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Measurement report: Balloon-borne in situ profiling of Saharan dust over Cyprus with the UCASS optical particle counter

2021, Kezoudi, Maria, Tesche, Matthias, Smith, Helen, Tsekeri, Alexandra, Baars, Holger, Dollner, Maximilian, Estellés, Víctor, Bühl, Johannes, Weinzierl, Bernadett, Ulanowski, Zbigniew, Müller, Detlef, Amiridis, Vassilis

This paper presents measurements of mineral dust concentration in the diameter range from 0.4 to 14.0 µm with a novel balloon-borne optical particle counter, the Universal Cloud and Aerosol Sounding System (UCASS). The balloon launches were coordinated with ground-based active and passive remote-sensing observations and airborne in situ measurements with a research aircraft during a Saharan dust outbreak over Cyprus from 20 to 23 April 2017. The aerosol optical depth at 500 nm reached values up to 0.5 during that event over Cyprus, and particle number concentrations were as high as 50 cm−3 for the diameter range between 0.8 and 13.9 µm. Comparisons of the total particle number concentration and the particle size distribution from two cases of balloon-borne measurements with aircraft observations show reasonable agreement in magnitude and shape despite slight mismatches in time and space. While column-integrated size distributions from balloon-borne measurements and ground-based remote sensing show similar coarse-mode peak concentrations and diameters, they illustrate the ambiguity related to the missing vertical information in passive sun photometer observations. Extinction coefficient inferred from the balloon-borne measurements agrees with those derived from coinciding Raman lidar observations at height levels with particle number concentrations smaller than 10 cm−3 for the diameter range from 0.8 to 13.9 µm. An overestimation of the UCASS-derived extinction coefficient of a factor of 2 compared to the lidar measurement was found for layers with particle number concentrations that exceed 25 cm−3, i.e. in the centre of the dust plume where particle concentrations were highest. This is likely the result of a variation in the refractive index and the shape and size dependency of the extinction efficiency of dust particles along the UCASS measurements. In the future, profile measurements of the particle number concentration and particle size distribution with the UCASS could provide a valuable addition to the measurement capabilities generally used in field experiments that are focussed on the observation of coarse aerosols and clouds.

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On the upper tropospheric formation and occurrence of high and thin cirrus clouds during anticyclonic poleward Rossby wave breaking events

2010, Eixmann, Ronald, Peters, Dieter H.W., Zülicke, Christoph, Gerding, Michael, Dörnbrack, Andreas

Ground-based lidar measurements and balloon soundings were employed to examine the dynamical link between anticyclonic Rossby wave breaking and cirrus clouds from 13 to 15 February 2006. For this event, an air mass with low Ertel’s potential vorticity appeared over Central Europe. In the tropopause region, this air mass was accompanied with both an area of extreme cold temperatures placed northeastward, and an area of high specific humidity, located southwestward. ECMWF analyses reveal a strong adiabatic northeastward and upward transport of water vapour within the warm conveyor belt on the western side of the ridge over Mecklenburg, Northern Germany. The backscatter lidar at K¨uhlungsborn (54.1◦N, 11.8◦E) clearly identified cirrus clouds at between 9 and 11.4 km height. In the tropopause region high-vertical resolution radiosoundings showed layers of subsaturated water vapour over ice but with a relative humidity over ice >80%. Over Northern Germany radiosondes indicated anticyclonically rotating winds in agreement with backward trajectories of ECMWF analyses in the upper troposphere, which were accompanied by a relatively strong increase of the tropopause height on 14 February. Based on ECMWF data the strong link between the large-scale structure, updraft and ice water content was shown.