67±45Mm..1 (MAL) and 68±37Mm..1 (SAL). The 532 nm optical depth of the lofted SAL was found to be, on average, 0:15±0:13 during the ship cruise. The comparably low values of the SAL mean lidar ratio and depolarization ratio (compared to typical pure dust values of 50-60 sr and 0.3, respectively) in combination with backward trajectories indicate a smoke contribution to light extinction of the order of 20% during May 2013, at the end of the burning season in central-western Africa. 1.
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    Three-dimensional evolution of Saharan dust transport towards Europe based on a 9-year EARLINET-optimized CALIPSO dataset
    (Katlenburg-Lindau : EGU, 2017) Marinou, Eleni; Amiridis, Vassilis; Binietoglou, Ioannis; Tsikerdekis, Athanasios; Solomos, Stavros; Proestakis, Emannouil; Konsta, Dimitra; Papagiannopoulos, Nikolaos; Tsekeri, Alexandra; Vlastou, Georgia; Zanis, Prodromos; Balis, Dimitrios; Wandinger, Ulla; Ansmann, Albert
    In this study we use a new dust product developed using CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) observations and EARLINET (European Aerosol Research Lidar Network) measurements and methods to provide a 3-D multiyear analysis on the evolution of Saharan dust over North Africa and Europe. The product uses a CALIPSO L2 backscatter product corrected with a depolarization-based method to separate pure dust in external aerosol mixtures and a Saharan dust lidar ratio (LR) based on long-term EARLINET measurements to calculate the dust extinction profiles. The methodology is applied on a 9-year CALIPSO dataset (2007-2015) and the results are analyzed here to reveal for the first time the 3-D dust evolution and the seasonal patterns of dust over its transportation paths from the Sahara towards the Mediterranean and Continental Europe. During spring, the spatial distribution of dust shows a uniform pattern over the Sahara desert. The dust transport over the Mediterranean Sea results in mean dust optical depth (DOD) values up to 0.1. During summer, the dust activity is mostly shifted to the western part of the desert where mean DOD near the source is up to 0.6. Elevated dust plumes with mean extinction values between 10 and 75 Mm-1 are observed throughout the year at various heights between 2 and 6 km, extending up to latitudes of 40° N. Dust advection is identified even at latitudes of about 60° N, but this is due to rare events of episodic nature. Dust plumes of high DOD are also observed above the Balkans during the winter period and above northwest Europe during autumn at heights between 2 and 4 km, reaching mean extinction values up to 50 Mm-1. The dataset is considered unique with respect to its potential applications, including the evaluation of dust transport models and the estimation of cloud condensation nuclei (CCN) and ice nuclei (IN) concentration profiles. Finally, the product can be used to study dust dynamics during transportation, since it is capable of revealing even fine dynamical features such as the particle uplifting and deposition on European mountainous ridges such as the Alps and Carpathian Mountains.
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    Sun photometer retrievals of Saharan dust properties over Barbados during SALTRACE
    (Katlenburg-Lindau : EGU, 2019) Toledano, Carlos; Torres, Benjamín; Velasco-Merino, Cristian; Althausen, Dietrich; Groß, Silke; Wiegner, Matthias; Weinzierl, Bernadett; Gasteiger, Josef; Ansmann, Albert; González, Ramiro; Mateos, David; Farrel, David; Müller, Thomas; Haarig, Moritz; Cachorro, Victoria E.
    The Saharan Aerosol Long-Range Transport and Aerosol-Cloud-Interaction Experiment (SALTRACE) was devoted to the investigation of Saharan dust properties over the Caribbean. The campaign took place in June-July 2013. A wide set of ground-based and airborne aerosol instrumentation was deployed at the island of Barbados for a comprehensive experiment. Several sun photometers performed measurements during this campaign: two AERONET (Aerosol Robotic Network) Cimel sun photometers and the Sun and Sky Automatic Radiometer (SSARA). The sun photometers were co-located with the ground-based multi-wavelength lidars BERTHA (Backscatter Extinction lidar Ratio Temperature Humidity profiling Apparatus) and POLIS (Portable Lidar System). Aerosol properties derived from direct sun and sky radiance observations are analyzed, and a comparison with the co-located lidar and in situ data is provided. The time series of aerosol optical depth (AOD) allows identifying successive dust events with short periods in between in which the marine background conditions were observed. The moderate aerosol optical depth in the range of 0.3 to 0.6 was found during the dust periods. The sun photometer infrared channel at the 1640nm wavelength was used in the retrieval to investigate possible improvements to aerosol size retrievals, and it was expected to have a larger sensitivity to coarse particles. The comparison between column (aerosol optical depth) and surface (dust concentration) data demonstrates the connection between the Saharan Air Layer and the boundary layer in the Caribbean region, as is shown by the synchronized detection of the successive dust events in both datasets. However the differences of size distributions derived from sun photometer data and in situ observations reveal the difficulties in carrying out a column closure study. © 2019 All rights reserved.
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    The sensitivity of the colour of dust in MSG-SEVIRI Desert Dust infrared composite imagery to surface and atmospheric conditions
    (Göttingen : Copernicus GmbH, 2019) Banks, J.R.; Hünerbein, A.; Heinold, B.; Brindley, H.E.; Deneke, H.; Schepanski, K.
    Infrared "Desert Dust" composite imagery taken by the Spinning Enhanced Visible and InfraRed Imager (SEVIRI), onboard the Meteosat Second Generation (MSG) series of satellites above the equatorial East Atlantic, has been widely used for more than a decade to identify and track the presence of dust storms from and over the Sahara Desert, the Middle East, and southern Africa. Dust is characterised by distinctive pink colours in the Desert Dust false-colour imagery; however, the precise colour is influenced by numerous environmental properties, such as the surface thermal emissivity and skin temperature, the atmospheric water vapour content, the quantity and height of dust in the atmosphere, and the infrared optical properties of the dust itself. For this paper, simulations of SEVIRI infrared measurements and imagery have been performed using a modelling system, which combines dust concentrations simulated by the aerosol transport model COSMO-MUSCAT (COSMO: COnsortium for Small-scale MOdelling; MUSCAT: MUltiScale Chemistry Aerosol Transport Model) with radiative transfer simulations from the RTTOV (Radiative Transfer for TOVS) model. Investigating the sensitivity of the synthetic infrared imagery to the environmental properties over a 6-month summertime period from 2011 to 2013, it is confirmed that water vapour is a major control on the apparent colour of dust, obscuring its presence when the moisture content is high. Of the three SEVIRI channels used in the imagery (8.7, 10.8, and 12.0 μm), the channel at 10.8 μm has the highest atmospheric transmittance and is therefore the most sensitive to the surface skin temperature. A direct consequence of this sensitivity is that the background desert surface exhibits a strong diurnal cycle in colour, with light blue colours possible during the day and purple hues prevalent at night. In dusty scenes, the clearest pink colours arise from high-altitude dust in dry atmospheres. Elevated dust influences the dust colour primarily by reducing the contrast in atmospheric transmittance above the dust layer between the SEVIRI channels at 10.8 and 12.0 μm, thereby boosting red and pink colours in the imagery. Hence, the higher the dust altitude, the higher the threshold column moisture needed for dust to be obscured in the imagery: for a sample of dust simulated to have an aerosol optical depth (AOD) at 550 nm of 2-3 at an altitude of 3-4 km, the characteristic colour of the dust may only be impaired when the total column water vapour is particularly moist ('39 mm). Meanwhile, dust close to the surface (altitude < 1 km) is only likely to be apparent when the atmosphere is particularly dry and when the surface is particularly hot, requiring column moisture/13 mm and skin temperatures '314 K, and is highly unlikely to be apparent when the skin temperature is/300 K. Such low-altitude dust will regularly be almost invisible within the imagery, since it will usually be beneath much of the atmospheric water vapour column. It is clear that the interpretation of satellite-derived dust imagery is greatly aided by knowledge of the background environment.
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    Saharan dust contribution to the Caribbean summertime boundary layer - A lidar study during SALTRACE
    (München : European Geopyhsical Union, 2016) Groß, Silke; Gasteiger, Josef; Freudenthaler, Volker; Müller, Thomas; Sauer, Daniel; Toledano, Carlos; Ansmann, Albert
    Dual-wavelength lidar measurements with the small lidar system POLIS of the Ludwig-Maximilians-Universität München were performed during the SALTRACE experiment at Barbados in June and July 2013. Based on high-accuracy measurements of the linear depolarization ratio down to about 200 m above ground level, the dust volume fraction and the dust mass concentration within the convective marine boundary layer can be derived. Additional information from radiosonde launches at the ground-based measurement site provide independent information on the convective marine boundary layer height and the meteorological situation within the convective marine boundary layer. We investigate the lidar-derived optical properties, the lidar ratio and the particle linear depolarization ratio at 355 and 532 nm and find mean values of 0.04 (SD 0.03) and 0.05 (SD 0.04) at 355 and 532 nm, respectively, for the particle linear depolarization ratio, and (26 ± 5) sr for the lidar ratio at 355 and 532 nm. For the concentration of dust in the convective marine boundary layer we find that most values were between 20 and 50 µgm−3. On most days the dust contribution to total aerosol volume was about 30–40 %. Comparing the dust contribution to the column-integrated sun-photometer measurements we see a correlation between high dust contribution, high total aerosol optical depth and a low Angström exponent, and of low dust contribution with low total aerosol optical depth.
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    Optical properties of long-range transported Saharan dust over Barbados as measured by dual-wavelength depolarization Raman lidar measurements
    (München : European Geopyhsical Union, 2015) Groß, S.; Freudenthaler, V.; Schepanski, K.; Toledano, C.; Schäfler, A.; Ansmann, A.; Weinzierl, B.
    Dual-wavelength Raman and depolarization lidar observations were performed during the Saharan Aerosol Long-range Transport and Aerosol-Cloud interaction Experiment in Barbados in June and July 2013 to characterize the optical properties and vertical distribution of long-range transported Saharan dust after transport across the Atlantic Ocean. Four major dust events were studied during the measurements from 15 June to 13 July 2013 with aerosol optical depths at 532 nm of up to 0.6. The vertical aerosol distribution was characterized by a three-layer structure consisting of the boundary layer, the entrainment or mixing layer and the pure Saharan dust layer. The upper boundary of the pure dust layer reached up to 4.5 km in height. The contribution of the pure dust layer was about half of the total aerosol optical depth at 532 nm. The total dust contribution was about 50–70 % of the total aerosol optical depth at 532 nm. The lidar ratio within the pure dust layer was found to be wavelength independent with mean values of 53 ± 5 sr at 355 nm and 56 ± 7 sr at 532 nm. For the particle linear depolarization ratio, wavelength-independent mean values of 0.26 ± 0.03 at 355 nm and 0.27 ± 0.01 at 532 nm have been found.