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Attractive Dipolar Coupling between Stacked Exciton Fluids

2019, Hubert, Colin, Baruchi, Yifat, Mazuz-Harpaz, Yotam, Cohen, Kobi, Biermann, Klaus, Lemeshko, Mikhail, West, Ken, Pfeiffer, Loren, Rapaport, Ronen, Santos, Paulo

Dipolar coupling plays a fundamental role in the interaction between electrically or magnetically polarized species such as magnetic atoms and dipolar molecules in a gas or dipolar excitons in the solid state. Unlike Coulomb or contactlike interactions found in many atomic, molecular, and condensed-matter systems, this interaction is long-ranged and highly anisotropic, as it changes from repulsive to attractive depending on the relative positions and orientation of the dipoles. Because of this unique property, many exotic, symmetry-breaking collective states have been recently predicted for cold dipolar gases, but only a few have been experimentally detected and only in dilute atomic dipolar Bose-Einstein condensates. Here, we report on the first observation of attractive dipolar coupling between excitonic dipoles using a new design of stacked semiconductor bilayers. We show that the presence of a dipolar exciton fluid in one bilayer modifies the spatial distribution and increases the binding energy of excitonic dipoles in a vertically remote layer. The binding energy changes are explained using a many-body polaron model describing the deformation of the exciton cloud due to its interaction with a remote dipolar exciton. The surprising nonmonotonic dependence on the cloud density indicates the important role of dipolar correlations, which is unique to dense, strongly interacting dipolar solid-state systems. Our concept provides a route for the realization of dipolar lattices with strong anisotropic interactions in semiconductor systems, which open the way for the observation of theoretically predicted new and exotic collective phases, as well as for engineering and sensing their collective excitations.

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Exploring the intrinsic limit of the charge-carrier-induced increase of the Curie temperature of Lu- and La-doped EuO thin films

2020, Held, R., Mairoser, T., Melville, A., Mundy, J.A., Holtz, M.E., Hodash, D., Wang, Z., Heron, J.T., Dacek, S.T., Holländer, B., Muller, D.A., Schlom, D.G.

Raising the Curie temperature TC of the highly spin-polarized semiconductor EuO by doping it with rare-earth elements is a strategy to make EuO more technologically relevant to spintronics. The increase of TC with free carrier density n and the surprisingly low dopant activation p, found in Gd-doped EuO thin films [Mairoser et al., Phys. Rev. Lett. 105, 257206 (2010)], raised the important question of whether TC could be considerably enhanced by increasing p. Using a low-temperature growth method for depositing high-quality Lu-doped EuO films we attain high dopant activation (p) values of up to 67%, effectively more than doubling p as compared to adsorption-controlled growth of Lu- and Gd-doped EuO. Relating n, p, and lattice compression of La- and Lu-doped EuO films grown at different temperatures to the TC of these samples allows us to identify several different mechanisms influencing TC and causing an experimental maximum in TC. In addition, scanning transmission electron microscopy in combination with electron energy loss spectroscopy measurements on La-doped EuO indicate that extensive dopant clustering is one, but not the sole reason for dopant deactivation in rare-earth doped EuO films.