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Now showing 1 - 6 of 6
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    Strong anisotropy of the electron-phonon interaction in NbP probed by magnetoacoustic quantum oscillations
    (Woodbury, NY : Inst., 2020) Schindler, Clemens; Gorbunov, Denis; Zherlitsyn, Sergei; Galeski, Stanislaw; Schmidt, Marcus; Wosnitza, Jochen; Gooth, Johannes
    In this study, we report on the observation of de Haas-van Alphen-type quantum oscillations (QOs) in the ultrasound velocity of NbP as well as "giant QOs"in the ultrasound attenuation in pulsed magnetic fields. The difference in the QO amplitude for different acoustic modes reveals a strong anisotropy of the effective deformation potential, which we estimate to be as high as 9eV for certain parts of the Fermi surface. Furthermore, the natural filtering of QO frequencies and the tracing of the individual Landau levels to the quantum limit allows for a more detailed investigation of the Fermi surface of NbP, as was previously achieved by means of analyzing QOs observed in magnetization or electrical resistivity. © 2020 authors. Published by the American Physical Society.
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    Predicting the orientation of magnetic microgel rods for soft anisotropic biomimetic hydrogels
    (Cambridge : RSC Publ., 2020) Rose, Jonas C.; Fölster, Maaike; Kivilip, Lukas; Gerardo-Nava, Jose L.; Jaekel, Esther E.; Gehlen, David B.; Rohlfs, Wilko; De Laporte, Laura
    Living multicellular organisms comprise a high degree of soft anisotropic tissues but the development of controlled artificial assembly processes to mimic them remains challenging. Therefore, injectable, polymeric, magneto-responsive microgel rods are fabricated to orient within a low magnetic field. The incorporated superparamagnetic nanoparticles induce local dipole moments, resulting in a total magnetic torque that endows microgels with different structural, mechanical, and biochemical properties. In this report, a predictive macroscopic model based on an ellipsoidal element dispersed in a Newtonian fluid is adjusted using experimental data, which enables the prediction of the orientation rate and the required magnetic field strength for various microgel design parameters and fluid viscosities. The ordered microgels are fixed by crosslinking of a surrounding hydrogel, and can be employed for a wide variety of applications where anisotropic composite hydrogels play a crucial role; for instance as adaptive materials or in biomedical applications, wherein the model predictions can reduce animal experiments. © 2019 The Royal Society of Chemistry.
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    Tunable chirality of noncentrosymmetric magnetic Weyl semimetals in rare-earth carbides
    ([London] : Nature Publishing Group, 2022) Ray, Rajyavardhan; Sadhukhan, Banasree; Richter, Manuel; Facio, Jorge I.; van den Brink, Jeroen
    Even if Weyl semimetals are characterized by quasiparticles with well-defined chirality, exploiting this experimentally is severely hampered by Weyl lattice fermions coming in pairs with opposite chirality, typically causing the net chirality picked up by experimental probes to vanish. Here, we show this issue can be circumvented in a controlled manner when both time-reversal- and inversion symmetry are broken. To this end, we investigate chirality disbalance in the carbide family RMC2 (R a rare-earth and M a transition metal), showing several members to be Weyl semimetals. Using the noncentrosymmetric ferromagnet NdRhC2 as an illustrating example, we show that an odd number of Weyl nodes can be stabilized at its Fermi surface by properly tilting its magnetization. The chiral configuration endows a topological phase transition as the Weyl node transitions across the Fermi sheets, which triggers interesting chiral electromagnetic responses. Further, the tilt direction determines the sign of the resulting net chirality, opening up a simple route to control its sign and strength.
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    Mueller matrix imaging microscope using dual continuously rotating anisotropic mirrors
    (Washington, DC : Soc., 2021) Ruder, Alexander; Wright, Brandon; Feder, Rene; Kilic, Ufuk; Hilfiker, Matthew; Schubert, Eva; Herzinger, Craig M.; Schubert, Mathias
    We demonstrate calibration and operation of a Mueller matrix imaging microscope using dual continuously rotating anisotropic mirrors for polarization state generation and analysis. The mirrors contain highly spatially coherent nanostructure slanted columnar titanium thin films deposited onto optically thick titanium layers on quartz substrates. The first mirror acts as polarization state image generator and the second mirror acts as polarization state image detector. The instrument is calibrated using samples consisting of laterally homogeneous properties such as straight-through-air, a clear aperture linear polarizer, and a clear aperture linear retarder waveplate. Mueller matrix images are determined for spatially varying anisotropic samples consisting of a commercially available (Thorlabs) birefringent resolution target and a spatially patterned titanium slanted columnar thin film deposited onto a glass substrate. Calibration and operation are demonstrated at a single wavelength (530 nm) only, while, in principle, the instrument can operate regardless of wavelength. We refer to this imaging ellipsometry configuration as rotating-anisotropic-mirror-sample-rotating-anisotropic-mirror ellipsometry (RAM-S-RAM-E).
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    Anisotropic fractal magnetic domain pattern in bulk Mn1.4PtSn
    (Woodbury, NY : Inst., 2020) Sukhanov, A.S.; Zuniga Cespedes, B.E.; Vir, P.; Cameron, A.S.; Heinemann, A.; Martin, N.; Chaboussant, G.; Kumar, V.; Milde, P.; Eng, L.M.; Felser, C.; Inosov, D.S.
    The tetragonal compound Mn1.4PtSn with D2d symmetry recently attracted attention as the first known material that hosts magnetic antiskyrmions, which differ from the skyrmions known so far by their internal structure. The latter have been found in a number of magnets with the chiral crystal structure. In previous works, the existence of antiskyrmions in Mn1.4PtSn was unambiguously demonstrated in real space by means of Lorentz transmission electron microscopy on thin-plate samples (∼100 nm thick). In the present study, we used small-angle neutron scattering and magnetic force microscopy to perform reciprocal- and real-space imaging of the magnetic texture of bulk Mn1.4PtSn single crystals at different temperatures and in applied magnetic field. We found that the magnetic texture in the bulk differs significantly from that of thin-plate samples. Instead of spin helices or an antiskyrmion lattice, we observe an anisotropic fractal magnetic pattern of closure domains in zero field above the spin-reorientation transition temperature, which transforms into a set of bubble domains in high field. Below the spin-reorientation transition temperature the strong in-plane anisotropy as well as the fractal self-affinity in zero field is gradually lost, while the formation of bubble domains in high field remains robust. The results of our study highlight the importance of dipole-dipole interactions in thin-plate samples for the stabilization of antiskyrmions and identify criteria which should guide the search for potential (anti)skyrmion host materials. Moreover, they provide consistent interpretations of the previously reported magnetotransport anomalies of the bulk crystals. © 2020 authors. Published by the American Physical Society. Published by the American Physical Society under the terms of the "https://creativecommons.org/licenses/by/4.0/"Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI. Open access publication funded by the Max Planck Society.
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    Benchmark study using a multi-scale, multi-methodological approach for the petrophysical characterization of reservoir sandstones
    (Göttingen : Copernicus Publ., 2021) Haruzi, Peleg; Katsman, Regina; Halisch, Matthias; Waldmann, Nicolas; Spiro, Baruch
    This paper presents a detailed description and evaluation of a multi-methodological petrophysical approach for the comprehensive multi-scale characterization of reservoir sandstones. The suggested methodology enables the identification of links between Darcy-scale permeability and an extensive set of geometrical, textural and topological rock descriptors quantified at the pore scale. This approach is applied to the study of samples from three consecutive sandstone layers of Lower Cretaceous age in northern Israel. These layers differ in features observed at the outcrop, hand specimen, petrographic microscope and micro-CT scales. Specifically, laboratory porosity and permeability measurements of several centimetre-sized samples show low variability in the quartz arenite (top and bottom) layers but high variability in the quartz wacke (middle) layer. The magnitudes of this variability are also confirmed by representative volume sizes and by anisotropy evaluations conducted on micro-CT-imaged 3-D pore geometries. Two scales of directional porosity variability are revealed in quartz arenite sandstone of the top layer: the pore size scale of ∼0.1 mm in all directions and ∼3.5 mm scale related to the occurrence of high- and low-porosity horizontal bands occluded by Fe oxide cementation. This millimetre-scale variability controls the laboratory-measured macroscopic rock permeability. More heterogeneous pore structures were revealed in the quartz wacke sandstone of the intermediate layer, which shows high inverse correlation between porosity and clay matrix in the vertical direction attributed to depositional processes and comprises an internal spatial irregularity. Quartz arenite sandstone of the bottom layer is homogenous and isotropic in the investigated domain, revealing porosity variability at a ∼0.1 mm scale, which is associated with the average pore size. Good agreement between the permeability upscaled from the pore-scale modelling and the estimates based on laboratory measurements is shown for the quartz arenite layers. The proposed multi-methodological approach leads to an accurate petrophysical characterization of reservoir sandstones with broad ranges of textural, topological and mineralogical characteristics and is particularly applicable for describing anisotropy and heterogeneity of sandstones on various rock scales. The results of this study also contribute to the geological interpretation of the studied stratigraphic units.