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- ItemVerbundprojekt: Grundlegende Untersuchungen zu neuen Konzepten für Ultrakurzpuls-Laser, Teilvorhaben: Abstimmbare diodengepumpte Ultrakurzpulslaser im NIR (1.1-1.6[my]): Modensynchronisation von Cr4+-dotierten Festkörpermaterialien : Abschlußbericht(Berlin : Max-Born-Institut für Nichtlineare Optik und Kurzzeitspektroskopie, 2001) Noack, Frank; Jäger, Frank[no abstract available]
- ItemForscherverbund: German Israeli cooperation in ultrafast laser technologies (GILCULT) : Projekt: Femtosecond coherent control for nonlinear spectroscopy ; Abschlußbericht(Hannover : Technische Informationsbibliothek (TIB), 2004) Korn, G.; Silberberg, Yaron; Zhavoronkov, Nikolay; Laarmann, Tim[no abstract available]
- ItemSchlussbericht vom 10.08.2004 zum Thema: Verbundprojekt: Aufbau und Test eines Messstandes zur Untersuchung gespeicherter Nanopartikel mit Synchrotronstrahlung : bmb+f-Förderschwerpunkt Kondensierte Materie, Großgeräte der physikalischen Grundlagenforschung(Hannover : Technische Informationsbibliothek (TIB), 2004) Widdra, Wolf[no abstract available]
- ItemAn ultrashort X-ray emission from gas clusters irradiated by ultrashort laser pulses : final report for the project FST-D-ISR-10 ; [Forscherverbund: German Israeli Cooperation in Ultrafast Laser Technologies (GILCULT)](Hannover : Technische Informationsbibliothek (TIB), 2004) MBI[no abstract available]
- ItemMikrooptische Dünnschicht-Komponenten zur Effizienzverbesserung der Kollimation von Diodenlaser-Arrays (MDK)(Berlin : Max-Born-Institut für Nichtlineare Optik und Kurzzeitspektroskopie, 2002) Nerreter, S.; Seewald, G.; Fischer, A.; Neumann, U.; Tischer, M.; Grunwald, R.[no abstract available]
- ItemKramers-Kronig relations and high order nonlinear susceptibilities(Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2011) Brée, Carsten; Demircan, Ayhan; Steinmeyer, GünterAs previous theoretical results recently revealed, a Kramers-Kronig transform of multiphoton absorption rates allows for a precise prediction on the dispersion of the nonlinear refractive index $n_2$ in the near IR. It was shown that this method allows to reproduce recent experimental results on the importance of the higher-order Kerr effect. Extending these results, the current manuscript provides the dispersion of $n_2$ for all noble gases in excellent agreement with reference data. It is furthermore established that the saturation and inversion of the nonlinear refractive index is highly dispersive with wavelength, which indicates the existence of different filamentation regimes. While shorter laser wavelengths favor the well-established plasma clamping regime, the influence of the higher-order Kerr effect dominates in the long wavelength regime.
- ItemCascaded self-compression of femtosecond pulses in filaments(Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2010) Brée, Carsten; Bethge, Jens; Skupin, Stefan; Demircan, Ayhan; Steinmeyer, GünterHighly nonlinear wave propagation scenarios hold the potential to serve for energy concentration or pulse duration reduction of the input wave form, provided that a small range of input parameters be maintained. In particular when phenomena like rogue-wave formation or few-cycle optical pulses generation come into play, it becomes increasingly difficult to maintain control of the waveforms. Here we suggest an alternative approach towards the control of waveforms in a highly nonlinear system. Cascading pulse self-compression cycles at reduced nonlinearity limits the increase of input parameter sensitivity while still enabling an enhanced compression effect. This cascaded method is illustrated by experiments and in numerical simulations of the Nonlinear Schrödinger Equation, simulating the propagation of short optical pulses in a self-generated plasma.
- ItemMethod for computing the nonlinear refractive index via Keldysh theory(Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2008) Brée, Carsten; Demircan, Ayhan; Steinmeyer, GünterBy making use of the multiphoton limit of Keldysh theory, we show that for the case of two-photon absorption a Kramers-Kronig expansion can be used to calculate the nonlinear refractive index for different wavelenghts. We apply this method to various inert gases and compare the obtained numerical values to different experimental and theoretical results for the dispersion of the Kerr nonlinearity.
- ItemFilamentary pulse self-compression : the impact of the cell windows(Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2011) Brée, Carsten; Demircan, Ayhan; Bethge, Jens; Nibbering, Erik T.J.; Skupin, Stefan; Bergé, Luc; Steinmeyer, GünterSelf-compression of multi-millijoule laser pulses during filamentary propagation is usually explained by the interplay of self-focusing and defocusing effects, causing a substantial concentration of energy on the axis of the propagating optical pulse. Recently, it has been argued that cell windows may play a decisive role in the self-compression mechanism. As such windows have to be used for media other than air their presence is often unavoidable, yet they present a sudden non-adiabatic change in dispersion and nonlinearity that should lead to a destruction of the temporal and spatial integrity of the light bullets generated in the self-compression mechanism. We now experimentally prove that there is in fact a self-healing mechanism that helps to overcome the potentially destructive consequences of the cell windows. We show in two carefully conducted experiments that the cell window position decisively influences activation or inhibition of the self-healing mechanism. A comparison with a windowless cell shows that presence of this mechanism is an important prerequisite for the exploitation of self-compression effects in windowed cells filled with inert gases.
- ItemNon-instantaneous polarization dynamics in dielectric media(Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2014) Hofmann, Michael; Hyyti, Janne; Birkholz, Simon; Bock, Martin; Das, Susanta K.; Grunwald, Rüdiger; Hoffmann, Mathias; Nagy, Tamas; Demircan, Ayhan; Jupé, Marco; Ristau, Detlev; Morgner, Uwe; Brée, Carsten; Woerner, Michael; Elsaesser, Thomas; Steinmeyer, GünterThird-order optical nonlinearities play a vital role for generation1,2 and characterization 3-5 of some of the shortest optical pulses to date, for optical switching applications6,7, and for spectroscopy8,9. In many cases, nonlinear optical effects are used far off resonance, and then an instantaneous temporal response is expected. Here, we show for the first time resonant frequency-resolved optical gating measurements1012 that indicate substantial nonlinear polarization relaxation times up to 6.5 fs in dielectric media, i.e., significantly beyond the shortest pulses directly available from commercial lasers. These effects are among the fastest effects observed in ultrafast spectroscopy. Numerical solutions of the time-dependent Schrödinger equation13,14 are in excellent agreement with experimental observations. The simulations indicate that pulse generation and characterization in the ultraviolet may be severely affected by this previously unreported effect. Moreover, our approach opens an avenue for application of frequency-resolved optical gating as a highly selective spectroscopic probe in high-field physics.
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