2021, Hort, O., Dubrouil, A., Khokhlova, M.A., Descamps, D., Petit, S., Burgy, F., Mével, E., Constant, E., Strelkov, V.V.

Extreme ultraviolet (XUV) radiation finds numerous applications in spectroscopy. When the XUV light is generated via high-order harmonic generation (HHG), it may be produced in the form of attosecond pulses, allowing access to unprecedented ultrafast phenomena. However, the HHG efficiency remains limited. Here we present an observation of a new regime of coherent XUV emission which has a potential to provide higher XUV intensity, vital for applications. We explain the process by high-order parametric generation, involving the combined emission of THz and XUV photons, where the phase matching is very robust against ionization. This introduces a way to use higher-energy driving pulses, thus generating more XUV photons.

2010, Mauritsson, J., Remetter, T., Swoboda, M., Klünder, K., L'Huillier, A., Schafer, K.J., Ghafur, O., Kelkensberg, F., Siu, W., Johnsson, P., Vrakking, M.J.J., Znakovskaya, I., Uphues, T., Zherebtsov, S., Kling, M.F., Lépine, F., Benedetti, E., Ferrari, F., Sansone, G., Nisoli, M.

We present an interferometric pump-probe technique for the characterization of attosecond electron wave packets (WPs) that uses a free WP as a reference to measure a bound WP. We demonstrate our method by exciting helium atoms using an attosecond pulse (AP) with a bandwidth centered near the ionization threshold, thus creating both a bound and a free WP simultaneously. After a variable delay, the bound WP is ionized by a few-cycle infrared laser precisely synchronized to the original AP. By measuring the delay-dependent photoelectron spectrum we obtain an interferogram that contains both quantum beats as well as multipath interference. Analysis of the interferogram allows us to determine the bound WP components with a spectral resolution much better than the inverse of the AP duration. © 2010 The American Physical Society.