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Impact of Mn-Pn intermixing on magnetic properties of an intrinsic magnetic topological insulator: the µSR perspective

2023, Sahoo, M., Salman, Z., Allodi, G., Isaeva, A., Folkers, L., Wolter, A.U.B., Büchner, B., De Renzi, R.

We investigated the magnetic properties of polycrystalline samples of the intrinsic magnetic topological insulators MnPn2Te4, with pnictogen Pn = Sb, Bi, by bulk magnetization and μSR. DC susceptibility detects the onset of magnetic ordering at TN = 27 K and 24 K and a field dependence of the macroscopic magnetization compatible with ferri- (or ferro-) and atiferro- magnetic ordering, respectively. Weak transverse field (wTF) Muon Spin Rotation (μSR) confirms the homogeneous bulk nature of magnetic ordering at the same two distinct transition temperatures. Zero Field (ZF) μSR shows that the Sb based material displays a broader distribution of internal field at the muon, in accordance with a larger deviation from the stoichiomectric composition and a higher degree of positional disorder (Mn at the Pn(6c) site), which however does not affect significantly the sharpness of the thermodynamic transition, as detected by the muon magnetic volume fraction and the observability of a critical divergence in the longitudinal and transverse muon relaxation rates.

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Piezoelectric-driven uniaxial pressure cell for muon spin relaxation and neutron scattering experiments

2020, Ghosh, Shreenanda, Brückner, Felix, Nikitin, Artem, Grinenko, Vadim, Elender, Matthias, Mackenzie, Andrew P., Luetkens, Hubertus, Klauss, Hans-Henning, Hicks, Clifford W.

We present a piezoelectric-driven uniaxial pressure cell that is optimized for muon spin relaxation and neutron scattering experiments and that is operable over a wide temperature range including cryogenic temperatures. To accommodate the large samples required for these measurement techniques, the cell is designed to generate forces up to ∼1000 N. To minimize the background signal, the space around the sample is kept as open as possible. We demonstrate here that by mounting plate-like samples with epoxy, a uniaxial stress exceeding 1 GPa can be achieved in an active volume of at least 5 mm3. We show that for practical operation, it is important to monitor both the force and displacement applied to the sample. In addition, because time is critical during facility experiments, samples are mounted in detachable holders that can be rapidly exchanged. The piezoelectric actuators are likewise contained in an exchangeable cartridge. © 2020 Author(s).