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- ItemIntercomparison study and optical asphericity measurements of small ice particles in the CERN CLOUD experiment(Katlenburg-Lindau : Copernicus, 2017) Nichman, Leonid; Järvinen, Emma; Dorsey, James; Connolly, Paul; Duplissy, Jonathan; Fuchs, Claudia; Ignatius, Karoliina; Sengupta, Kamalika; Stratmann, Frank; Möhler, Ottmar; Schnaiter, Martin; Gallagher, MartinOptical probes are frequently used for the detection of microphysical cloud particle properties such as liquid and ice phase, size and morphology. These properties can eventually influence the angular light scattering properties of cirrus clouds as well as the growth and accretion mechanisms of single cloud particles. In this study we compare four commonly used optical probes to examine their response to small cloud particles of different phase and asphericity. Cloud simulation experiments were conducted at the Cosmics Leaving OUtdoor Droplets (CLOUD) chamber at European Organisation for Nuclear Research (CERN). The chamber was operated in a series of multi-step adiabatic expansions to produce growth and sublimation of ice particles at super- and subsaturated ice conditions and for initial temperatures of -30, -40 and -50°C. The experiments were performed for ice cloud formation via homogeneous ice nucleation. We report the optical observations of small ice particles in deep convection and in situ cirrus simulations. Ice crystal asphericity deduced from measurements of spatially resolved single particle light scattering patterns by the Particle Phase Discriminator mark 2 (PPD-2K, Karlsruhe edition) were compared with Cloud and Aerosol Spectrometer with Polarisation (CASPOL) measurements and image roundness captured by the 3View Cloud Particle Imager (3V-CPI). Averaged path light scattering properties of the simulated ice clouds were measured using the Scattering Intensity Measurements for the Optical detectioN of icE (SIMONE) and single particle scattering properties were measured by the CASPOL. We show the ambiguity of several optical measurements in ice fraction determination of homogeneously frozen ice in the case where sublimating quasi-spherical ice particles are present. Moreover, most of the instruments have difficulties of producing reliable ice fraction if small aspherical ice particles are present, and all of the instruments cannot separate perfectly spherical ice particles from supercooled droplets. Correlation analysis of bulk averaged path depolarisation measurements and single particle measurements of these clouds showed higher R2 values at high concentrations and small diameters, but these results require further confirmation. We find that none of these instruments were able to determine unambiguously the phase of the small particles. These results have implications for the interpretation of atmospheric measurements and parametrisations for modelling, particularly for low particle number concentration clouds.
- ItemPolarization lidar: An extended three-signal calibration approach(Katlenburg-Lindau : Copernicus, 2019) Jimenez, Cristofer; Ansmann, Albert; Engelmann, Ronny; Haarig, Moritz; Schmidt, Jörg; Wandinger, UllaWe present a new formalism to calibrate a threesignal polarization lidar and to measure highly accurate height profiles of the volume linear depolarization ratios under realistic experimental conditions. The methodology considers elliptically polarized laser light, angular misalignment of the receiver unit with respect to the main polarization plane of the laser pulses, and cross talk among the receiver channels. A case study of a liquid-water cloud observation demonstrates the potential of the new technique. Long-term observations of the calibration parameters corroborate the robustness of the method and the long-term stability of the three-signal polarization lidar. A comparison with a second polarization lidar shows excellent agreement regarding the derived volume linear polarization ratios in different scenarios: A biomass burning smoke event throughout the troposphere and the lower stratosphere up to 16 km in height, a dust case, and also a cirrus cloud case. © Author(s) 2019.
- ItemThe global aerosol-climate model ECHAM6.3-HAM2.3-Part 2: Cloud evaluation, aerosol radiative forcing, and climate sensitivity(Katlenburg-Lindau : Copernicus, 2019) Neubauer, David; Ferrachat, Sylvaine; Siegenthaler-Le Drian, Colombe; Stier, Philip; Partridge, Daniel G.; Tegen, Ina; Bey, Isabelle; Stanelle, Tanja; Kokkola, Harri; Lohmann, UlrikeThe global aerosol–climate model ECHAM6.3–HAM2.3 (E63H23) as well as the previous model versions ECHAM5.5–HAM2.0 (E55H20) and ECHAM6.1–HAM2.2 (E61H22) are evaluated using global observational datasets for clouds and precipitation. In E63H23, the amount of low clouds, the liquid and ice water path, and cloud radiative effects are more realistic than in previous model versions. E63H23 has a more physically based aerosol activation scheme, improvements in the cloud cover scheme, changes in the detrainment of convective clouds, changes in the sticking efficiency for the accretion of ice crystals by snow, consistent ice crystal shapes throughout the model, and changes in mixed-phase freezing; an inconsistency in ice crystal number concentration (ICNC) in cirrus clouds was also removed. Common biases in ECHAM and in E63H23 (and in previous ECHAM–HAM versions) are a cloud amount in stratocumulus regions that is too low and deep convective clouds over the Atlantic and Pacific oceans that form too close to the continents (while tropical land precipitation is underestimated). There are indications that ICNCs are overestimated in E63H23. Since clouds are important for effective radiative forcing due to aerosol–radiation and aerosol–cloud interactions (ERFari+aci) and equilibrium climate sensitivity (ECS), differences in ERFari+aci and ECS between the model versions were also analyzed. ERFari+aci is weaker in E63H23 (−1.0 W m−2) than in E61H22 (−1.2 W m−2) (or E55H20; −1.1 W m−2). This is caused by the weaker shortwave ERFari+aci (a new aerosol activation scheme and sea salt emission parameterization in E63H23, more realistic simulation of cloud water) overcompensating for the weaker longwave ERFari+aci (removal of an inconsistency in ICNC in cirrus clouds in E61H22). The decrease in ECS in E63H23 (2.5 K) compared to E61H22 (2.8 K) is due to changes in the entrainment rate for shallow convection (affecting the cloud amount feedback) and a stronger cloud phase feedback. Experiments with minimum cloud droplet number concentrations (CDNCmin) of 40 cm−3 or 10 cm−3 show that a higher value of CDNCmin reduces ERFari+aci as well as ECS in E63H23.
- ItemCoupling aerosols to (cirrus) clouds in the global EMAC-MADE3 aerosol–climate model(Katlenburg-Lindau : Copernicus, 2020) Righi, Mattia; Hendricks, Johannes; Lohmann, Ulrike; Beer, Christof Gerhard; Hahn, Valerian; Heinold, Bernd; Heller, Romy; Krämer, Martina; Ponater, Michael; Rolf, Christian; Tegen, Ina; Voigt, ChristianeA new cloud microphysical scheme including a detailed parameterization for aerosol-driven ice formation in cirrus clouds is implemented in the global ECHAM/MESSy Atmospheric Chemistry (EMAC) chemistry–climate model and coupled to the third generation of the Modal Aerosol Dynamics model for Europe adapted for global applications (MADE3) aerosol submodel. The new scheme is able to consistently simulate three regimes of stratiform clouds – liquid, mixed-, and ice-phase (cirrus) clouds – considering the activation of aerosol particles to form cloud droplets and the nucleation of ice crystals. In the cirrus regime, it allows for the competition between homogeneous and heterogeneous freezing for the available supersaturated water vapor, taking into account different types of ice-nucleating particles, whose specific ice-nucleating properties can be flexibly varied in the model setup. The new model configuration is tuned to find the optimal set of parameters that minimizes the model deviations with respect to observations. A detailed evaluation is also performed comparing the model results for standard cloud and radiation variables with a comprehensive set of observations from satellite retrievals and in situ measurements. The performance of EMAC-MADE3 in this new coupled configuration is in line with similar global coupled models and with other global aerosol models featuring ice cloud parameterizations. Some remaining discrepancies, namely a high positive bias in liquid water path in the Northern Hemisphere and overestimated (underestimated) cloud droplet number concentrations over the tropical oceans (in the extratropical regions), which are both a common problem in these kinds of models, need to be taken into account in future applications of the model. To further demonstrate the readiness of the new model system for application studies, an estimate of the anthropogenic aerosol effective radiative forcing (ERF) is provided, showing that EMAC-MADE3 simulates a relatively strong aerosol-induced cooling but within the range reported in the Intergovernmental Panel on Climate Change (IPCC) assessments.
- ItemCloud mask algorithm from the EarthCARE Multi-Spectral Imager: the M-CM products(Katlenburg-Lindau : Copernicus, 2023) Hünerbein, Anja; Bley, Sebastian; Horn, Stefan; Deneke, Hartwig; Walther, AndiThe EarthCARE (Earth Clouds, Aerosols and Radiation Explorer) satellite mission will provide new insights into aerosol-cloud-radiation interactions by means of synergistic observations of the Earth's atmosphere from a collection of active and passive remote sensing instruments, flying on a single satellite platform. The Multi-Spectral Imager (MSI) will provide visible and infrared images in the cross-track direction with a 150km swath and a pixel sampling at 500m. The suite of MSI cloud algorithms will deliver cloud macro- and microphysical properties complementary to the vertical profiles measured from the Atmospheric Lidar (ATLID) and the Cloud Profiling Radar (CPR) instruments. This paper provides an overview of the MSI cloud mask algorithm (M-CM) being developed to derive the cloud flag, cloud phase and cloud type products, which are essential inputs to downstream EarthCARE algorithms providing cloud optical and physical properties (M-COP) and aerosol optical properties (M-AOT). The MSI cloud mask algorithm has been applied to simulated test data from the EarthCARE end-to-end simulator and satellite data from the Moderate Resolution Imaging Spectroradiometer (MODIS) as well as from the Spinning Enhanced Visible InfraRed Imager (SEVIRI). Verification of the MSI cloud mask algorithm to the simulated test data and the official cloud products from SEVIRI and MODIS demonstrates a good performance of the algorithm. Some discrepancies are found, however, for the detection of thin cirrus clouds over bright surfaces like desert or snow. This will be improved by tuning of the thresholds once real observations are available.
- ItemCloud-Aerosol Transport System (CATS) 1064 nm calibration and validation(Katlenburg-Lindau : Copernicus, 2019) Pauly, Rebecca M.; Yorks, John E.; Hlavka, Dennis L.; McGill, Matthew J.; Amiridis, Vassilis; Palm, Stephen P.; Rodier, Sharon D.; Vaughan, Mark A.; Selmer, Patrick A.; Kupchock, Andrew W.; Baars, Holger; Gialitaki, AnnaThe Cloud-Aerosol Transport System (CATS) lidar on board the International Space Station (ISS) operated from 10 February 2015 to 30 October 2017 providing range-resolved vertical backscatter profiles of Earth's atmosphere at 1064 and 532 nm. The CATS instrument design and ISS orbit lead to a higher 1064 nm signal-to-noise ratio than previous space-based lidars, allowing for direct atmospheric calibration of the 1064 nm signals. Nighttime CATS version 3-00 data were calibrated by scaling the measured data to a model of the expected atmospheric backscatter between 22 and 26 km a.m.s.l. (above mean sea level). The CATS atmospheric model is constructed using molecular backscatter profiles derived from Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2) reanalysis data and aerosol scattering ratios measured by the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP). The nighttime normalization altitude region was chosen to simultaneously minimize aerosol loading and variability within the CATS data frame, which extends from 28 to −2 km a.m.s.l. Daytime CATS version 3-00 data were calibrated through comparisons with nighttime measurements of the layer-integrated attenuated total backscatter (iATB) from strongly scattering, rapidly attenuating opaque cirrus clouds. The CATS nighttime 1064 nm attenuated total backscatter (ATB) uncertainties for clouds and aerosols are primarily related to the uncertainties in the CATS nighttime calibration technique, which are estimated to be ∼9 %. Median CATS V3-00 1064 nm ATB relative uncertainty at night within cloud and aerosol layers is 7 %, slightly lower than these calibration uncertainty estimates. CATS median daytime 1064 nm ATB relative uncertainty is 21 % in cloud and aerosol layers, similar to the estimated 16 %–18 % uncertainty in the CATS daytime cirrus cloud calibration transfer technique. Coincident daytime comparisons between CATS and the Cloud Physics Lidar (CPL) during the CATS-CALIPSO Airborne Validation Experiment (CCAVE) project show good agreement in mean ATB profiles for clear-air regions. Eight nighttime comparisons between CATS and the PollyXT ground-based lidars also show good agreement in clear-air regions between 3 and 12 km, with CATS having a mean ATB of 19.7 % lower than PollyXT. Agreement between the two instruments (∼7 %) is even better within an aerosol layer. Six-month comparisons of nighttime ATB values between CATS and CALIOP also show that iATB comparisons of opaque cirrus clouds agree to within 19 %. Overall, CATS has demonstrated that direct calibration of the 1064 nm channel is possible from a space-based lidar using the atmospheric normalization technique.