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Plasma induced pulse breaking in filamentary self-compression
A plasma induced temporal break-up in filamentary propagation has recently been identified as one of the key events in the temporal self-compression of femtosecond laser pulses. An analysis of the Nonlinear Schrödinger Equation coupled to a noninstantaneous plasma response yields a set of stationary states. This analysis clearly indicates that the emergence of double-hump, characteristically asymmetric temporal on-axis intensity profiles in regimes where plasma defocusing saturates the optical collapse caused by Kerr self-focusing is an inherent property of the underlying dynamical model.
Rogue wave formation by accelerated solitons at an optical event horizon
Rogue waves, by definition, are rare events of extreme amplitude, but at the same time they are frequent in the sense that they can exist in a wide range of physical contexts. While many mechanisms have been demonstrated to explain the appearance of rogue waves in various specific systems, there is no known generic mechanism or general set of criteria shown to rule their appearance. Presupposing only the existence of a nonlinear Schrödinger-type equation together with a concave dispersion profile around a zero dispersion wavelength we demonstrate that solitons may experience acceleration and strong reshaping due to the interaction with continuum radiation, giving rise to extreme-value phenomena. The mechanism is independent of the optical Raman effect. A strong increase of the peak power is accompanied by a mild increase of the pulse energy and carrier frequency, whereas the photon number of the soliton remains practically constant. This reshaping mechanism is particularly robust and is naturally given in optics in the supercontinuum generation process.
Method for computing the nonlinear refractive index via Keldysh theory
By making use of the multiphoton limit of Keldysh theory, we show that for the case of two-photon absorption a Kramers-Kronig expansion can be used to calculate the nonlinear refractive index for different wavelenghts. We apply this method to various inert gases and compare the obtained numerical values to different experimental and theoretical results for the dispersion of the Kerr nonlinearity.
Symmetry breaking and strong persistent plasma currents via resonant destabilization of atoms
The ionization rate of an atom in a strong optical field can be resonantly enhanced by the presence of long-living atomic levels (so called Freeman resonances). This process is most prominent in the multiphoton ionization regime meaning that ionization event takes many optical cycles. Nevertheless, here we show that these resonances can lead to fast subcycle-scale plasma buildup at the resonant values of the intensity in the pump pulse. The fast buildup can break the cycletocycle symmetry of the ionization process, resulting in generation of persistent macroscopic plasma currents which remain after the end of the pulse. This, in turn, gives rise to a broadband radiation of unusual spectral structure forming a comb from terahertz (THz) to visible. This radiation contains fingerprints of the attosecond electronic dynamics in Rydberg states during ionization.
Saturation of the all-optical Kerr effect
Saturation of the intensity dependence of the refractive index is directly computed from ionization rates via a Kramers-Kronig transform. The linear intensity dependence and its dispersion are found in excellent agreement with complete quantum mechanical orbital computations. Higher-order terms concur with solutions of the time-dependent Schrödinger equation. Expanding the formalism to all orders up to the ionization potential of the atom, we derive a model for saturation of the Kerr effect. This model widely confirms recently published and controversially discussed experimental data and corroborates the importance of higher-order Kerr terms for filamentation.
Modulation instability in filamentary self-compression
We numerically analyze filamentary propagation for various medium- and input pulse parameters and show that temporal self-compression can greatly benefit from refocusing events. Analyzing the dynamical behavior in the second focal spot, it turns out that a dispersive temporal break-up may appear due to the emission of a hyperbolic shock-wave from the self-steepened trailing edge of the pulse. This break-up event enhances the self-compression capabilities of laser filaments, enabling up to 12-fold temporal compression. Only slightly perturbing the input pulse parameters, we further identify a regime in which refocusing events give rise to extended subdiffractive propagation in a weakly ionized channel.
Ultrafast spatio-temporal dynamics of terahertz generation by ionizing two-color femtosecond pulses in gases
We present a combined theoretical and experimental study of spatio-temporal propagation effects in terahertz (THz) generation in gases using two-color ionizing laser pulses. The observed strong broadening of the THz spectra with increasing gas pressure reveals the prominent role of spatio-temporal reshaping and of a plasma-induced blue-shift of the pump pulses in the generation process. Results obtained from (3+1)-dimensional simulations are in good agreement with experimental findings and clarify the mechanisms responsible for THz emission.
Directionality of THz emission from photoinduced gas plasmas
Forward and backward THz emission by ionizing two-color laser pulses in gas is investigated by means of a simple semi-analytical model based on Jefimenko's equation and rigorous Maxwell simulations in one and two dimensions. We find the emission in backward direction having a much smaller spectral bandwidth than in forward direction and explain this by interference effects. Forward THz radiation is generated predominantly at the ionization front and is thus almost not affected by the opacity of the plasma, in excellent agreement with results obtained from a unidirectional pulse propagation model.
Kramers-Kronig relations and high order nonlinear susceptibilities
As previous theoretical results recently revealed, a Kramers-Kronig transform of multiphoton absorption rates allows for a precise prediction on the dispersion of the nonlinear refractive index $n_2$ in the near IR. It was shown that this method allows to reproduce recent experimental results on the importance of the higher-order Kerr effect. Extending these results, the current manuscript provides the dispersion of $n_2$ for all noble gases in excellent agreement with reference data. It is furthermore established that the saturation and inversion of the nonlinear refractive index is highly dispersive with wavelength, which indicates the existence of different filamentation regimes. While shorter laser wavelengths favor the well-established plasma clamping regime, the influence of the higher-order Kerr effect dominates in the long wavelength regime.
Tailoring THz radiation by controlling tunnel photoionization events in gases
Applications ranging from nonlinear terahertz spectroscopy to remote sensing require broadband and intense THz radiation which can be generated by focusing two-color laser pulses into a gas. In this setup, THz radiation originates from the buildup of the electron density in sharp steps of attosecond duration due to tunnel ionization, and subsequent acceleration of free electrons in the laser field. We show that the spectral shape of the THz pulses generated by this mechanism is determined by superposition of contributions from individual ionization events. This provides a straightforward analogy with linear diffraction theory, where the ionization events play the role of slits in a grating. This analogy offers simple explanations for recent experimental observations and opens new avenues for THz pulse shaping based on temporal control of the ionization events. We illustrate this novel technique by tailoring the spectral width and position of the resulting radiation using multi-color pump pulses.