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- ItemInvestigation of an Ablation-dominated Arc in a Model Chamber by Optical Emission Spectroscopy(Praha : Czech Technical University in Prague, Faculty of Electrical Engineering, Department of Physics, 2017) Methling, R.; Khakpour, A.; Wetzeler, S.; Uhrlandt, D.A switching arc in a model chamber is investigated by means of optical emission spectroscopy. Ignition wire is applied to initiate an arc of several kiloampere between tungsten−copper electrodes. Radiation emitted by the arc plasma is absorbed by a surrounding PTFE nozzle, leading to an ablation–dominated discharge. Video spectroscopy is carried out using an imaging spectrometer combined with a high–speed video camera. Carbon ion and fluorine atom line emission from the heating channel as well as copper, oxygen and nitrogen from ignition wire and ambient air are analyzed with focus on the low–current phases at the beginning of discharge and near current zero. Additionally, electrical parameters and total pressure are recorded while the general behavior of the discharge is observed by another video camera. Considering rotational symmetry of the arc the corresponding radial emission coefficients are determined. Finally, radial temperature profiles are calculated.
- ItemTime-reversal symmetry breaking type-II Weyl state in YbMnBi2(London : Nature Publishing Group, 2019) Borisenko, S.; Evtushinsky, D.; Gibson, Q.; Yaresko, A.; Koepernik, K.; Kim, T.; Ali, M.; van den Brink, J.; Hoesch, M.; Fedorov, A.; Haubold, E.; Kushnirenko, Y.; Soldatov, I.; Schäfer, R.; Cava, R.J.Spectroscopic detection of Dirac and Weyl fermions in real materials is vital for both, promising applications and fundamental bridge between high-energy and condensed-matter physics. While the presence of Dirac and noncentrosymmetric Weyl fermions is well established in many materials, the magnetic Weyl semimetals still escape direct experimental detection. In order to find a time-reversal symmetry breaking Weyl state we design two materials and present here experimental and theoretical evidence of realization of such a state in one of them, YbMnBi2. We model the time-reversal symmetry breaking observed by magnetization and magneto-optical microscopy measurements by canted antiferromagnetism and find a number of Weyl points. Using angle-resolved photoemission, we directly observe two pairs of Weyl points connected by the Fermi arcs. Our results not only provide a fundamental link between the two areas of physics, but also demonstrate the practical way to design novel materials with exotic properties.
- ItemTailor-made nanostructures bridging chaos and order for highly efficient white organic light-emitting diodes(London : Nature Publishing Group, 2019) Li, Y.; Kovačič, M.; Westphalen, J.; Oswald, S.; Ma, Z.; Hänisch, C.; Will, P.-A.; Jiang, L.; Junghaehnel, M.; Scholz, R.; Lenk, S.; Reineke, S.Organic light-emitting diodes (OLEDs) suffer from notorious light trapping, resulting in only moderate external quantum efficiencies. Here, we report a facile, scalable, lithography-free method to generate controllable nanostructures with directional randomness and dimensional order, significantly boosting the efficiency of white OLEDs. Mechanical deformations form on the surface of poly(dimethylsiloxane) in response to compressive stress release, initialized by reactive ions etching with periodicity and depth distribution ranging from dozens of nanometers to micrometers. We demonstrate the possibility of independently tuning the average depth and the dominant periodicity. Integrating these nanostructures into a two-unit tandem white organic light-emitting diode, a maximum external quantum efficiency of 76.3% and a luminous efficacy of 95.7 lm W−1 are achieved with extracted substrate modes. The enhancement factor of 1.53 ± 0.12 at 10,000 cd m−2 is obtained. An optical model is built by considering the dipole orientation, emitting wavelength, and the dipole position on the sinusoidal nanotexture.
- ItemObservation of giant spin-split Fermi-arc with maximal Chern number in the chiral topological semimetal PtGa(London : Nature Publishing Group, 2020) Yao, M.; Manna, K.; Yang, Q.; Fedorov, A.; Voroshnin, V.; Valentin Schwarze, B.; Hornung, J.; Chattopadhyay, S.; Sun, Z.; Guin, S.N.; Wosnitza, J.; Borrmann, H.; Shekhar, C.; Kumar, N.; Fink, J.; Sun, Y.; Felser, C.Non-symmorphic chiral topological crystals host exotic multifold fermions, and their associated Fermi arcs helically wrap around and expand throughout the Brillouin zone between the high-symmetry center and surface-corner momenta. However, Fermi-arc splitting and realization of the theoretically proposed maximal Chern number rely heavily on the spin-orbit coupling (SOC) strength. In the present work, we investigate the topological states of a new chiral crystal, PtGa, which has the strongest SOC among all chiral crystals reported to date. With a comprehensive investigation using high-resolution angle-resolved photoemission spectroscopy, quantum-oscillation measurements, and state-of-the-art ab initio calculations, we report a giant SOC-induced splitting of both Fermi arcs and bulk states. Consequently, this study experimentally confirms the realization of a maximal Chern number equal to ±4 in multifold fermionic systems, thereby providing a platform to observe large-quantized photogalvanic currents in optical experiments.
- ItemNitric oxide density distributions in the effluent of an RF argon APPJ: Effect of gas flow rate and substrate(Bristol : IOP, 2014) Iseni, S.; Zhang, S.; Van Gessel, A.F.H.; Hofmann, S.; Van Ham, B.T.J.; Reuter, S.; Weltmann, K.-D.; Bruggeman, P.J.The effluent of an RF argon atmospheric pressure plasma jet, the so-called kinpen, is investigated with focus on the nitric-oxide (NO) distribution for laminar and turbulent flow regimes. An additional dry air gas curtain is applied around the plasma effluent to prevent interaction with the ambient humid air. By means of laser-induced fluorescence (LIF) the absolute spatially resolved NO density is measured as well as the rotational temperature and the air concentration. While in the laminar case, the transport of NO is attributed to thermal diffusion; in the turbulent case, turbulent mixing is responsible for air diffusion. Additionally, measurements with a molecular beam mass-spectrometer (MBMS) absolutely calibrated for NO are performed and compared with the LIF measurements. Discrepancies are explained by the contribution of the NO2 and N2O to the MBMS NO signal. Finally, the effect of a conductive substrate in front of the plasma jet on the spatial distribution of NO and air diffusion is also investigated.
- ItemMulti-watt, multi-octave, mid-infrared femtosecond source(Washington D.C. : AAAS, 2018) Seidel, Marcus; Xiao, Xiao; Hussain, Syed A.; Arisholm, Gunnar; Hartung, Alexander; Zawilski, Kevin T.; Schunemann, Peter G.; Habel, Florian; Trubetskov, Michael; Pervak, Vladimir; Pronin, Oleg; Krausz, FerencSpectroscopy in the wavelength range from 2 to 11 μm (900 to 5000 cm−1) implies a multitude of applications in fundamental physics, chemistry, as well as environmental and life sciences. The related vibrational transitions, which all infrared-active small molecules, the most common functional groups, as well as biomolecules like proteins, lipids, nucleic acids, and carbohydrates exhibit, reveal information about molecular structure and composition. However, light sources and detectors in the mid-infrared have been inferior to those in the visible or near-infrared, in terms of power, bandwidth, and sensitivity, severely limiting the performance of infrared experimental techniques. This article demonstrates the generation of femtosecond radiation with up to 5 W at 4.1 μm and 1.3 W at 8.5 μm, corresponding to an order-of-magnitude average power increase for ultrafast light sources operating at wavelengths longer than 5 μm. The presented concept is based on power-scalable near-infrared lasers emitting at a wavelength near 1 μm, which pump optical parametric amplifiers. In addition, both wavelength tunability and supercontinuum generation are reported, resulting in spectral coverage from 1.6 to 10.2 μm with power densities exceeding state-of-the-art synchrotron sources over the entire range. The flexible frequency conversion scheme is highly attractive for both up-conversion and frequency comb spectroscopy, as well as for a variety of time-domain applications.Spectroscopy in the wavelength range from 2 to 11 μm (900 to 5000 cm−1) implies a multitude of applications in fundamental physics, chemistry, as well as environmental and life sciences. The related vibrational transitions, which all infrared-active small molecules, the most common functional groups, as well as biomolecules like proteins, lipids, nucleic acids, and carbohydrates exhibit, reveal information about molecular structure and composition. However, light sources and detectors in the mid-infrared have been inferior to those in the visible or near-infrared, in terms of power, bandwidth, and sensitivity, severely limiting the performance of infrared experimental techniques. This article demonstrates the generation of femtosecond radiation with up to 5 W at 4.1 μm and 1.3 W at 8.5 μm, corresponding to an order-of-magnitude average power increase for ultrafast light sources operating at wavelengths longer than 5 μm. The presented concept is based on power-scalable near-infrared lasers emitting at a wavelength near 1 μm, which pump optical parametric amplifiers. In addition, both wavelength tunability and supercontinuum generation are reported, resulting in spectral coverage from 1.6 to 10.2 μm with power densities exceeding state-of-the-art synchrotron sources over the entire range. The flexible frequency conversion scheme is highly attractive for both up-conversion and frequency comb spectroscopy, as well as for a variety of time-domain applications.
- ItemTerahertz quantum-cascade lasers for spectroscopic applications(Berlin : Technische Universität Berlin, 2018) Röben, Benjamin Malte; Grahn, Holger T.Terahertz (THz) quantum-cascade lasers (QCLs) are unipolar semiconductor heterostructure lasers that emit in the far-infrared spectral range. They are very attractive radiation sources for spectroscopy, since they are very compact and exhibit typical output powers of severalmWas well as linewidths in the MHz to kHz range. This thesis presents the development of methods to tailor the emission characteristics of THz QCLs and employ them for spectroscopy with highest resolution and sensitivity. In many cases, these spectroscopic applications require that the far-field distribution of the THz QCLs exhibits only a single lobe. However, multiple lobes in the far-field distribution of THz QCLs were experimentally observed, which were unambiguously attributed to the typically employed mounting geometry and to the cryogenic operation environment such as the optical window. Based on these results, a method to obtain a single-lobed far-field distribution is demonstrated. A critical requirement to employ a THz QCL for high-resolution spectroscopy of a single absorption or emission line is the precise control of its emission frequency. This long-standing problem is solved by a newly developed technique relying on the mechanical polishing of the front facet. A QCL fabricated in this manner allows for spectroscopy at a maximal resolution in the MHz to kHz range, but its accessible bandwidth is usually limited to a few GHz. In contrast, a newly developed method to utilize QCLs as sources for THz Fourier transform spectrometers enables highly sensitive spectroscopy over a significantly larger bandwidth of at least 72 GHz with a maximal resolution of typically 100 MHz. The application of QCLs as sources for THz Fourier transform spectroscopy leads to a signal-to-noise ratio and dynamic range that is substantially increased by a factor of 10 to 100 as compared to conventional sources. The results presented in this thesis pave the way to routinely employ THz QCLs for spectroscopic applications in the near future.