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- ItemLong-term study on coarse mode aerosols in the Amazon rain forest with the frequent intrusion of Saharan dust plumes(Katlenburg-Lindau : EGU, 2018) Moran-Zuloaga, Daniel; Ditas, Florian; Walter, David; Saturno, Jorge; Brito, Joel; Carbone, Samara; Chi, Xuguang; Hrabě de Angelis, Isabella; Baars, Holger; Godoi, Ricardo H. M.; Heese, Birgit; Holanda, Bruna A.; Lavrič, Jošt V.; Martin, Scot T.; Ming, Jing; Pöhlker, Mira L.; Ruckteschler, Nina; Su, Hang; Wang, Yaqiang; Wang, Qiaoqiao; Wang, Zhibin; Weber, Bettina; Wolff, Stefan; Artaxo, Paulo; Pöschl, Ulrich; Andreae, Meinrat O.; Pöhlker, ChristopherIn the Amazonian atmosphere, the aerosol coarse mode comprises a complex, diverse, and variable mixture of bioaerosols emitted from the rain forest ecosystem, long-range transported Saharan dust (we use Sahara as shorthand for the dust source regions in Africa north of the Equator), marine aerosols from the Atlantic Ocean, and coarse smoke particles from deforestation fires. For the rain forest, the coarse mode particles are of significance with respect to biogeochemical and hydrological cycling, as well as ecology and biogeography. However, knowledge on the physicochemical and biological properties as well as the ecological role of the Amazonian coarse mode is still sparse. This study presents results from multi-year coarse mode measurements at the remote Amazon Tall Tower Observatory (ATTO) site. It combines online aerosol observations, selected remote sensing and modeling results, as well as dedicated coarse mode sampling and analysis. The focal points of this study are a systematic characterization of aerosol coarse mode abundance and properties in the Amazonian atmosphere as well as a detailed analysis of the frequent, pulse-wise intrusion of African long-range transport (LRT) aerosols (comprising Saharan dust and African biomass burning smoke) into the Amazon Basin.We find that, on a multi-year time scale, the Amazonian coarse mode maintains remarkably constant concentration levels (with 0.4 cmĝ'3 and 4.0 μg mĝ'3 in the wet vs. 1.2 cmĝ'3 and 6.5 μg mĝ'3 in the dry season) with rather weak seasonality (in terms of abundance and size spectrum), which is in stark contrast to the pronounced biomass burning-driven seasonality of the submicron aerosol population and related parameters. For most of the time, bioaerosol particles from the forest biome account for a major fraction of the coarse mode background population. However, from December to April there are episodic intrusions of African LRT aerosols, comprising Saharan dust, sea salt particles from the transatlantic passage, and African biomass burning smoke. Remarkably, during the core period of this LRT season (i.e., February-March), the presence of LRT influence, occurring as a sequence of pulse-like plumes, appears to be the norm rather than an exception. The LRT pulses increase the coarse mode concentrations drastically (up to 100 μg mĝ'3) and alter the coarse mode composition as well as its size spectrum. Efficient transport of the LRT plumes into the Amazon Basin takes place in response to specific mesoscale circulation patterns in combination with the episodic absence of rain-related aerosol scavenging en route. Based on a modeling study, we estimated a dust deposition flux of 5-10 kg haĝ'1 aĝ'1 in the region of the ATTO site. Furthermore, a chemical analysis quantified the substantial increase of crustal and sea salt elements under LRT conditions in comparison to the background coarse mode composition. With these results, we estimated the deposition fluxes of various elements that are considered as nutrients for the rain forest ecosystem. These estimates range from few g haĝ'1 aĝ'1 up to several hundreds of g haĝ'1 aĝ'1 in the ATTO region.The long-term data presented here provide a statistically solid basis for future studies of the manifold aspects of the dynamic coarse mode aerosol cycling in the Amazon. Thus, it may help to understand its biogeochemical relevance in this ecosystem as well as to evaluate to what extent anthropogenic influences have altered the coarse mode cycling already.
- ItemA State-Of-The-Art Perspective on the Characterization of Subterranean Estuaries at the Regional Scale(Lausanne : Frontiers Media, 2021) Moosdorf, Nils; Böttcher, Michael Ernst; Adyasari, Dini; Erkul, Ercan; Gilfedder, Benjamin S.; Greskowiak, Janek; Jenner, Anna-Kathrina; Kotwicki, Lech; Massmann, Gudrun; Müller-Petke, Mike; Oehler, Till; Post, Vincent; Prien, Ralf; Scholten, Jan; Siemon, Bernhard; Ehlert von Ahn, Cátia Milene; Walther, Marc; Waska, Hannelore; Wunderlich, Tina; Mallast, UlfSubterranean estuaries the, subsurface mixing zones of terrestrial groundwater and seawater, substantially influence solute fluxes to the oceans. Solutes brought by groundwater from land and solutes brought from the sea can undergo biogeochemical reactions. These are often mediated by microbes and controlled by reactions with coastal sediments, and determine the composition of fluids discharging from STEs (i.e., submarine groundwater discharge), which may have consequences showing in coastal ecosystems. While at the local scale (meters), processes have been intensively studied, the impact of subterranean estuary processes on solute fluxes to the coastal ocean remains poorly constrained at the regional scale (kilometers). In the present communication, we review the processes that occur in STEs, focusing mainly on fluid flow and biogeochemical transformations of nitrogen, phosphorus, carbon, sulfur and trace metals. We highlight the spatio-temporal dynamics and measurable manifestations of those processes. The objective of this contribution is to provide a perspective on how tracer studies, geophysical methods, remote sensing and hydrogeological modeling could exploit such manifestations to estimate the regional-scale impact of processes in STEs on solute fluxes to the coastal ocean.
- ItemThe Earth system model CLIMBER-X v1.0 - Part 2: The global carbon cycle(Katlenburg-Lindau : Copernicus, 2023) Willeit, Matteo; Ilyina, Tatiana; Liu, Bo; Heinze, Christoph; Perrette, Mahé; Heinemann, Malte; Dalmonech, Daniela; Brovkin, Victor; Munhoven, Guy; Börker, Janine; Hartmann, Jens; Romero-Mujalli, Gibran; Ganopolski, AndreyThe carbon cycle component of the newly developed Earth system model of intermediate complexity CLIMBER-X is presented. The model represents the cycling of carbon through the atmosphere, vegetation, soils, seawater and marine sediments. Exchanges of carbon with geological reservoirs occur through sediment burial, rock weathering and volcanic degassing. The state-of-the-art HAMOCC6 model is employed to simulate ocean biogeochemistry and marine sediment processes. The land model PALADYN simulates the processes related to vegetation and soil carbon dynamics, including permafrost and peatlands. The dust cycle in the model allows for an interactive determination of the input of the micro-nutrient iron into the ocean. A rock weathering scheme is implemented in the model, with the weathering rate depending on lithology, runoff and soil temperature. CLIMBER-X includes a simple representation of the methane cycle, with explicitly modelled natural emissions from land and the assumption of a constant residence time of CH4 in the atmosphere. Carbon isotopes 13C and 14C are tracked through all model compartments and provide a useful diagnostic for model-data comparison. A comprehensive evaluation of the model performance for the present day and the historical period shows that CLIMBER-X is capable of realistically reproducing the historical evolution of atmospheric CO2 and CH4 but also the spatial distribution of carbon on land and the 3D structure of biogeochemical ocean tracers. The analysis of model performance is complemented by an assessment of carbon cycle feedbacks and model sensitivities compared to state-of-the-art Coupled Model Intercomparison Project Phase 6 (CMIP6) models. Enabling an interactive carbon cycle in CLIMBER-X results in a relatively minor slow-down of model computational performance by ∼ 20 % compared to a throughput of ∼ 10 000 simulation years per day on a single node with 16 CPUs on a high-performance computer in a climate-only model set-up. CLIMBER-X is therefore well suited to investigating the feedbacks between climate and the carbon cycle on temporal scales ranging from decades to >100000 years.