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Evidence for Efficient Pathway to Produce Slow Electrons by Ground-state Dication in Clusters

2017, You, Daehyun, Fukuzawa, Hironobu, Sakakibara, Yuta, Takanashi, Tsukasa, Ito, Yuta, Maliyar, Gianluigi G., Motomura, Koji, Nagaya, Kiyonobu, Nishiyama, Toshiyuki, Asa, Kazuki, Sato, Yuhiro, Saito, Norio, Oura, Masaki, Schöffler, Markus, Kastirke, Gregor, Hergenhahn, Uwe, Stumpf, Vasili, Gohkberg, Kirill, Kuleff, Alexander I., Cederbaum, Lorenz S., Ueda, Kiyoshi

We present an experimental evidence for a so-far unobserved, but potentially very important step relaxation cascades following inner-shell ionization of a composite system: Multiply charged ionic states created after Auger decay may be neutralized by electron transfer from a neighboring species, producing at the same time a low-energy free electron. This electron transfer-mediated decay (ETMD) called process is effective even after Auger decay into the dicationic ground state. Here, we report the ETMD of Ne2+ produced after Ne 1s photoionization in Ne-Kr mixed clusters.