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- ItemA DNS study of aerosol and small-scale cloud turbulence interaction(München : European Geopyhsical Union, 2016) Babkovskaia, Natalia; Rannik, Ullar; Phillips, Vaughan; Siebert, Holger; Wehner, Birgit; Boy, MichaelThe purpose of this study is to investigate the interaction between small-scale turbulence and aerosol and cloud microphysical properties using direct numerical simulations (DNS). We consider the domain located at the height of about 2000 m from the sea level, experiencing transient high supersaturation due to atmospheric fluctuations of temperature and humidity. To study the effect of total number of particles (Ntot) on air temperature, activation and supersaturation, we vary Ntot. To investigate the effect of aerosol dynamics on small-scale turbulence and vertical air motion, we vary the intensity of turbulent fluctuations and the buoyant force. We find that even a small number of aerosol particles (55.5 cm−3), and therefore a small droplet number concentration, strongly affects the air temperature due to release of latent heat. The system comes to an equilibrium faster and the relative number of activated particles appears to be smaller for larger Ntot. We conclude that aerosol particles strongly affect the air motion. In a case of updraught coursed by buoyant force, the presence of aerosol particles results in acceleration of air motion in vertical direction and increase of turbulent fluctuations.
- ItemAerosols-cloud microphysics-thermodynamics-turbulence: Evaluating supersaturation in a marine stratocumulus cloud(München : European Geopyhsical Union, 2012) Ditas, F.; Shaw, R.A.; Siebert, H.; Simmel, M.; Wehner, B.; Wiedensohler, A.This work presents a unique combination of aerosol, cloud microphysical, thermodynamic and turbulence variables to characterize supersaturation fluctuations in a turbulent marine stratocumulus (SC) layer. The analysis is based on observations with the helicopter-borne measurement platform ACTOS and a detailed cloud microphysical parcel model following three different approaches: (1) From the comparison of aerosol number size distributions inside and below the SC layer, the number of activated particles is calculated as 435±87 cm−3 and compares well with the observed median droplet number concentration of Nd = 464 cm−3. Furthermore, a 50% activation diameter of Dp50≈115 nm was derived, which was linked to a critical supersaturation Scrit of 0.16% via Köhler theory. From the shape of the fraction of activated particles, we estimated a standard deviation of supersaturation fluctuations of σS' = 0.09%. (2) These estimates are compared to more direct thermodynamic observations at cloud base. Therefore, supersaturation fluctuations (S') are calculated based on highly-resolved thermodynamic data showing a standard deviation of S' ranging within 0.1%≤σS'≤0.3 %. (3) The sensitivity of the supersaturation on observed vertical wind velocity fluctuations is investigated with the help of a detailed cloud microphysical model. These results show highest fluctuations of S' with σS'=0.1% at cloud base and a decreasing σS' with increasing liquid water content and droplet number concentration. All three approaches are independent of each other and vary only within a factor of about two.
- ItemAtmospheric boundary layer top height in South Africa: Measurements with lidar and radiosonde compared to three atmospheric models(München : European Geopyhsical Union, 2014) Korhonen, K.; Giannakaki, E.; Mielonen, T.; Pfüller, A.; Laakso, L.; Vakkari, V.; Baars, H.; Engelmann, R.; Beukes, J.P.; Van Zyl, P.G.; Ramandh, A.; Ntsangwane, L.; Josipovic, M.; Tiitta, P.; Fourie, G.; Ngwana, I.; Chiloane, K.; Komppula, M.Atmospheric lidar measurements were carried out at Elandsfontein measurement station, on the eastern Highveld approximately 150 km east of Johannesburg in South Africa throughout 2010. The height of the planetary boundary layer (PBL) top was continuously measured using a Raman lidar, PollyXT (POrtabLe Lidar sYstem eXTended). High atmospheric variability together with a large surface temperature range and significant seasonal changes in precipitation were observed, which had an impact on the vertical mixing of particulate matter, and hence, on the PBL evolution. The results were compared to radiosondes, CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) space-borne lidar measurements and three atmospheric models that followed different approaches to determine the PBL top height. These models included two weather forecast models operated by ECMWF (European Centre for Medium-range Weather Forecasts) and SAWS (South African Weather Service), and one mesoscale prognostic meteorological and air pollution regulatory model TAPM (The Air Pollution Model). The ground-based lidar used in this study was operational for 4935 h during 2010 (49% of the time). The PBL top height was detected 86% of the total measurement time (42% of the total time). Large seasonal and diurnal variations were observed between the different methods utilised. High variation was found when lidar measurements were compared to radiosonde measurements. This could be partially due to the distance between the lidar measurements and the radiosondes, which were 120 km apart. Comparison of lidar measurements to the models indicated that the ECMWF model agreed the best with mean relative difference of 15.4%, while the second best correlation was with the SAWS model with corresponding difference of 20.1%. TAPM was found to have a tendency to underestimate the PBL top height. The wind speeds in the SAWS and TAPM models were strongly underestimated which probably led to underestimation of the vertical wind and turbulence and thus underestimation of the PBL top height. Comparison between ground-based and satellite lidar shows good agreement with a correlation coefficient of 0.88. On average, the daily maximum PBL top height in October (spring) and June (winter) was 2260 m and 1480 m, respectively. To our knowledge, this study is the first long-term study of PBL top heights and PBL growth rates in South Africa.
- ItemHigh-resolution measurement of cloud microphysics and turbulence at a mountaintop station(München : European Geopyhsical Union, 2015) Siebert, H.; Shaw, R.A.; Ditas, J.; Schmeissner, T.; Malinowski, S.P.; Bodenschatz, E.; Xu, H.Mountain research stations are advantageous not only for long-term sampling of cloud properties but also for measurements that are prohibitively difficult to perform on airborne platforms due to the large true air speed or adverse factors such as weight and complexity of the equipment necessary. Some cloud–turbulence measurements, especially Lagrangian in nature, fall into this category. We report results from simultaneous, high-resolution and collocated measurements of cloud microphysical and turbulence properties during several warm cloud events at the Umweltforschungsstation Schneefernerhaus (UFS) on Zugspitze in the German Alps. The data gathered were found to be representative of observations made with similar instrumentation in free clouds. The observed turbulence shared all features known for high-Reynolds-number flows: it exhibited approximately Gaussian fluctuations for all three velocity components, a clearly defined inertial subrange following Kolmogorov scaling (power spectrum, and second- and third-order Eulerian structure functions), and highly intermittent velocity gradients, as well as approximately lognormal kinetic energy dissipation rates. The clouds were observed to have liquid water contents on the order of 1 g m−3 and size distributions typical of continental clouds, sometimes exhibiting long positive tails indicative of large drop production through turbulent mixing or coalescence growth. Dimensionless parameters relevant to cloud–turbulence interactions, the Stokes number and settling parameter are in the range typically observed in atmospheric clouds. Observed fluctuations in droplet number concentration and diameter suggest a preference for inhomogeneous mixing. Finally, enhanced variance in liquid water content fluctuations is observed at high frequencies, and the scale break occurs at a value consistent with the independently estimated phase relaxation time from microphysical measurements.
- ItemSchneefernerhaus as a mountain research station for clouds and turbulence(München : European Geopyhsical Union, 2015) Risius, S.; Xu, H.; Di Lorenzo, F.; Xi, H.; Siebert, H.; Shaw, R.A.; Bodenschatz, E.Cloud measurements are usually carried out with airborne campaigns, which are expensive and are limited by temporal duration and weather conditions. Ground-based measurements at high-altitude research stations therefore play a complementary role in cloud study. Using the meteorological data (wind speed, direction, temperature, humidity, visibility, etc.) collected by the German Weather Service (DWD) from 2000 to 2012 and turbulence measurements recorded by multiple ultrasonic sensors (sampled at 10 Hz) in 2010, we show that the Umweltforschungsstation Schneefernerhaus (UFS) located just below the peak of Zugspitze in the German Alps, at a height of 2650 m, is a well-suited station for cloud–turbulence research. The wind at UFS is dominantly in the east–west direction and nearly horizontal. During the summertime (July and August) the UFS is immersed in warm clouds about 25 % of the time. The clouds are either from convection originating in the valley in the east, or associated with synoptic-scale weather systems typically advected from the west. Air turbulence, as measured from the second- and third-order velocity structure functions that exhibit well-developed inertial ranges, possesses Taylor microscale Reynolds numbers up to 104, with the most probable value at ~ 3000. In spite of the complex topography, the turbulence appears to be nearly as isotropic as many laboratory flows when evaluated on the "Lumley triangle".
- ItemALADINA - An unmanned research aircraft for observing vertical and horizontal distributions of ultrafine particles within the atmospheric boundary layer(München : European Geopyhsical Union, 2015) Altstädter, B.; Platis, A.; Wehner, B.; Scholtz, A.; Wildmann, N.; Hermann, M.; Käthner, R.; Baars, H.; Bange, J.; Lampert, A.This paper presents the unmanned research aircraft Carolo P360 "ALADINA" (Application of Light-weight Aircraft for Detecting IN situ Aerosol) for investigating the horizontal and vertical distribution of ultrafine particles in the atmospheric boundary layer (ABL). It has a wingspan of 3.6 m, a maximum take-off weight of 25 kg and is equipped with aerosol instrumentation and meteorological sensors. A first application of the system, together with the unmanned research aircraft MASC (Multi-Purpose Airborne Carrier) of the Eberhard Karls University of Tübingen (EKUT), is described. As small payload for ALADINA, two condensation particle counters (CPC) and one optical particle counter (OPC) were miniaturised by re-arranging the vital parts and composing them in a space-saving way in the front compartment of the airframe. The CPCs are improved concerning the lower detection threshold and the response time to less than 1.3 s. Each system was characterised in the laboratory and calibrated with test aerosols. The CPCs are operated in this study with two different lower detection threshold diameters of 11 and 18 nm. The amount of ultrafine particles, which is an indicator for new particle formation, is derived from the difference in number concentrations of the two CPCs (ΔN). Turbulence and thermodynamic structure of the boundary layer are described by measurements of fast meteorological sensors that are mounted at the aircraft nose. A first demonstration of ALADINA and a feasibility study were conducted in Melpitz near Leipzig, Germany, at the Global Atmosphere Watch (GAW) station of the Leibniz Institute for Tropospheric Research (TROPOS) on 2 days in October 2013. There, various ground-based instruments are installed for long-term atmospheric monitoring. The ground-based infrastructure provides valuable additional background information to embed the flights in the continuous atmospheric context and is used for validation of the airborne results. The development of the boundary layer, derived from backscatter signals of a portable Raman lidar POLLYXT, allows a quick overview of the current vertical structure of atmospheric particles. Ground-based aerosol number concentrations are consistent with the results from flights in heights of a few metres. In addition, a direct comparison of ALADINA aerosol data and ground-based aerosol data, sampling the air at the same location for more than 1 h, shows comparable values within the range of ± 20 %. MASC was operated simultaneously with complementary flight patterns. It is equipped with the same meteorological instruments that offer the possibility to determine turbulent fluxes. Therefore, additional information about meteorological conditions was collected in the lowest part of the atmosphere. Vertical profiles up to 1000 m in altitude indicate a high variability with distinct layers of aerosol, especially for the small particles of a few nanometres in diameter on 1 particular day. The stratification was almost neutral and two significant aerosol layers were detected with total aerosol number concentrations up to 17 000 ± 3400 cm−3 between 180 and 220 m altitude and 14 000 ± 2800 cm−3 between 550 and 650 m. Apart from those layers, the aerosol distribution was well mixed and reached the total number concentration of less than 8000 ± 1600 cm−3. During another day, the distribution of the small particles in the lowermost ABL was related to the stratification, with continuously decreasing number concentrations from 16 000 ± 3200 cm−3 to a minimum of 4000 ± 800 cm−3 at the top of the inversion at 320 m. Above this, the total number concentration was rather constant. In the region of 500 to 600 m altitude, a significant difference of both CPCs was observed. This event occurred during the boundary layer development in the morning and represents a particle burst within the ABL.
- ItemObservations of turbulence-induced new particle formation in the residual layer(München : European Geopyhsical Union, 2010) Wehner, B.; Siebert, H.; Ansmann, A.; Ditas, F.; Seifert, P.; Stratmann, F.; Wiedensohler, A.; Apituley, A.; Shaw, R.A.; Manninen, H.E.; Kulmala, M.Aerosol particle measurements in the atmospheric boundary layer performed by a helicopter-borne measurement payload and by a lidar system from a case study during the IMPACT field campaign in Cabauw (NL) are presented. Layers of increased number concentrations of ultrafine particles were observed in the residual layer, indicating relatively recent new-particle formation. These layers were characterized by a sub-critical Richardson number and concomitant increased turbulence. Turbulent mixing is likely to lead to local supersaturation of possible precursor gases which are essential for new particle formation. Observed peaks in the number concentrations of ultrafine particles at ground level are connected to the new particle formation in the residual layer by boundary layer development and vertical mixing.
- ItemDerivation of turbulent energy dissipation rate with the Middle Atmosphere Alomar Radar System (MAARSY) and radiosondes at Andøya, Norway(München : European Geopyhsical Union, 2016) Li, Qiang; Rapp, Markus; Schrön, Anne; Schneider, Andreas; Stober, GunterWe present the derivation of turbulent energy dissipation rate ε from a total of 522 days of observations with the Middle Atmosphere Alomar Radar SYstem (MAARSY) mesosphere–stratosphere–troposphere (MST) radar running tropospheric experiments during the period of 2010–2013 as well as with balloon-borne radiosondes based on a campaign in the summer 2013. Spectral widths are converted to ε after the removal of the broadening effects due to the finite beam width of the radar. With the simultaneous in situ measurements of ε with balloon-borne radiosondes at the MAARSY radar site, we compare the ε values derived from both techniques and reach an encouraging agreement between them. Using all the radar data available, we present a preliminary climatology of atmospheric turbulence in the UTLS (upper troposphere and lower stratosphere) region above the MAARSY site showing a variability of more than 5 orders of magnitude inherent in turbulent energy dissipation rates. The derived ε values reveal a log-normal distribution with a negative skewness, and the ε profiles show an increase with height which is also the case for each individual month. Atmospheric turbulence based on our radar measurements reveals a seasonal variation but no clear diurnal variation in the UTLS region. Comparison of ε with the gradient Richardson number Ri shows that only 1.7 % of all the data with turbulence occur under the condition of Ri < 1 and that the values of ε under the condition of Ri < 1 are significantly larger than those under Ri > 1. Further, there is a roughly negative correlation between ε and Ri that is independent of the scale dependence of Ri. Turbulence under active dynamical conditions (velocity of horizontal wind U > 10 m s−1) is significantly stronger than under quiet conditions (U < 10 m s−1). Last but not least, the derived ε values are compared with the corresponding vertical shears of background wind velocity showing a linear relation with a corresponding correlation coefficient r = 58 % well above the 99.9 % significance level. This implies that wind shears play an important role in the turbulence generation in the troposphere and lower stratosphere (through the Kelvin–Helmholtz instability).
- ItemThe Turbopause experiment: Atmospheric stability and turbulent structure spanning the turbopause altitude(München : European Geopyhsical Union, 2011) Lehmacher, G.A.; Scott, T.D.; Larsen, M.F.; Bilén, S.G.; Croskey, C.L.; Mitchell, J.D.; Rapp, M.; Lübken, F.-J.; Collins, R.L.Very few sequences of high resolution wind and temperature measurements in the lower thermosphere are available in the literature, which makes it difficult to verify the simulation results of models that would provide better understanding of the complex dynamics of the region. To address this problem the Turbopause experiment used four rockets launched over a period of approximately two hours from Poker Flat Research Range, Alaska (64° N, 147° W) on the night of 17–18 February 2009. All four rocket payloads released trimethyl aluminum trails for neutral wind and turbulence measurements, and two of the rockets carried ionization gauges and fixed-bias Langmuir probes measuring neutral and electron densities, small-scale fluctuations and neutral temperatures. Two lidars monitored temperature structure and sodium densities. The observations were made under quiet geomagnetic conditions and show persistence in the wind magnitudes and shears throughout the observing period while being modulated by inertia-gravity waves. High resolution temperature profiles show the winter polar mesosphere and lower thermosphere in a state of relatively low stability with several quasi-adiabatic layers between 74 and 103 km. Temperature and wind data were combined to calculate Richardson number profiles. Evidence for turbulence comes from simultaneous observations of density fluctuations and downward transport of sodium in a mixed layer near 75 km; the observation of turbulent fluctuations and energy dissipation from 87–90 km; and fast and irregular trail expansion at 90–93 km, and especially between 95 to 103 km. The regions of turbulent trails agree well with regions of quasi-adiabatic temperature gradients. Above 103 km, trail diffusion was mainly laminar; however, unusual features and vortices in the trail diffusion were observed up to 118 km that have not been as prevalent or as clearly evident in earlier trail releases.
- ItemSmall-scale structures in neutrals and charged aerosol particles as observed during the ECOMA/MASS rocket campaign(München : European Geopyhsical Union, 2009) Strelnikov, B.; Rapp, M.; Strelnikova, I.; Engler, N.; Latteck, R.We present results of in situ measurements of neutral temperature during the ECOMA/MASS rocket campaign. We present and compare results of turbulence measurements conducted simultaneously by both in situ and doppler radar techniques. We show that the derived values of the turbulence energy dissipation rates are similar on average. We also find a region with a near adiabatic lapse rate with turbulence detected at the upper and lower edge. We note that it is consistent with expectation for a Kelvin-Helmholtz instability. We also present an estimate of the Schmidt numbers, Sc, for the charged aerosols that utilizes in situ measured small-scale density fluctuations of charged aerosols and both in situ and radar turbulence measurements. The derived Schmidt numbers fall within the range between 100 and 4500. This result agrees with previous estimates based on multi-frequency observations of PMSE (Rapp et al., 2008) and also with estimates of microphysical parameters presented in the companion paper by Rapp et al. (2009).