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- ItemStripe-yzmagnetic order in the triangular-lattice antiferromagnet KCeS2(Bristol : IOP Publ., 2021) Kulbakov, Anton A.; Avdoshenko, Stanislav M.; Puente-Orench, Inés; Deeb, Mahmoud; Doerr, Mathias; Schlender, Philipp; Doert, Thomas; Inosov, Dmytro S.Yb- and Ce-based delafossites were recently identified as effective spin-1/2 antiferromagnets on the triangular lattice. Several Yb-based systems, such as NaYbO2, NaYbS2, and NaYbSe2, exhibit no long-range order down to the lowest measured temperatures and therefore serve as putative candidates for the realization of a quantum spin liquid. However, their isostructural Ce-based counterpart KCeS2 exhibits magnetic order below TN = 400 mK, which was so far identified only in thermodynamic measurements. Here we reveal the magnetic structure of this long-range ordered phase using magnetic neutron diffraction. We show that it represents the so-called 'stripe-yz' type of antiferromagnetic order with spins lying approximately in the triangular-lattice planes orthogonal to the nearest-neighbor Ce–Ce bonds. No structural lattice distortions are revealed below TN, indicating that the triangular lattice of Ce3+ ions remains geometrically perfect down to the lowest temperatures. We propose an effective Hamiltonian for KCeS2, based on a fit to the results of ab initio calculations, and demonstrate that its magnetic ground state matches the experimental spin structure.
- ItemMagnetism in curved geometries(Bristol : IOP Publ., 2016) Streubel, Robert; Fischer, Peter; Kronast, Florian; Kravchuk, Volodymyr P.; Sheka, Denis D.; Gaididei, Yuri; Schmidt, Oliver G.; Makarov, DenysExtending planar two-dimensional structures into the three-dimensional space has become a general trend in multiple disciplines, including electronics, photonics, plasmonics and magnetics. This approach provides means to modify conventional or to launch novel functionalities by tailoring the geometry of an object, e.g. its local curvature. In a generic electronic system, curvature results in the appearance of scalar and vector geometric potentials inducing anisotropic and chiral effects. In the specific case of magnetism, even in the simplest case of a curved anisotropic Heisenberg magnet, the curvilinear geometry manifests two exchange-driven interactions, namely effective anisotropy and antisymmetric exchange, i.e. Dzyaloshinskii–Moriya-like interaction. As a consequence, a family of novel curvature-driven effects emerges, which includes magnetochiral effects and topologically induced magnetization patterning, resulting in theoretically predicted unlimited domain wall velocities, chirality symmetry breaking and Cherenkov-like effects for magnons. The broad range of altered physical properties makes these curved architectures appealing in view of fundamental research on e.g. skyrmionic systems, magnonic crystals or exotic spin configurations. In addition to these rich physics, the application potential of three-dimensionally shaped objects is currently being explored as magnetic field sensorics for magnetofluidic applications, spin-wave filters, advanced magneto-encephalography devices for diagnosis of epilepsy or for energy-efficient racetrack memory devices. These recent developments ranging from theoretical predictions over fabrication of three-dimensionally curved magnetic thin films, hollow cylinders or wires, to their characterization using integral means as well as the development of advanced tomography approaches are in the focus of this review.
- ItemMagnetocaloric properties of multicomponent Laves phase compounds and their composites(Bristol : IOP Publ., 2021) Ćwik, J.; Koshkid’ko, Yu; Nenkov, K.; Kolchugina, N.Heat capacity measurements have been performed for multicomponent (Ho0.9Er0.1)1-xGdxCo2 compounds with x = 0.05, 0.1, and 0.15. The isothermal magnetic entropy change, ΔSmag, allowing the estimation of the magnetocaloric effect, was determined based on the heat capacity measurements in magnetic fields up to 2 T. A numerical method, with the magnetic entropy change of individual (Ho0.9Er0.1)1-xGdxCo2 compounds, was used to calculate the optimal molar composition of the constituents and the resulting change of the isothermal magnetic entropy of composite, ΔScomp. The results show that proposed composite can be considered as a refrigerant material in magnetic refrigerators performing an Ericsson cycle in a temperature range of 90-130 K.
- ItemSplitting of the magnetic monopole pair-creation energy in spin ice(Bristol : IOP Publ., 2020) Hornung, J.; Gottschall, T.; Opherden, L.; Antlauf, M.; Schwarz, M.; Kroke, E.; Herrmannsdörfer, T.; Wosnitza, J.The thermodynamics in spin-ice systems are governed by emergent magnetic monopole excitations and, until now, the creation of a pair of these topological defects was associated with one specific pair-creation energy. Here, we show that the electric dipole moments inherent to the magnetic monopoles lift the degeneracy of their creation process and lead to a splitting of the pair-creation energy. We consider this finding to extend the model of magnetic relaxation in spin-ice systems and show that an electric dipole interaction in the theoretically estimated order of magnitude leads to a splitting which can explain the controversially discussed discrepancies between the measured temperature dependence of the magnetic relaxation times and previous theory. By applying our extended model to experimental data of, various spin-ice systems, we show its universal applicability and determine a dependence of the electric dipole interaction on the system parameters, which is in accordance with the theoretical model of electric dipole formation. © 2020 The Author(s). Published by IOP Publishing Ltd.
- ItemOccurrence of Flux Jumps in MgB2 Bulk Magnets during Pulse-Field Magnetization(Bristol : IOP Publ., 2020) Sakai, N.; Oka, T.; Yamanaka, K.; Dadiel, L.; Oki, H.; Ogawa, J.; Fukui, S.; Scheiter, J.; Häßler, W.; Yokoyama, K; Noudem, J.; Miryala, M.; Murakami, M.The magnetic flux capturing of MgB2 bulk magnets made by spark plasma sintering process has been precisely investigated to clarify the mechanism of flux motions during the pulse-field magnetization processes. The field trapping ratio B T/B P was evaluated as a key parameter of field trapping ability which strongly relates to the heat generation due to the rapid flux motion in the samples. The time dependence of magnetic flux density revealed the actual flux motion which penetrated the samples. The trapped fields B T and field trapping ratios B T/B P of various samples were classified into three regions of 'no flux flow', 'fast flux flow' and 'flux jump' according to the generation of heat and its propagation. A flux jump was observed late at 280 ms from the beginning of PFM process, while the field penetration B P showed its peak at 10 ms. Considering the heat propagation speed, the long-delayed flux jump should be attributed to the macroscopic barriers against the heat propagation to the surface centre of bulk magnet. © Published under licence by IOP Publishing Ltd.
- ItemTransition to the quantum hall regime in InAs nanowire cross-junctions(Bristol : IOP Publ., 2019) Gooth, Johannes; Borg, Mattias; Schmid, Heinz; Bologna, Nicolas; Rossell, Marta D.; Wirths, Stephan; Moselund, Kirsten; Nielsch, Kornelius; Riel, HeikeWe present a low-temperature electrical transport study on four-terminal ballistic InAs nanowire cross-junctions in magnetic fields aligned perpendicular to the cross-plane. Two-terminal longitudinal conductance measurements between opposing contact terminals reveal typical 1D conductance quantization at zero magnetic field. As the magnetic field is applied, the 1D bands evolve into hybrid magneto-electric sub-levels that eventually transform into Landau levels for the widest nanowire devices investigated (width = 100 nm). Hall measurements in a four-terminal configuration on these devices show plateaus in the transverse Hall resistance at high magnetic fields that scale with (ve 2 /h) -1 . e is the elementary charge, h denotes Planck's constant and v is an integer that coincides with the Landau level index determined from the longitudinal conductance measurements. While the 1D conductance quantization in zero magnetic field is fragile against disorder at the NW surface, the plateaus in the Hall resistance at high fields remain robust as expected for a topologically protected Quantum Hall phase. © 2019 IOP Publishing Ltd.
- ItemPhotoluminescence investigation of strictly ordered Ge dots grown on pit-patterned Si substrates(Bristol : IOP Publ., 2015) Brehm, Moritz; Grydlik, Martyna; Tayagaki, Takeshi; Langer, Gregor; Schäffler, Friedrich; Schmidt, Oliver G.We investigate the optical properties of ordered Ge quantum dots (QDs) by means of micro-photoluminescence spectroscopy (PL). These were grown on pit-patterned Si(001) substrates with a wide range of pit-periods and thus inter QD-distances (425–3400 nm). By exploiting almost arbitrary inter-QD distances achievable in this way we are able to choose the number of QDs that contribute to the PL emission in a range between 70 and less than three QDs. This well-defined system allows us to clarify, by PL-investigation, several points which are important for the understanding of the formation and optical properties of ordered QDs. We directly trace and quantify the amount of Ge transferred from the surrounding wetting layer (WL) to the QDs in the pits. Moreover, by exploiting different pit-shapes, we reveal the role of strain-induced activation energy barriers that have to be overcome for charge carriers generated outside the dots. These need to diffuse between the energy minimum of the WL in and between the pits, and the one in the QDs. In addition, we demonstrate that the WL in the pits is already severely intermixed with Si before upright QDs nucleate, which further enhances intermixing of ordered QDs as compared to QDs grown on planar substrates. Furthermore, we quantitatively determine the amount of Ge transferred by surface diffusion through the border region between planar and patterned substrate. This is important for the growth of ordered islands on patterned fields of finite size. We highlight that the Ge WL-facets in the pits act as PL emission centres, similar to upright QDs.
- ItemImpact of Mn-Pn intermixing on magnetic properties of an intrinsic magnetic topological insulator: the µSR perspective(Bristol : IOP Publ., 2023) Sahoo, M.; Salman, Z.; Allodi, G.; Isaeva, A.; Folkers, L.; Wolter, A.U.B.; Büchner, B.; De Renzi, R.We investigated the magnetic properties of polycrystalline samples of the intrinsic magnetic topological insulators MnPn2Te4, with pnictogen Pn = Sb, Bi, by bulk magnetization and μSR. DC susceptibility detects the onset of magnetic ordering at TN = 27 K and 24 K and a field dependence of the macroscopic magnetization compatible with ferri- (or ferro-) and atiferro- magnetic ordering, respectively. Weak transverse field (wTF) Muon Spin Rotation (μSR) confirms the homogeneous bulk nature of magnetic ordering at the same two distinct transition temperatures. Zero Field (ZF) μSR shows that the Sb based material displays a broader distribution of internal field at the muon, in accordance with a larger deviation from the stoichiomectric composition and a higher degree of positional disorder (Mn at the Pn(6c) site), which however does not affect significantly the sharpness of the thermodynamic transition, as detected by the muon magnetic volume fraction and the observability of a critical divergence in the longitudinal and transverse muon relaxation rates.
- ItemMagnetic granularity in pulsed laser deposited YBCO films on technical templates at 5 K(Bristol : IOP Publ., 2017-9-4) Lao, M.; Hecher, J.; Pahlke, P.; Sieger, M.; Hühne, R.; Eisterer, M.The manifestation of granularity in the superconducting properties of pulsed laser deposited YBCO films on commercially available metallic templates was investigated by scanning Hall probe microscopy at 5 K and was related to local orientation mapping of the YBCO layer. The YBCO films on stainless steel templates with a textured buffer layer of yttrium stabilized ZrO2 grown by alternating beam assisted deposition have a mean grain size of less than with a sharp texture. This results in a homogeneous trapped field profile and spatial distribution of the current density. On the other hand, YBCO films on biaxially textured NiW substrates show magnetic granularity that persists down to a temperature of 5 K and up to an applied magnetic field of 4 T. The origin of the granular field profile is directly correlated to the microstructural properties of the YBCO layer adopted from the granular NiW substrate which leads to a spatially inhomogeneous current density. Grain-to-grain in-plane tilts lead to grain boundaries that obstruct the current while out-of-plane tilts mainly affect the grain properties, resulting in areas with low . Hence, not all grain boundaries cause detrimental effects on since the orientation of individual NiW grains also contributes to observed inhomogeneity and granularity.
- ItemTowards a reliable bridge joint between REBCO coated conductors(Bristol : IOP Publ., 2020) Kirchner, A.; Nielsch, K.; Hühne, R.REBa2Cu3O7-x (REBCO; RE = Y, Gd) coated conductor wires are commercially available up to a length of about 1 km. However, for large-scale devices like superconducting coils for high-field magnets several kilometres of a coated conductors are required. Therefore, it is desirable to use joints, which exhibit similar superconducting properties as the coated conductor itself. In this study, we jointed commercial REBCO coated conductors by a two-step procedure. At first, a superconducting soldering solution was developed and deposited on unstabilized coated conductors via chemical solution deposition. The soldering precursor is based on a Cu-rich solution with a metal cation ratio Y:Ba:Cu of 1:2:4. Secondly, a piece of the coated conductor was delaminated between the superconducting and the buffer layer and used as bridge between two other conductors covered with the soldering layer. Annealing the resulting bridge joint under pressure results in a mechanical stable configuration. © Published under licence by IOP Publishing Ltd.
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