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- ItemReactive Halogens in the Marine Boundary Layer (RHaMBLe): The tropical North Atlantic experiments(München : European Geopyhsical Union, 2010) Lee, J.D.; McFiggans, G.; Allan, J.D.; Baker, A.R.; Ball, S.M.; Benton, A.K.; Carpenter, L.J.; Commane, R.; Finley, B.D.; Evans, M.; Fuentes, E.; Furneaux, K.; Goddard, A.; Good, N.; Hamilton, J.F.; Heard, D.E.; Herrmann, H.; Hollingsworth, A.; Hopkins, J.R.; Ingham, T.; Irwin, M.; Jones, C.E.; Jones, R.L.; Keene, W.C.; Lawler, M.J.; Lehmann, S.; Lewis, A.C.; Long, M.S.; Mahajan, A.; Methven, J.; Moller, S.J.; Müller, K.; Müller, T.; Niedermeier, N.; O'Doherty, S.; Oetjen, H.; Plane, J.M.C.; Pszenny, A.A.P.; Read, K.A.; Saiz-Lopez, A.; Saltzman, E.S.; Sander, R.; von Glasow, R.; Whalley, L.; Wiedensohler, A.; Young, D.The NERC UK SOLAS-funded Reactive Halogens in the Marine Boundary Layer (RHaMBLe) programme comprised three field experiments. This manuscript presents an overview of the measurements made within the two simultaneous remote experiments conducted in the tropical North Atlantic in May and June 2007. Measurements were made from two mobile and one ground-based platforms. The heavily instrumented cruise D319 on the RRS Discovery from Lisbon, Portugal to São Vicente, Cape Verde and back to Falmouth, UK was used to characterise the spatial distribution of boundary layer components likely to play a role in reactive halogen chemistry. Measurements onboard the ARSF Dornier aircraft were used to allow the observations to be interpreted in the context of their vertical distribution and to confirm the interpretation of atmospheric structure in the vicinity of the Cape Verde islands. Long-term ground-based measurements at the Cape Verde Atmospheric Observatory (CVAO) on São Vicente were supplemented by long-term measurements of reactive halogen species and characterisation of additional trace gas and aerosol species during the intensive experimental period. This paper presents a summary of the measurements made within the RHaMBLe remote experiments and discusses them in their meteorological and chemical context as determined from these three platforms and from additional meteorological analyses. Air always arrived at the CVAO from the North East with a range of air mass origins (European, Atlantic and North American continental). Trace gases were present at stable and fairly low concentrations with the exception of a slight increase in some anthropogenic components in air of North American origin, though NOx mixing ratios during this period remained below 20 pptv (note the non-IUPAC adoption in this manuscript of pptv and ppbv, equivalent to pmol mol−1 and nmol mol−1 to reflect common practice). Consistency with these air mass classifications is observed in the time series of soluble gas and aerosol composition measurements, with additional identification of periods of slightly elevated dust concentrations consistent with the trajectories passing over the African continent. The CVAO is shown to be broadly representative of the wider North Atlantic marine boundary layer; measurements of NO, O3 and black carbon from the ship are consistent with a clean Northern Hemisphere marine background. Aerosol composition measurements do not indicate elevated organic material associated with clean marine air. Closer to the African coast, black carbon and NO levels start to increase, indicating greater anthropogenic influence. Lower ozone in this region is possibly associated with the increased levels of measured halocarbons, associated with the nutrient rich waters of the Mauritanian upwelling. Bromide and chloride deficits in coarse mode aerosol at both the CVAO and on D319 and the continuous abundance of inorganic gaseous halogen species at CVAO indicate significant reactive cycling of halogens. Aircraft measurements of O3 and CO show that surface measurements are representative of the entire boundary layer in the vicinity both in diurnal variability and absolute levels. Above the inversion layer similar diurnal behaviour in O3 and CO is observed at lower mixing ratios in the air that had originated from south of Cape Verde, possibly from within the ITCZ. ECMWF calculations on two days indicate very different boundary layer depths and aircraft flights over the ship replicate this, giving confidence in the calculated boundary layer depth.
- ItemLong-term measurements of aerosol and carbon monoxide at the ZOTTO tall tower to characterize polluted and pristine air in the Siberian taiga(München : European Geopyhsical Union, 2013) Chi, X.; Winderlich, J.; Mayer, J.-C.; Panov, A.V.; Heimann, M.; Birmili, W.; Heintzenberg, J.; Cheng, Y.; Andreae, M.O.Siberia is one of few continental regions in the Northern Hemisphere where the atmosphere may sometimes approach pristine background conditions. We present the time series of aerosol and carbon monoxide (CO) measurements between September 2006 and December 2011 at the Zotino Tall Tower Observatory (ZOTTO) in Central Siberia (61° N; 89° E). We investigate the seasonal, weekly and diurnal variations of aerosol properties (including absorption and scattering coefficients and derived parameters, such as equivalent black carbon (BCe), Ångström exponent, single scattering albedo, and backscattering ratio) and the CO mixing ratios. Criteria were established to distinguish polluted from near-pristine air masses, providing quantitative characteristics for each type. Depending on the season, 23–36% of the sampling time at ZOTTO was found to be representative of a clean atmosphere. The summer pristine data indicate that primary biogenic and secondary organic aerosol formation are quite strong particle sources in the Siberian taiga. The summer seasons 2007–2008 were dominated by an Aitken mode around 80 nm size, whereas the summer 2009 with prevailing easterly winds produced particles in the accumulation mode around 200 nm size. We found these differences to be mainly related to air temperature, through its effect on the production rates of biogenic volatile organic compounds (VOC) precursor gases. In winter, the particle size distribution peaked at 160 nm, and the footprint of clean background air was characteristic for aged particles from anthropogenic sources at great distances from ZOTTO and diluted biofuel burning emissions from domestic heating. The wintertime polluted air originates mainly from large cities south and southwest of the site; these particles have a dominant mode around 100 nm, and the ΔBCe / ΔCO ratio of 7–11 ng m−3 ppb−1 suggests dominant contributions from coal and biofuel burning for heating. During summer, anthropogenic emissions are the dominant contributor to the pollution particles at ZOTTO, while only 12% of the polluted events are classified as biomass-burning-dominated, but then often associated with extremely high CO concentrations and aerosol absorption coefficients. Two biomass-burning case studies revealed different ΔBCe / ΔCO ratios from different fire types, with the agricultural fires in April~2008 yielding a very high ratio of 21 ng m−3 ppb−1. Overall, we find that anthropogenic sources dominate the aerosol population at ZOTTO most of the time, even during nominally clean episodes in winter, and that near-pristine conditions are encountered only in the growing season and then only episodically.
- ItemRole of CO2, climate and land use in regulating the seasonal amplitude increase of carbon fluxes in terrestrial ecosystems: A multimodel analysis(München : European Geopyhsical Union, 2016) Zhao, Fang; Zeng, Ning; Asrar, Ghassem; Friedlingstein, Pierre; Ito, Akihiko; Jain, Atul; Kalnay, Eugenia; Kato, Etsushi; Koven, Charles D.; Poulter, Ben; Rafique, Rashid; Sitch, Stephen; Shu, Shijie; Stocker, Beni; Viovy, Nicolas; Wiltshire, Andy; Zaehle, SonkeWe examined the net terrestrial carbon flux to the atmosphere (FTA) simulated by nine models from the TRENDY dynamic global vegetation model project for its seasonal cycle and amplitude trend during 1961–2012. While some models exhibit similar phase and amplitude compared to atmospheric inversions, with spring drawdown and autumn rebound, others tend to rebound early in summer. The model ensemble mean underestimates the magnitude of the seasonal cycle by 40 % compared to atmospheric inversions. Global FTA amplitude increase (19 ± 8 %) and its decadal variability from the model ensemble are generally consistent with constraints from surface atmosphere observations. However, models disagree on attribution of this long-term amplitude increase, with factorial experiments attributing 83 ± 56 %, −3 ± 74 and 20 ± 30 % to rising CO2, climate change and land use/cover change, respectively. Seven out of the nine models suggest that CO2 fertilization is the strongest control – with the notable exception of VEGAS, which attributes approximately equally to the three factors. Generally, all models display an enhanced seasonality over the boreal region in response to high-latitude warming, but a negative climate contribution from part of the Northern Hemisphere temperate region, and the net result is a divergence over climate change effect. Six of the nine models show that land use/cover change amplifies the seasonal cycle of global FTA: some are due to forest regrowth, while others are caused by crop expansion or agricultural intensification, as revealed by their divergent spatial patterns. We also discovered a moderate cross-model correlation between FTA amplitude increase and increase in land carbon sink (R2 = 0.61). Our results suggest that models can show similar results in some benchmarks with different underlying mechanisms; therefore, the spatial traits of CO2 fertilization, climate change and land use/cover changes are crucial in determining the right mechanisms in seasonal carbon cycle change as well as mean sink change.
- ItemAerosol decadal trends - Part 2: In-situ aerosol particle number concentrations at GAW and ACTRIS stations(München : European Geopyhsical Union, 2013) Asmi, A.; Collaud Coen, M.; Ogren, J.A.; Andrews, E.; Sheridan, P.; Jefferson, A.; Weingartner, E.; Baltensperger, U.; Bukowiecki, N.; Lihavainen, H.; Kivekäs, N.; Asmi, E.; Aalto, P.P.; Kulmala, M.; Wiedensohler, A.; Birmili, W.; Hamed, A.; O'Dowd, C.; Jennings, S.G.; Weller, R.; Flentje, H.; Fjaeraa, A.M.; Fiebig, M.; Myhre, C.L.; Hallar, A.G.; Swietlicki, E.; Kristensson, A.; Laj, P.We have analysed the trends of total aerosol particle number concentrations (N) measured at long-term measurement stations involved either in the Global Atmosphere Watch (GAW) and/or EU infrastructure project ACTRIS. The sites are located in Europe, North America, Antarctica, and on Pacific Ocean islands. The majority of the sites showed clear decreasing trends both in the full-length time series, and in the intra-site comparison period of 2001–2010, especially during the winter months. Several potential driving processes for the observed trends were studied, and even though there are some similarities between N trends and air temperature changes, the most likely cause of many northern hemisphere trends was found to be decreases in the anthropogenic emissions of primary particles, SO2 or some co-emitted species. We could not find a consistent agreement between the trends of N and particle optical properties in the few stations with long time series of all of these properties. The trends of N and the proxies for cloud condensation nuclei (CCN) were generally consistent in the few European stations where the measurements were available. This work provides a useful comparison analysis for modelling studies of trends in aerosol number concentrations.
- ItemThe importance of snow albedo for ice sheet evolution over the last glacial cycle(München : European Geopyhsical Union, 2018) Willeit, Matteo; Ganopolski, AndreyThe surface energy and mass balance of ice sheets strongly depends on the amount of solar radiation absorbed at the surface, which is mainly controlled by the albedo of snow and ice. Here, using an Earth system model of intermediate complexity, we explore the role played by surface albedo for the simulation of glacial cycles. We show that the evolution of the Northern Hemisphere ice sheets over the last glacial cycle is very sensitive to the representation of snow albedo in the model. It is well known that the albedo of snow depends strongly on snow grain size and the content of light-absorbing impurities. Excluding either the snow aging effect or the dust darkening effect on snow albedo leads to an excessive ice build-up during glacial times and consequently to a failure in simulating deglaciation. While the effect of snow grain growth on snow albedo is well constrained, the albedo reduction due to the presence of dust in snow is much more uncertain because the light-absorbing properties of dust vary widely as a function of dust mineral composition. We also show that assuming slightly different optical properties of dust leads to very different ice sheet and climate evolutions in the model. Conversely, ice sheet evolution is less sensitive to the choice of ice albedo in the model. We conclude that a proper representation of snow albedo is a fundamental prerequisite for a successful simulation of glacial cycles.
- ItemCoupled Northern Hemisphere permafrost-ice-sheet evolution over the last glacial cycle(München : European Geopyhsical Union, 2015) Willeit, M.; Ganopolski, A.Permafrost influences a number of processes which are relevant for local and global climate. For example, it is well known that permafrost plays an important role in global carbon and methane cycles. Less is known about the interaction between permafrost and ice sheets. In this study a permafrost module is included in the Earth system model CLIMBER-2, and the coupled Northern Hemisphere (NH) permafrost–ice-sheet evolution over the last glacial cycle is explored. The model performs generally well at reproducing present-day permafrost extent and thickness. Modeled permafrost thickness is sensitive to the values of ground porosity, thermal conductivity and geothermal heat flux. Permafrost extent at the Last Glacial Maximum (LGM) agrees well with reconstructions and previous modeling estimates. Present-day permafrost thickness is far from equilibrium over deep permafrost regions. Over central Siberia and the Arctic Archipelago permafrost is presently up to 200–500 m thicker than it would be at equilibrium. In these areas, present-day permafrost depth strongly depends on the past climate history and simulations indicate that deep permafrost has a memory of surface temperature variations going back to at least 800 ka. Over the last glacial cycle permafrost has a relatively modest impact on simulated NH ice sheet volume except at LGM, when including permafrost increases ice volume by about 15 m sea level equivalent in our model. This is explained by a delayed melting of the ice base from below by the geothermal heat flux when the ice sheet sits on a porous sediment layer and permafrost has to be melted first. Permafrost affects ice sheet dynamics only when ice extends over areas covered by thick sediments, which is the case at LGM.
- ItemTropospheric forcing of the boreal polar vortex splitting in January 2003(München : European Geopyhsical Union, 2010) Peters, D.H.W.; Vargin, P.; Gabriel, A.; Tsvetkova, N.; Yushkov, V.e dynamical evolution of the relatively warm stratospheric winter season 2002–2003 in the Northern Hemisphere was studied and compared with the cold winter 2004–2005 based on NCEP-Reanalyses. Record low temperatures were observed in the lower and middle stratosphere over the Arctic region only at the beginning of the 2002–2003 winter. Six sudden stratospheric warming events, including the major warming event with a splitting of the polar vortex in mid-January 2003, have been identified. This led to a very high vacillation of the zonal mean circulation and a weakening of the stratospheric polar vortex over the whole winter season. An estimate of the mean chemical ozone destruction inside the polar vortex showed a total ozone loss of about 45 DU in winter 2002–2003; that is about 2.5 times smaller than in winter 2004–2005. Embedded in a winter with high wave activity, we found two subtropical Rossby wave trains in the troposphere before the major sudden stratospheric warming event in January 2003. These Rossby waves propagated north-eastwards and maintained two upper tropospheric anticyclones. At the same time, the amplification of an upward propagating planetary wave 2 in the upper troposphere and lower stratosphere was observed, which could be caused primarily by those two wave trains. Furthermore, two extratropical Rossby wave trains over the North Pacific Ocean and North America were identified a couple of days later, which contribute mainly to the vertical planetary wave activity flux just before and during the major warming event. It is shown that these different tropospheric forcing processes caused the major warming event and contributed to the splitting of the polar vortex.
- ItemSimilarities and differences in polar mesosphere summer echoes observed in the Arctic and Antarctica(München : European Geopyhsical Union, 2008) Latteck, R.; Singer, W.; Morris, R.J.; Hocking, W.K.; Murphy, D.J.; Holdsworth, D.A.; Swarnalingam, N.Polar Mesosphere Summer Echoes (PMSE) have been observed in the high latitudes of the Northern and Southern Hemisphere for several years using VHF radars located at Andenes/Norway (69° N, 16° E), Resolute Bay/Canada (75° N, 95° W), and Davis/Antarctica (69° S, 78° E). The VHF radars at the three sites were calibrated using the same methods (noise source and delayed transmitting signal) and identical equipment. Volume reflectivity was derived from the calibrated echo power and the characteristics of the seasonal variation of PMSE were estimated at the sites for the years 2004 to 2007. The largest peak volume reflectivity of about 2×10−9 m−1 was observed at Andenes compared with their counterparts at Davis (~4×10−11 m−1) and Resolute Bay (~6×10−12 m−1). The peak of the PMSE height distribution is 85.6 km at Davis which is about 1 km higher than at Andenes. At Resolute Bay the height distribution peaks at about 85 km but only a few layers were found below 84 km. The mean PMSE occurrence rate is 83% at Andenes, 38% at Davis with larger variability and only 18% at Resolute Bay (in late summer). The duration of the PMSE season varies at Andenes from 104 to 113 days and at Davis from 88 to 93 days. In general the PMSE seasons starts about 5 days later at Davis and ends about 10 days earlier compared to Andenes. In all three seasons the PMSE occurrence suddenly drops to a much lower level at Davis about 32 days after solstice whereas the PMSE season decays smoothly at Andenes. The duration of the PMSE season at Andenes and Davis is highly correlated with the presence of equatorward directed winds, the observed differences in PMSE occurrence are related to the mesospheric temperatures at both sites.
- ItemFive-day planetary waves in the middle atmosphere from Odin satellite data and ground-based instruments in Northern Hemisphere summer 2003, 2004, 2005 and 2007(München : European Geopyhsical Union, 2008) Belova, A.; Kirkwood, S.; Murtagh, D.; Mitchell, N.; Singer, W.; Hocking, W.A number of studies have shown that 5-day planetary waves modulate noctilucent clouds and the closely related Polar Mesosphere Summer Echoes (PMSE) at the summer mesopause. Summer stratospheric winds should inhibit wave propagation through the stratosphere and, although some numerical models (Geisler and Dickinson, 1976) do show a possibility for upward wave propagation, it has also been suggested that the upward propagation may in practice be confined to the winter hemisphere with horizontal propagation of the wave from the winter to the summer hemisphere at mesosphere heights causing the effects observed at the summer mesopause. It has further been proposed (Garcia et al., 2005) that 5-day planetary waves observed in the summer mesosphere could be excited in-situ by baroclinic instability in the upper mesosphere. In this study, we first extract and analyze 5-day planetary wave characteristics on a global scale in the middle atmosphere (up to 54 km in temperature, and up to 68 km in ozone concentration) using measurements by the Odin satellite for selected days during northern hemisphere summer from 2003, 2004, 2005 and 2007. Second, we show that 5-day temperature fluctuations consistent with westward-traveling 5-day waves are present at the summer mesopause, using local ground-based meteor-radar observations. Finally we examine whether any of three possible sources of the detected temperature fluctuations at the summer mesopause can be excluded: upward propagation from the stratosphere in the summer-hemisphere, horizontal propagation from the winter-hemisphere or in-situ excitation as a result of the baroclinic instability. We find that in one case, far from solstice, the baroclinic instability is unlikely to be involved. In one further case, close to solstice, upward propagation in the same hemisphere seems to be ruled out. In all other cases, all or any of the three proposed mechanisms are consistent with the observations.
- ItemHistorical greenhouse gas concentrations for climate modelling (CMIP6)(München : European Geopyhsical Union, 2017) Meinshausen, Malte; Vogel, Elisabeth; Nauels, Alexander; Lorbacher, Katja; Meinshausen, Nicolai; Etheridge, David M.; Fraser, Paul J.; Montzka, Stephen A.; Rayner, Peter J.; Trudinger, Cathy M.; Krummel, Paul B.; Beyerle, Urs; Canadell, Josep G.; Daniel, John S.; Enting, Ian G.; Law, Rachel M. Law; Lunder, Chris R.; O'Doherty, Simon; Prinn, Ron G.; Reimann, Stefan; Rubino, Mauro; Velders, Guus J.M.; Vollmer, Martin K.; Wang, Ray H.J.; Weiss, RayAtmospheric greenhouse gas (GHG) concentrations are at unprecedented, record-high levels compared to the last 800000 years. Those elevated GHG concentrations warm the planet and – partially offset by net cooling effects by aerosols – are largely responsible for the observed warming over the past 150 years. An accurate representation of GHG concentrations is hence important to understand and model recent climate change. So far, community efforts to create composite datasets of GHG concentrations with seasonal and latitudinal information have focused on marine boundary layer conditions and recent trends since the 1980s. Here, we provide consolidated datasets of historical atmospheric concentrations (mole fractions) of 43 GHGs to be used in the Climate Model Intercomparison Project – Phase 6 (CMIP6) experiments. The presented datasets are based on AGAGE and NOAA networks, firn and ice core data, and archived air data, and a large set of published studies. In contrast to previous intercomparisons, the new datasets are latitudinally resolved and include seasonality. We focus on the period 1850–2014 for historical CMIP6 runs, but data are also provided for the last 2000 years. We provide consolidated datasets in various spatiotemporal resolutions for carbon dioxide (CO2), methane (CH4) and nitrous oxide (N2O), as well as 40 other GHGs, namely 17 ozone-depleting substances, 11 hydrofluorocarbons (HFCs), 9 perfluorocarbons (PFCs), sulfur hexafluoride (SF6), nitrogen trifluoride (NF3) and sulfuryl fluoride (SO2F2). In addition, we provide three equivalence species that aggregate concentrations of GHGs other than CO2, CH4 and N2O, weighted by their radiative forcing efficiencies. For the year 1850, which is used for pre-industrial control runs, we estimate annual global-mean surface concentrations of CO2 at 284.3ppm, CH4 at 808.2ppb and N2O at 273.0ppb. The data are available at https://esgf-node.llnl.gov/search/input4mips/ and http://www.climatecollege.unimelb.edu.au/cmip6. While the minimum CMIP6 recommendation is to use the global- and annual-mean time series, modelling groups can also choose our monthly and latitudinally resolved concentrations, which imply a stronger radiative forcing in the Northern Hemisphere winter (due to the latitudinal gradient and seasonality).