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Dura, J.
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Hummert, J.
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Kornilov, O.
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Loriot, V.
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Lépine, F.
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Reitsma, G.
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Vrakking, M.J.J.
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cationic excitation energy
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electronic relaxation of molecules
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energy transfer
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Journal of physics: Conference Series 1412 (2020), Nr. 7
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Delayed relaxation of highly excited naphthalene cations
(
Bristol : IOP Publ.,
2020
)
Reitsma, G.
;
Hummert, J.
;
Dura, J.
;
Loriot, V.
;
Vrakking, M.J.J.
;
Lépine, F.
;
Kornilov, O.
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The efficiency of energy transfer in ultrafast electronic relaxation of molecules depends strongly on the complex interplay between electronic and nuclear motion. In this study we use wavelength-selected XUV pulses to induce relaxation dynamics of highly excited cationic states of naphthalene. Surprisingly, the observed relaxation lifetimes increase with the cationic excitation energy. We propose that this is a manifestation of a quantum mechanical population trapping that leads to delayed relaxation of molecules in the regions with a high density of excited states. © 2019 Published under licence by IOP Publishing Ltd.
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