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- ItemThe influence of the baseline drift on the resulting extinction values of a cavity attenuated phase shift-based extinction monitor (CAPS PMex)(Katlenburg-Lindau : Copernicus, 2020) Pfeifer, Sascha; Müller, Thomas; Freedman, Andrew; Wiedensohler, AlfredThe effect of the baseline drift on the resulting extinction values of three cavity attenuated phase shift-based extinction monitors (CAPS PMex) with different wavelengths and the respective correlation with NO2 was analysed for an urban background station. A drift of more than 0.8 Mm−1min−1 was observed for ambient air, with high probability caused by traffic-emissions-driven changes in carrier gas composition. The baseline drift leads to characteristic measurement artefacts for particle extinction. Artificial particle extinction values of approximately 4 Mm−1 were observed using a baseline period of 5 min. These values can be even higher for longer baseline periods. Two methods are shown to minimize this effect. Modified continuous baseline values are calculated in a post-processing step using simple linear interpolation and cubic smoothing splines. Both methods are useful to reduce artefacts, although the use of cubic smoothing splines gives slightly better results. The extinction artefacts are diminished and the effective scattering of the resulting extinction values is reduced by about 50 %.
- ItemStabilizing effect of mélange buttressing on the marine ice-cliff instability of the West Antarctic Ice Sheet(Katlenburg-Lindau : Copernicus, 2022) Schlemm, Tanja; Feldmann, Johannes; Winkelmann, Ricarda; Levermann, AndersOwing to global warming and particularly high regional ocean warming, both Thwaites and Pine Island Glaciers in the Amundsen region of the Antarctic Ice Sheet could lose their buttressing ice shelves over time. We analyse the possible consequences using the parallel ice sheet model (PISM), applying a simple cliff-calving parameterization and an ice mélange-buttressing model. We find that the instantaneous loss of ice-shelf buttressing, due to enforced ice-shelf melting, initiates grounding-line retreat and triggers marine ice sheet instability (MISI). As a consequence, the grounding line progresses into the interior of the West Antarctic Ice Sheet and leads to a sea level contribution of 0.6m within 100a. By subjecting the exposed ice cliffs to cliff calving using our simplified parameterization, we also analyse marine ice cliff instability (MICI). In our simulations it can double or even triple the sea level contribution depending on the only loosely constrained parameter that determines the maximum cliff-calving rate. The speed of MICI depends on this upper bound of the calving rate, which is given by the ice mélange buttressing the glacier. However, stabilization of MICI may occur for geometric reasons. Because the embayment geometry changes as MICI advances into the interior of the ice sheet, the upper bound on calving rates is reduced and the progress of MICI is slowed down. Although we cannot claim that our simulations bear relevant quantitative estimates of the effect of ice-mélange buttressing on MICI, the mechanism has the potential to stop the instability. Further research is needed to evaluate its role for the past and future evolution of the Antarctic Ice Sheet.
- ItemAtomic oxygen number densities in the mesosphere–lower thermosphere region measured by solid electrolyte sensors onWADIS-2(Katlenburg-Lindau : Copernicus, 2019) Eberhart, Martin; Löhle, Stefan; Strelnikov, Boris; Hedin, Jonas; Khaplanov, Mikhail; Fasoulas, Stefanos; Gumbel, Jörg; Lübken, Franz-Josef; Rapp, MarkusAbsolute profiles of atomic oxygen number densities with high vertical resolution have been determined in the mesosphere-lower thermosphere (MLT) region from in situ measurements by several rocket-borne solid electrolyte sensors. The amperometric sensors were operated in both controlled and uncontrolled modes and with various orientations on the foredeck and aft deck of the payload. Calibration was based on mass spectrometry in a molecular beam containing atomic oxygen produced in a microwave discharge. The sensor signal is proportional to the number flux onto the electrodes, and the mass flow rate in the molecular beam was additionally measured to derive this quantity from the spectrometer reading. Numerical simulations provided aerodynamic correction factors to derive the atmospheric number density of atomic oxygen from the sensor data. The flight results indicate a preferable orientation of the electrode surface perpendicular to the rocket axis. While unstable during the upleg, the density profiles measured by these sensors show an excellent agreement with the atmospheric models and photometer results during the downleg of the trajectory. The high spatial resolution of the measurements allows for the identification of small-scale variations in the atomic oxygen concentration. © Author(s) 2019. This work is distributed under the Creative Commons Attribution 4.0 License.
- ItemCharacterization and first results from LACIS-T : a moist-air wind tunnel to study aerosol–cloud–turbulence interactions(Katlenburg-Lindau : Copernicus, 2020) Niedermeier, Dennis; Voigtländer, Jens; Schmalfuß, Silvio; Busch, Daniel; Schumacher, Jörg; Shaw, Raymond A.; Stratmann, FrankThe interactions between turbulence and cloud microphysical processes have been investigated primarily through numerical simulation and field measurements over the last 10 years. However, only in the laboratory we can be confident in our knowledge of initial and boundary conditions and are able to measure under statistically stationary and repeatable conditions. In the scope of this paper, we present a unique turbulent moist-air wind tunnel, called the Turbulent Leipzig Aerosol Cloud Interaction Simulator (LACIS-T) which has been developed at TROPOS in order to study cloud physical processes in general and interactions between turbulence and cloud microphysical processes in particular. The investigations take place under well-defined and reproducible turbulent and thermodynamic conditions covering the temperature range of warm, mixed-phase and cold clouds (25∘C>T>−40∘C ). The continuous-flow design of the facility allows for the investigation of processes occurring on small temporal (up to a few seconds) and spatial scales (micrometer to meter scale) and with a Lagrangian perspective. The here-presented experimental studies using LACIS-T are accompanied and complemented by computational fluid dynamics (CFD) simulations which help us to design experiments as well as to interpret experimental results. In this paper, we will present the fundamental operating principle of LACIS-T, the numerical model, and results concerning the thermodynamic and flow conditions prevailing inside the wind tunnel, combining both characterization measurements and numerical simulations. Finally, the first results are depicted from deliquescence and hygroscopic growth as well as droplet activation and growth experiments. We observe clear indications of the effect of turbulence on the investigated microphysical processes.
- ItemREMIND2.1: transformation and innovation dynamics of the energy-economic system within climate and sustainability limits(Katlenburg-Lindau : Copernicus, 2021) Baumstark, Lavinia; Bauer, Nico; Benke, Falk; Bertram, Christoph; Bi, Stephen; Gong, Chen Chris; Dietrich, Jan Philipp; Dirnaichner, Alois; Giannousakis, Anastasis; Hilaire, Jerome; Klein, David; Koch, Johannes; Leimbach, Marian; Levesque, Antoine; Madeddu, Silvia; Malik, Aman; Merfort, Anne; Merfort, Leon; Odenweller, Adrian; Pehl, Michaja; Pietzcker, Robert C.; Piontek, Franziska; Rauner, Sebastian; Rodrigues, Renato; Rottoli, Marianna; Schreyer, Felix; Schultes, Anselm; Soergel, Bjoern; Soergel, Dominika; Strefler, Jessica; Ueckerdt, Falko; Kriegler, Elmar; Luderer, GunnarThis paper presents the new and now open-source version 2.1 of the REgional Model of INvestments and Development (REMIND). REMIND, as an integrated assessment model (IAM), provides an integrated view of the global energy–economy–emissions system and explores self-consistent transformation pathways. It describes a broad range of possible futures and their relation to technical and socio-economic developments as well as policy choices. REMIND is a multiregional model incorporating the economy and a detailed representation of the energy sector implemented in the General Algebraic Modeling System (GAMS). It uses non-linear optimization to derive welfare-optimal regional transformation pathways of the energy-economic system subject to climate and sustainability constraints for the time horizon from 2005 to 2100. The resulting solution corresponds to the decentralized market outcome under the assumptions of perfect foresight of agents and internalization of external effects. REMIND enables the analyses of technology options and policy approaches for climate change mitigation with particular strength in representing the scale-up of new technologies, including renewables and their integration in power markets. The REMIND code is organized into modules that gather code relevant for specific topics. Interaction between different modules is made explicit via clearly defined sets of input and output variables. Each module can be represented by different realizations, enabling flexible configuration and extension. The spatial resolution of REMIND is flexible and depends on the resolution of the input data. Thus, the framework can be used for a variety of applications in a customized form, balancing requirements for detail and overall runtime and complexity.
- ItemThe Earth system model CLIMBER-X v1.0 – Part 1: Climate model description and validation(Katlenburg-Lindau : Copernicus, 2022) Willeit, Matteo; Ganopolski, Andrey; Robinson, Alexander; Edwards, Neil R.The newly developed fast Earth system model CLIMBER-X is presented. The climate component of CLIMBER-X consists of a 2.5-D semi-empirical statistical-dynamical atmosphere model, a 3-D frictional-geostrophic ocean model, a dynamic-thermodynamic sea ice model and a land surface model. All the model components are discretized on a regular lat-long grid with a horizontal resolution of 5 ° ×5 °. The model has a throughput of ° ∼ 10 000 simulation years per day on a single node with 16 CPUs on a high-performance computer and is designed to simulate the evolution of the Earth system on temporal scales ranging from decades to >100000 years. A comprehensive evaluation of the model performance for the present day and the historical period shows that CLIMBER-X is capable of realistically reproducing many observed climate characteristics, with results that generally lie within the range of state-of-the-art general circulation models. The analysis of model performance is complemented by a thorough assessment of climate feedbacks and model sensitivities to changes in external forcings and boundary conditions. Limitations and applicability of the model are critically discussed. CLIMBER-X also includes a detailed representation of the global carbon cycle and is coupled to an ice sheet model, which will be described in separate papers. CLIMBER-X is available as open-source code and is expected to be a useful tool for studying past climate changes and for the investigation of the long-term future evolution of the climate.
- ItemValidation of Aeolus wind products above the Atlantic Ocean(Katlenburg-Lindau : Copernicus, 2020) Baars, Holger; Herzog, Alina; Heese, Birgit; Ohneiser, Kevin; Hanbuch, Karsten; Hofer, Julian; Yin, Zhenping; Engelmann, Ronny; Wandinger, UllaIn August 2018, the first Doppler wind lidar in space called Atmospheric Laser Doppler Instrument (ALADIN) was launched on board the satellite Aeolus by the European Space Agency (ESA). Aeolus measures profiles of one horizontal wind component (i.e., mainly the west-east direction) in the troposphere and lower stratosphere on a global basis. Furthermore, profiles of aerosol and cloud properties can be retrieved via the high spectral resolution lidar (HSRL) technique. The Aeolus mission is supposed to improve the quality of weather forecasts and the understanding of atmospheric processes. We used the opportunity to perform a unique validation of the wind products of Aeolus by utilizing the RV Polarstern cruise PS116 from Bremerhaven to Cape Town in November/December 2018. Due to concerted course modifications, six direct intersections with the Aeolus ground track could be achieved in the Atlantic Ocean west of the African continent. For the validation of the Aeolus wind products, we launched additional radiosondes and used the EARLINET/ACTRIS lidar Polly XT for atmospheric scene analysis. The six analyzed cases prove that Aeolus is able to measure horizontal wind speeds in the nearly west-east direction. Good agreements with the radiosonde observations could be achieved for both Aeolus wind products-the winds observed in clean atmospheric regions called Rayleigh winds and the winds obtained in cloud layers called Mie winds (according to the responsible scattering regime). Systematic and statistical errors of the Rayleigh winds were less than 1.5 and 3.3ms-1, respectively, when compared to radiosonde values averaged to the vertical resolution of Aeolus. For the Mie winds, a systematic and random error of about 1ms-1 was obtained from the six comparisons in different climate zones. However, it is also shown that the coarse vertical resolution of 2km in the upper troposphere, which was set in this early mission phase 2 months after launch, led to an underestimation of the maximum wind speed in the jet stream regions. In summary, promising first results of the first wind lidar space mission are shown and prove the concept of Aeolus for global wind observations. © 2020 Author(s).
- ItemShear-margin melting causes stronger transient ice discharge than ice-stream melting in idealized simulations(Katlenburg-Lindau : Copernicus, 2022) Feldmann, Johannes; Reese, Ronja; Winkelmann, Ricarda; Levermann, AndersBasal ice-shelf melting is the key driver of Antarctica's increasing sea-level contribution. In diminishing the buttressing force of the ice shelves that fringe the ice sheet, the melting increases the ice discharge into the ocean. Here we contrast the influence of basal melting in two different ice-shelf regions on the time-dependent response of an isothermal, inherently buttressed ice-sheet-shelf system. In the idealized numerical simulations, the basal-melt perturbations are applied close to the grounding line in the ice-shelf's (1) ice-stream region, where the ice shelf is fed by the fastest ice masses that stream through the upstream bed trough and (2) shear margins, where the ice flow is slower. The results show that melting below one or both of the shear margins can cause a decadal to centennial increase in ice discharge that is more than twice as large compared to a similar perturbation in the ice-stream region. We attribute this to the fact that melt-induced ice-shelf thinning in the central grounding-line region is attenuated very effectively by the fast flow of the central ice stream. In contrast, the much slower ice dynamics in the lateral shear margins of the ice shelf facilitate sustained ice-shelf thinning and thereby foster buttressing reduction. Regardless of the melt location, a higher melt concentration toward the grounding line generally goes along with a stronger response. Our results highlight the vulnerability of outlet glaciers to basal melting in stagnant, buttressing-relevant ice-shelf regions, a mechanism that may gain importance under future global warming.
- ItemCoupling framework (1.0) for the PISM (1.1.4) ice sheet model and the MOM5 (5.1.0) ocean model via the PICO ice shelf cavity model in an Antarctic domain(Katlenburg-Lindau : Copernicus, 2021) Kreuzer, Moritz; Reese, Ronja; Huiskamp, Willem Nicholas; Petri, Stefan; Albrecht, Torsten; Feulner, Georg; Winkelmann, RicardaThe past and future evolution of the Antarctic Ice Sheet is largely controlled by interactions between the ocean and floating ice shelves. To investigate these interactions, coupled ocean and ice sheet model configurations are required. Previous modelling studies have mostly relied on high-resolution configurations, limiting these studies to individual glaciers or regions over short timescales of decades to a few centuries. We present a framework to couple the dynamic ice sheet model PISM (Parallel Ice Sheet Model) with the global ocean general circulation model MOM5 (Modular Ocean Model) via the ice shelf cavity model PICO (Potsdam Ice-shelf Cavity mOdel). As ice shelf cavities are not resolved by MOM5 but are parameterized with the PICO box model, the framework allows the ice sheet and ocean components to be run at resolutions of 16 km and 3∘ respectively. This approach makes the coupled configuration a useful tool for the analysis of interactions between the Antarctic Ice Sheet and the global ocean over time spans of the order of centuries to millennia. In this study, we describe the technical implementation of this coupling framework: sub-shelf melting in the ice sheet component is calculated by PICO from modelled ocean temperatures and salinities at the depth of the continental shelf, and, vice versa, the resulting mass and energy fluxes from melting at the ice–ocean interface are transferred to the ocean component. Mass and energy fluxes are shown to be conserved to machine precision across the considered component domains. The implementation is computationally efficient as it introduces only minimal overhead. Furthermore, the coupled model is evaluated in a 4000 year simulation under constant present-day climate forcing and is found to be stable with respect to the ocean and ice sheet spin-up states. The framework deals with heterogeneous spatial grid geometries, varying grid resolutions, and timescales between the ice and ocean component in a generic way; thus, it can be adopted to a wide range of model set-ups.
- ItemApplication of TXRF in monitoring trace metals in particulate matter and cloud water(Katlenburg-Lindau : Copernicus, 2020) Fomba, Khanneh Wadinga; Deabji, Nabil; Barcha, Sayf El Islam; Ouchen, Ibrahim; Elbaramoussi, El Mehdi; El Moursli, Rajaa Cherkaoui; Harnafi, Mimoun; El Hajjaji, Souad; Mellouki, Abdelwahid; Herrmann, HartmutTrace metals in ambient particulate matter and cloud are considered key elements of atmospheric processes as they affect air quality, environmental ecosystems, and cloud formation. However, they are often available at trace concentrations in these media such that their analysis requires high-precision and sensitive techniques. In this study, different analytical methods were applied to quantify trace metals in particulate matter (PM) samples collected on quartz and polycarbonate filters as well as cloud water, using the Total reflection X-Ray Fluorescence (TXRF) technique. These methods considered the measurement of filter samples directly without and with chemical pretreatment. Direct measurements involved the analysis of PM samples collected on polycarbonate filters and cloud water samples after they are brought onto TXRF carrier substrates. The chemical treatment method involved the assessment of different acid digestion procedures on PM sampled on quartz filters. The solutions applied were reverse aqua regia, nitric acid, and a combination of nitric acid and hydrogen peroxide. The effect of cold-plasma treatment of samples on polycarbonate filters before TXRF measurements was also investigated. Digestion with the reverse aqua regia solution provided lower blanks and higher recovery in comparison to other tested procedures. The detection limits of the elements ranged from 0.3 to 44 ng cm−2. Ca, K, Zn, and Fe showed the highest detection limits of 44, 35, 6, and 1 ng cm−2, while As and Se had the lowest of 0.3 and 0.8 ng cm−2, respectively. The method showed higher recovery for most trace metals when applied to commercially available reference materials and field samples. TXRF measurements showed good agreement with results obtained from ion chromatography measurements for elements such as Ca and K. Cold-plasma treatment did not significantly lead to an increase in the detected concentration, and the results were element specific. Baking of the quartz filters prior to sampling showed a reduction of more than 20 % of the filter blanks for elements such as V, Sr, Mn, Zn, and Sb. The methods were applied successfully on ambient particulate matter and cloud water samples collected from the Atlas Mohammed V station in Morocco and the Cape Verde Atmospheric Observatory. The obtained concentrations were within the range reported using different techniques from similar remote and background regions elsewhere, especially for elements of anthropogenic origins such as V, Pb, and Zn with concentrations of up to 10, 19, and 28 ng m−3, respectively. Enrichment factor analysis indicated that crustal matter dominated the abundance of most of the elements, while anthropogenic activities also contributed to the abundance of elements such as Sb, Se, and Pb. The results confirm that TXRF is a useful complementary sensitive technique for trace metal analysis of particulate matter in the microgram range as well as in cloud water droplets.
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