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- ItemLong-range magnetic order in the ~S=1/2 triangular lattice antiferromagnet KCeS2(Amsterdam : SciPost Foundation, 2020) Bastien, Gaël; Rubrecht, Bastian; Haeussler, Ellen; Schlender, Philipp; Zangeneh, Ziba; Avdoshenko, Stanislav; Sarkar, Rajib; Alfonsov, Alexey; Luther, Sven; Onykiienko, Yevhen A.; Walker, Helen C.; Kühne, Hannes; Grinenko, Vadim; Guguchia, Zurab; Kataev, Vladislav; Klauss, Hans-Henning; Hozoi, Liviu; van den Brink, Jeroen; Inosov, Dmytro S.; Büchner, Bernd; Wolter, Anja U.B.; Doert, ThomasRecently, several putative quantum spin liquid (QSL) states were discovered in ~S=1/2 rare-earth based triangular-lattice antiferromagnets (TLAF) with the delafossite structure. A way to clarify the origin of the QSL state in these systems is to identify ways to tune them from the putative QSL state towards long-range magnetic order. Here, we introduce the Ce-based TLAF KCeS2 and show via low-temperature specific heat and μSR investigations that it yields magnetic order below TN=0.38 K despite the same delafossite structure. We identify a well separated ~S=1/2 ground state for KCeS2 from inelastic neutron scattering and embedded-cluster quantum chemical calculations. Magnetization and electron spin resonance measurements on single crystals indicate a strong easy-plane g~factor anisotropy, in agreement with the ab initio calculations. Finally, our specific-heat studies reveal an in-plane anisotropy of the magnetic field-temperature phase diagram which may indicate anisotropic magnetic interactions in KCeS2.
- ItemCurvature induced magnonic crystal in nanowires(Amsterdam : SciPost Foundation, 2019) Korniienko, Anastasiia; Kravchuk, Volodymyr P.; Pylypovskyi, Oleksandr V.; Sheka, Denis D.; van den Brink, Jeroen; Gaididei, YuriA new type of magnonic crystals, curvature induced ones, is realized in ferromagnetic nanowires with periodically deformed shape. A magnon band structure of such crystal is fully determined by its curvature: the developed theory is well confirmed by simulations. An application to nanoscale spintronic devices with the geometrically tunable parameters is proposed, namely, to filter elements.
- ItemSimulating Floquet topological phases in static systems(Amsterdam : SciPost Foundation, 2021) Franca, Selma; Hassler, Fabian; Fulga, Ion CosmaWe show that scattering from the boundary of static, higher-order topological insulators (HOTIs) can be used to simulate the behavior of (time-periodic) Floquet topological insulators. We consider D-dimensional HOTIs with gapless corner states which are weakly probed by external waves in a scattering setup. We find that the unitary reflection matrix describing back-scattering from the boundary of the HOTI is topologically equivalent to a (D-1)-dimensional nontrivial Floquet operator. To characterize the topology of the reflection matrix, we introduce the concept of `nested' scattering matrices. Our results provide a route to engineer topological Floquet systems in the lab without the need for external driving. As benefit, the topological system does not to suffer from decoherence and heating.
- ItemQuantum dynamics in 1D lattice models with synthetic horizons(Amsterdam : SciPost Foundation, 2022) Morice, Corentin; Chernyavsky, Dmitry; van Wezel, Jasper; van den Brink, Jeroen; Moghaddam, AliWe investigate the wave packet dynamics and eigenstate localization in recently proposed generalized lattice models whose low-energy dynamics mimics a quantum field theory in (1+1)D curved spacetime with the aim of creating systems analogous to black holes. We identify a critical slowdown of zero-energy wave packets in a family of 1D tight-binding models with power-law variation of the hopping parameter, indicating the presence of a horizon. Remarkably, wave packets with non-zero energies bounce back and reverse direction before reaching the horizon. We additionally observe a power-law localization of all eigenstates, each bordering a region of exponential suppression. These forbidden regions dictate the closest possible approach to the horizon of states with any given energy. These numerical findings are supported by a semiclassical description of the wave packet trajectories, which are shown to coincide with the geodesics expected for the effective metric emerging from the considered lattice models in the continuum limit.
- ItemBridging nano-optics and condensed matter formalisms in a unified description of inelastic scattering of relativistic electron beams(Amsterdam : SciPost Foundation, 2021) Lourenço-Martins, Hugo; Lubk, Axel; Kociak, MathieuIn the last decades, the blossoming of experimental breakthroughs in the domain of electron energy loss spectroscopy (EELS) has triggered a variety of theoretical developments. Those have to deal with completely different situations, from atomically resolved phonon mapping to electron circular dichroism passing by surface plasmon mapping. All of them rely on very different physical approximations and have not yet been reconciled, despite early attempts to do so. As an effort in that direction, we report on the development of a scalar relativistic quantum electrodynamic (QED) approach of the inelastic scattering of fast electrons. This theory can be adapted to describe all modern EELS experiments, and under the relevant approximations, can be reduced to any of the last EELS theories. In that aim, we present in this paper the state of the art and the basics of scalar relativistic QED relevant to the electron inelastic scattering. We then give a clear relation between the two once antagonist descriptions of the EELS, the retarded green Dyadic, usually applied to describe photonic excitations and the quasi-static mixed dynamic form factor (MDFF), more adapted to describe core electronic excitations of material. We then use this theory to establish two important EELS-related equations. The first one relates the spatially resolved EELS to the imaginary part of the photon propagator and the incoming and outgoing electron beam wavefunction, synthesizing the most common theories developed for analyzing spatially resolved EELS experiments. The second one shows that the evolution of the electron beam density matrix is proportional to the mutual coherence tensor, proving that quite universally, the electromagnetic correlations in the target are imprinted in the coherence properties of the probing electron beam.
- ItemSixfold fermion near the Fermi level in cubic PtBi2(Amsterdam : SciPost Foundation, 2021) Thirupathaiah, Setti; Kushnirenko, Yevhen; Koepernik, Klaus; Piening, Boy Roman; Büchner, Bernd; Aswartham, Saicharan; van den Brink, Jeroen; Borisenko, Sergey; Fulga, Ion CosmaWe show that the cubic compound PtBi2, is a topological semimetal hosting a sixfold band touching point in close proximity to the Fermi level. Using angle-resolved photoemission spectroscopy, we map the bandstructure of the system, which is in good agreement with results from density functional theory. Further, by employing a low energy effective Hamiltonian valid close to the crossing point, we study the effect of a magnetic field on the sixfold fermion. The latter splits into a total of twenty Weyl cones for a Zeeman field oriented in the diagonal, [111] direction. Our results mark cubic PtBi2, as an ideal candidate to study the transport properties of gapless topological systems beyond Dirac and Weyl semimetals.
- ItemBulk-boundary-defect correspondence at disclinations in rotation-symmetric topological insulators and superconductors(Amsterdam : SciPost Foundation, 2021) Geier, Max; Fulga, Ion Cosma; Lau, AlexanderWe study a link between the ground-state topology and the topology of the lattice via the presence of anomalous states at disclinations -- topological lattice defects that violate a rotation symmetry only locally. We first show the existence of anomalous disclination states, such as Majorana zero-modes or helical electronic states, in second-order topological phases by means of Volterra processes. Using the framework of topological crystals to construct d-dimensional crystalline topological phases with rotation and translation symmetry, we then identify all contributions to (d−2)-dimensional anomalous disclination states from weak and first-order topological phases. We perform this procedure for all Cartan symmetry classes of topological insulators and superconductors in two and three dimensions and determine whether the correspondence between bulk topology, boundary signatures, and disclination anomaly is unique.
- ItemEngineering spectral properties of non-interacting lattice Hamiltonians(Amsterdam : SciPost Foundation, 2021) Moghaddam, Ali G.; Chernyavsky, Dmitry; Morice, Corentin; van Wezel, Jasper; van den Brink, JeroenWe investigate the spectral properties of one-dimensional lattices with position-dependent hopping amplitudes and on-site potentials that are smooth bounded functions of the position. We find an exact integral form for the density of states (DOS) in the limit of an infinite number of sites, which we derive using a mixed Bloch-Wannier basis consisting of piecewise Wannier functions. Next, we provide an exact solution for the inverse problem of constructing the position-dependence of hopping in a lattice model yielding a given DOS. We confirm analytic results by comparing them to numerics obtained by exact diagonalization for various incarnations of position-dependent hoppings and on-site potentials. Finally, we generalize the DOS integral form to multi-orbital tight-binding models with longer-range hoppings and in higher dimensions.
- ItemStochastic field dynamics in models of spontaneous unitarity violation(Amsterdam : SciPost Foundation, 2024) Mertens, Lotte; Wesseling, Matthijs; van Wezel, JasperObjective collapse theories propose a solution to the quantum measurement problem by predicting deviations from Schrödinger's equation that can be tested experimentally. A class of objective theories based on spontaneous unitarity violation was recently introduced, in which the stochastic field required for obtaining Born's rule does not depend on the state of the system being measured. Here, we classify possible models for the stochastic field dynamics in theories of spontaneous unitarity violation. We show that for correlated stochastic dynamics, the field must be defined on a closed manifold. In two or more dimensions, it is then always possible to find stochastic dynamics yielding Born's rule, independent of the state being measured or the correlation time of the stochastic field. We show that the models defined this way are all isomorphic to the definition on a two-sphere, which we propose to be a minimal physical model for the stochastic field in models of spontaneous unitarity violation.
- ItemEngineering a pure Dirac regime in ZrTe5(Amsterdam : SciPost Foundation, 2023) Facio, Jorge I.; Nocerino, Elisabetta; Fulga, Ion Cosma; Wawrzynczak, Rafal; Brown, Joanna; Gu, Genda; Li, Qiang; Mansson, Martin; Sassa, Yasmine; Ivashko, Oleh; von Zimmermann, Martin; Mende, Felix; Gooth, Johannes; Galeski, Stanislaw; van den Brink, Jeroen; Meng, TobiasReal-world topological semimetals typically exhibit Dirac and Weyl nodes that coexist with trivial Fermi pockets. This tends to mask the physics of the relativistic quasiparticles. Using the example of ZrTe5, we show that strain provides a powerful tool for in-situ tuning of the band structure such that all trivial pockets are pushed far away from the Fermi energy, but only for a certain range of Van der Waals gaps. Our results naturally reconcile contradicting reports on the presence or absence of additional pockets in ZrTe5, and provide a clear map of where to find a pure three-dimensional Dirac semimetallic phase in the structural parameter space of the material.