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- ItemNew insights in sources of the sub-micrometre aerosol at Mt. Zeppelin observatory (Spitsbergen) in the year 2015(Stockholm : Stockholm University Press, 2019) Karl, Matthias; Leck, Caroline; Rad, Farshid Mashayekhy; Bäcklund, Are; Lopez-Aparicio, Susana; Heintzenberg, JostIn order to evaluate the potential impact of the Arctic anthropogenic emission sources it is essential to understand better the natural aerosol sources of the inner Arctic and the atmospheric processing of the aerosols during their transport in the Arctic atmosphere. A 1-year time series of chemically specific measurements of the sub-micrometre aerosol during 2015 has been taken at the Mt. Zeppelin observatory in the European Arctic. A source apportionment study combined measured molecular tracers as source markers, positive matrix factorization, analysis of the potential source distribution and auxiliary information from satellite data and ground-based observations. The annual average sub-micrometre mass was apportioned to regional background secondary sulphate (56%), sea spray (17%), biomass burning (15%), secondary nitrate (5.8%), secondary marine biogenic (4.5%), mixed combustion (1.6%), and two types of marine gel sources (together 0.7%). Secondary nitrate aerosol mainly contributed towards the end of summer and during autumn. During spring and summer, the secondary marine biogenic factor reached a contribution of up to 50% in some samples. The most likely origin of the mixed combustion source is due to oil and gas extraction activities in Eastern Siberia. The two marine polymer gel sources predominantly occurred in autumn and winter. The small contribution of the marine gel sources at Mt. Zeppelin observatory in summer as opposed to regions closer to the North Pole is attributed to differences in ocean biology, vertical distribution of phytoplankton, and the earlier start of the summer season.
- ItemInfluence of subtropical Rossby wave trains on planetary wave activity over Antarctica in September 2002(Stockholm : Stockholm University Press, 2015) Peters, Dieter H.W.; Vargin, PavelAt the beginning of September 2002, strong convection processes over south-eastern Indonesia and over south-eastern Africa have been observed. Due to the strong upper tropospheric divergent outflow, two Rossby wave trains (RWTs) were generated. Their south-eastward propagation was controlled by the mean background flow. These two wave trains are visible in observations. It is hypothesised that these wave trains cause enhanced planetary wave activity fluxes which are a result of an amplified planetary wave 2 in the upper troposphere/lower stratosphere over Antarctica. Such a change of the planetary wave structure was diagnosed in September 2002, prior to the first observed major sudden stratospheric warming event on the Southern Hemisphere. A simplified version of GCM ECHAM4 is used to evaluate the hypothesis. Sensitivity experiments were performed for a mean background flow similar to September 2002. Furthermore, the wave maker approach was used to generate Rossby waves in the subtropical upper troposphere at two distinct locations which are corresponding to the observed regions of divergent outflow. As a main result, after about 2 weeks of model integration with wave maker forcing, we find two RWTs with a south-eastward propagation inducing a polar amplification of planetary wave 2 in the upper troposphere and lower/middle stratosphere. The poleward wave activity flux is enhanced in comparison to the control run without any wave maker forcing. The convergence of the Eliassen–Palm flux causes a 25% deceleration of zonal mean zonal wind in the model stratosphere but no wind reversal. Sensitivity runs support the robustness of these results. The obtained model results highlight the mechanism and confirm the hypothesis that enhanced planetary wave activity in austral polar region in 2002 is caused by enhanced subtropical forcing of two RWTs.