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- ItemSurface and bulk electronic structure of the unconventional superconductor Sr2RuO4: Unusual splitting of the β band(Milton Park : Taylor & Francis, 2012) Zabolotnyy, V.B.; Carleschi, E.; Kim, T.K.; Kordyuk, A.A.; Trinckauf, J.; Geck, J.; Evtushinsky, D.; Doyle, B.P.; Fittipaldi, R.; Cuoco, M.; Vecchione, A.; Büchner, B.; Borisenko, S.V.We present an angle-resolved photoemission study of the surface and bulk electronic structure of the single layer ruthenate Sr2RuO4. As the early studies by photoemission and scanning tunneling microscopy were confronted with a problem of surface reconstruction, surface ageing was previously proposed as a possible remedy to access the bulk states. Here, we suggest an alternative way by demonstrating that, in the case of Sr2RuO4, circularly polarized light can be used to disentangle the signals from the bulk and surface layers, thus opening the possibility to investigate many-body interactions both in bulk and surface bands. The proposed procedure results in improved momentum resolution, which enabled us to detect an unexpected splitting of the surface β band. We discuss the origin of the splitting of the β band and the possible connection with the Rashba effect at the surface.
- ItemDynamics of graphene growth on a metal surface: A time-dependent photoemission study(Milton Park : Taylor & Francis, 2009) Grüneis, Alexander; Kummer, Kurt; Vyalikh, Denis V.Applying time-dependent photoemission we unravel the graphene growth process on a metallic surface by chemical vapor deposition (CVD). Graphene CVD growth is in stark contrast to the standard growth process of two-dimensional films because it is self-limiting and stops as soon as a monolayer of graphene has been synthesized. Most importantly, a novel phase of metastable graphene was discovered that is characterized by permanent and simultaneous construction and deconstruction. The high quality and large area graphene flakes are characterized by angle-resolved photoemission, proving that they are indeed monolayer and cover the whole 1×1 cm Ni(111) substrate. These findings are of high relevance to the intensive search for reliable synthesis methods for large graphene flakes of controlled layer number.