3 results
Search Results
Now showing 1 - 3 of 3
- ItemThe Pagami Creek smoke plume after long-range transport to the upper troposphere over Europe – Aerosol properties and black carbon mixing state(München : European Geopyhsical Union, 2014) Dahlkötter, F.; Gysel, M.; Sauer, D.; Minikin, A.; Baumann, R.; Seifert, P.; Ansmann, A.; Fromm, M.; Voigt, C.; Weinzierl, B.During the CONCERT 2011 field experiment with the DLR research aircraft Falcon, an enhanced aerosol layer with particle linear depolarization ratios of 6–8% at 532 nm was observed at altitudes above 10 km over northeast Germany on 16 September 2011. Dispersion simulations with HYSPILT suggest that the elevated aerosol layer originated from the Pagami Creek forest fire in Minnesota, USA, which caused pyro-convective uplift of particles and gases. The 3–4 day-old smoke plume had high total refractory black carbon (rBC) mass concentrations of 0.03–0.35 μg m−3 at standard temperature and pressure (STP) with rBC mass equivalent diameter predominantly smaller than 130 nm. Assuming a core-shell particle structure, the BC cores exhibit very thick (median: 105–136 nm) BC-free coatings. A large fraction of the BC-containing particles disintegrated into a BC-free fragment and a BC fragment while passing through the laser beam of the Single Particle Soot Photometer (SP2). In this study, the disintegration is a result of very thick coatings around the BC cores. This is in contrast to a previous study in a forest-fire plume, where it was hypothesized to be a result of BC cores being attached to a BC-free particle. For the high-altitude forest-fire aerosol layer observed in this study, increased mass specific light-absorption cross sections of BC can be expected due to the very thick coatings around the BC cores, while this would not be the case for the attached-type morphology. We estimate the BC mass import from the Pagami Creek forest fire into the upper troposphere/lower stratosphere (UTLS) region (best estimate: 25 Mg rBC). A comparison to black carbon emission rates from aviation underlines the importance of pyro-convection on the BC load in the UTLS region. Our study provides detailed information on the microphysics and the mixing state of BC in the forest-fire aerosol layer in the upper troposphere that can be used to better understand and investigate the radiative impact of such upper tropospheric aerosol layers.
- ItemOn the efficiency of rocket-borne particle detection in the mesosphere(München : European Geopyhsical Union, 2007) Hedin, J.; Gumbel, J.; Rapp, M.Meteoric smoke particles have been proposed as a key player in the formation and evolution of mesospheric phenomena. Despite their apparent importance still very little is known about these particles. Important questions concern the smoke number density and size distribution as a function of altitude as well as the fraction of charged particles. Sounding rockets are used to measure smoke in situ, but aerodynamics has remained a major challenge. Basically, the small smoke particles tend to follow the gas flow around the payload rather than reaching the detector if aerodynamics is not considered carefully in the detector design. So far only indirect evidence for the existence of meteoric smoke has been available from measurements of heavy charge carriers. Quantitative ways are needed that relate these measured particle population to the atmospheric particle population. This requires in particular knowledge about the size-dependent, altitude-dependent and charge-dependent detection efficiency for a given instrument. In this paper, we investigate the aerodynamics for a typical electrostatic detector design. We first quantify the flow field of the background gas, then introduce particles in the flow field and determine their trajectories around the payload structure. We use two different models to trace particles in the flow field, a Continuous motion model and a Brownian motion model. Brownian motion is shown to be of basic importance for the smallest particles. Detection efficiencies are determined for three detector designs, including two with ventilation holes to allow airflow through the detector. Results from this investigation show that rocket-borne smoke detection with conventional detectors is largely limited to altitudes above 75 km. The flow through a ventilated detector has to be relatively large in order to significantly improve the detection efficiency.
- ItemDistribution of meteoric smoke - Sensitivity to microphysical properties and atmospheric conditions(München : European Geopyhsical Union, 2006) Megner, L.; Rapp, M.; Gumbel, J.Meteoroids entering the Earth's atmosphere experience strong deceleration and ablate, whereupon the resulting material is believed to re-condense to nanometre-size "smoke particles". These particles are thought to be of great importance for many middle atmosphere phenomena, such as noctilucent clouds, polar mesospheric summer echoes, metal layers, and heterogeneous chemistry. The properties and distribution of meteoric smoke depend on poorly known or highly variable factors such as the amount, composition and velocity of incoming meteoric material, the efficiency of coagulation, and the state and circulation of the atmosphere. This work uses a one-dimensional microphysical model to investigate the sensitivities of meteoric smoke properties to these poorly known or highly variable factors. The resulting uncertainty or variability of meteoric smoke quantities such as number density, mass density, and size distribution are determined. It is found that the two most important factors are the efficiency of the coagulation and background vertical wind. The seasonal variation of the vertical wind in the mesosphere implies strong global and temporal variations in the meteoric smoke distribution. This contrasts the simplistic picture of a homogeneous global meteoric smoke layer, which is currently assumed in many studies of middle atmospheric phenomena. In particular, our results suggest a very low number of nanometre-sized smoke particles at the summer mesopause where they are thought to serve as condensation nuclei for noctilucent clouds.