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- ItemIncreasing the spatial resolution of cloud property retrievals from Meteosat SEVIRI by use of its high-resolution visible channel: implementation and examples(Katlenburg-Lindau : European Geosciences Union, 2021) Deneke, Hartwig; Barrientos-Velasco, Carola; Bley, Sebastian; Hünerbein, Anja; Lenk, Stephan; Macke, Andreas; Meirink, Jan Fokke; Schroedter-Homscheidt, Marion; Senf, Fabian; Wang, Ping; Werner, Frank; Witthuhn, JonasThe modification of an existing cloud property retrieval scheme for the Spinning Enhanced Visible and Infrared Imager (SEVIRI) instrument on board the geostationary Meteosat satellites is described to utilize its high-resolution visible (HRV) channel for increasing the spatial resolution of its physical outputs. This results in products with a nadir spatial resolution of 1×1ĝ€¯km2 compared to the standard 3×3ĝ€¯km2 resolution offered by the narrowband channels. This improvement thus greatly reduces the resolution gap between current geostationary and polar-orbiting meteorological satellite imagers. In the first processing step, cloudiness is determined from the HRV observations by a threshold-based cloud masking algorithm. Subsequently, a linear model that links the 0.6ĝ€¯μm, 0.8ĝ€¯μm, and HRV reflectances provides a physical constraint to incorporate the spatial high-frequency component of the HRV observations into the retrieval of cloud optical depth. The implementation of the method is described, including the ancillary datasets used. It is demonstrated that the omission of high-frequency variations in the cloud-absorbing 1.6ĝ€¯μm channel results in comparatively large uncertainties in the retrieved cloud effective radius, likely due to the mismatch in channel resolutions. A newly developed downscaling scheme for the 1.6ĝ€¯μm reflectance is therefore applied to mitigate the effects of this scale mismatch. Benefits of the increased spatial resolution of the resulting SEVIRI products are demonstrated for three example applications: (i) for a convective cloud field, it is shown that significantly better agreement between the distributions of cloud optical depth retrieved from SEVIRI and from collocated MODIS observations is achieved. (ii) The temporal evolution of cloud properties for a growing convective storm at standard and HRV spatial resolutions are compared, illustrating an improved contrast in growth signatures resulting from the use of the HRV channel. (iii) An example of surface solar irradiance, determined from the retrieved cloud properties, is shown, for which the HRV channel helps to better capture the large spatiotemporal variability induced by convective clouds. These results suggest that incorporating the HRV channel into the retrieval has potential for improving Meteosat-based cloud products for several application domains.
- ItemAerosol characteristics and particle production in the upper troposphere over the Amazon Basin(Katlenburg-Lindau : EGU, 2018) Andreae, Meinrat O.; Afchine, Armin; Albrecht, Rachel; Holanda, Bruna Amorim; Artaxo, Paulo; Barbosa, Henrique M. J.; Borrmann, Stephan; Cecchini, Micael A.; Costa, Anja; Dollner, Maximilian; Fütterer, Daniel; Järvinen, Emma; Jurkat, Tina; Klimach, Thomas; Konemann, Tobias; Knote, Christoph; Krämer, Martina; Krisna, Trismono; Machado, Luiz A. T.; Mertes, Stephan; Minikin, Andreas; Pöhlker, Christopher; Pöhlker, Mira L.; Pöschl, Ulrich; Rosenfeld, Daniel; Sauer, Daniel; Schlager, Hans; Schnaiter, Martin; Schneider, Johannes; Schulz, Christiane; Spanu, Antonio; Sperling, Vinicius B.; Voigt, Christiane; Walser, Adrian; Wang, Jian; Weinzierl, Bernadett; Wendisch, Manfred; Ziereis, HelmutAirborne observations over the Amazon Basin showed high aerosol particle concentrations in the upper troposphere (UT) between 8 and 15ĝ€km altitude, with number densities (normalized to standard temperature and pressure) often exceeding those in the planetary boundary layer (PBL) by 1 or 2 orders of magnitude. The measurements were made during the German–Brazilian cooperative aircraft campaign ACRIDICON–CHUVA, where ACRIDICON stands for
Aerosol, Cloud, Precipitation, and Radiation Interactions and Dynamics of Convective Cloud Systems
and CHUVA is the acronym forCloud Processes of the Main Precipitation Systems in Brazil: A Contribution to Cloud Resolving Modeling and to the GPM (global precipitation measurement)
, on the German High Altitude and Long Range Research Aircraft (HALO). The campaign took place in September–October 2014, with the objective of studying tropical deep convective clouds over the Amazon rainforest and their interactions with atmospheric trace gases, aerosol particles, and atmospheric radiation.
Aerosol enhancements were observed consistently on all flights during which the UT was probed, using several aerosol metrics, including condensation nuclei (CN) and cloud condensation nuclei (CCN) number concentrations and chemical species mass concentrations. The UT particles differed sharply in their chemical composition and size distribution from those in the PBL, ruling out convective transport of combustion-derived particles from the boundary layer (BL) as a source. The air in the immediate outflow of deep convective clouds was depleted of aerosol particles, whereas strongly enhanced number concentrations of small particles (< 90ĝ€nm diameter) were found in UT regions that had experienced outflow from deep convection in the preceding 5–72ĝ€h. We also found elevated concentrations of larger (> 90ĝ€nm) particles in the UT, which consisted mostly of organic matter and nitrate and were very effective CCN.
Our findings suggest a conceptual model, where production of new aerosol particles takes place in the continental UT from biogenic volatile organic material brought up by deep convection and converted to condensable species in the UT. Subsequently, downward mixing and transport of upper tropospheric aerosol can be a source of particles to the PBL, where they increase in size by the condensation of biogenic volatile organic compound (BVOC) oxidation products. This may be an important source of aerosol particles for the Amazonian PBL, where aerosol nucleation and new particle formation have not been observed. We propose that this may have been the dominant process supplying secondary aerosol particles in the pristine atmosphere, making clouds the dominant control of both removal and production of atmospheric particles. - ItemScheme for calculation of multi-layer cloudiness and precipitation for climate models of intermediate complexity(München : European Geopyhsical Union, 2013) Eliseev, A.V.; Coumou, D.; Chernokulsky, A.V.; Petoukhov, V.; Petri, S.In this study we present a scheme for calculating the characteristics of multi-layer cloudiness and precipitation for Earth system models of intermediate complexity (EMICs). This scheme considers three-layer stratiform cloudiness and single-column convective clouds. It distinguishes between ice and droplet clouds as well. Precipitation is calculated by using cloud lifetime, which depends on cloud type and phase as well as on statistics of synoptic and convective disturbances. The scheme is tuned to observations by using an ensemble simulation forced by the ERA-40-derived climatology for 1979–2001. Upon calibration, the scheme realistically reproduces basic features of fields of cloud fractions, cloud water path, and precipitation. The simulated globally and annually averaged total cloud fraction is 0.59, and the simulated globally averaged annual precipitation is 100 cm yr−1. Both values agree with empirically derived values. The simulated cloud water path is too small, probably because the simulated vertical extent of stratiform clouds is too small. Geographical distribution and seasonal changes of calculated cloud fraction and precipitation are broadly realistic as well. However, some important regional biases still remain in the scheme, e.g. too little precipitation in the tropics. We discuss possibilities for future improvements in the scheme.
- ItemSources, seasonality, and trends of southeast US aerosol: an integrated analysis of surface, aircraft, and satellite observations with the GEOS-Chem chemical transport model(Katlenburg-Lindau : EGU, 2015) Kim, P.S.; Jacob, D.J.; Fisher, J.A.; Travis, K.; Yu, K.; Zhu, L.; Yantosca, R.M.; Sulprizio, M.P.; Jimenez, J.L.; Campuzano-Jost, P.; Froyd, K.D.; Liao, J.; Hair, J.W.; Fenn, M.A.; Butler, C.F.; Wagner, N.L.; Gordon, T.D.; Welti, A.; Wennberg, P.O.; Crounse, J.D.; St. Clair, J.M.; Teng, A.P.; Millet, D.B.; Schwarz, J.P.; Markovic, M.Z.; Perring, A.E.We use an ensemble of surface (EPA CSN, IMPROVE, SEARCH, AERONET), aircraft (SEAC4RS), and satellite (MODIS, MISR) observations over the southeast US during the summer–fall of 2013 to better understand aerosol sources in the region and the relationship between surface particulate matter (PM) and aerosol optical depth (AOD). The GEOS-Chem global chemical transport model (CTM) with 25 × 25 km2 resolution over North America is used as a common platform to interpret measurements of different aerosol variables made at different times and locations. Sulfate and organic aerosol (OA) are the main contributors to surface PM2.5 (mass concentration of PM finer than 2.5 μm aerodynamic diameter) and AOD over the southeast US. OA is simulated successfully with a simple parameterization, assuming irreversible uptake of low-volatility products of hydrocarbon oxidation. Biogenic isoprene and monoterpenes account for 60 % of OA, anthropogenic sources for 30 %, and open fires for 10 %. 60 % of total aerosol mass is in the mixed layer below 1.5 km, 25 % in the cloud convective layer at 1.5–3 km, and 15 % in the free troposphere above 3 km. This vertical profile is well captured by GEOS-Chem, arguing against a high-altitude source of OA. The extent of sulfate neutralization (f = [NH4+]/(2[SO42−] + [NO3−]) is only 0.5–0.7 mol mol−1 in the observations, despite an excess of ammonia present, which could reflect suppression of ammonia uptake by OA. This would explain the long-term decline of ammonium aerosol in the southeast US, paralleling that of sulfate. The vertical profile of aerosol extinction over the southeast US follows closely that of aerosol mass. GEOS-Chem reproduces observed total column aerosol mass over the southeast US within 6 %, column aerosol extinction within 16 %, and space-based AOD within 8–28 % (consistently biased low). The large AOD decline observed from summer to winter is driven by sharp declines in both sulfate and OA from August to October. These declines are due to shutdowns in both biogenic emissions and UV-driven photochemistry. Surface PM2.5 shows far less summer-to-winter decrease than AOD and we attribute this in part to the offsetting effect of weaker boundary layer ventilation. The SEAC4RS aircraft data demonstrate that AODs measured from space are consistent with surface PM2.5. This implies that satellites can be used reliably to infer surface PM2.5 over monthly timescales if a good CTM representation of the aerosol vertical profile is available.
- ItemNear-global aerosol mapping in the upper troposphere and lowermost stratosphere with data from the CARIBIC project(Milton Park : Taylor & Francis, 2017) Heintzenberg, Jost; Hermann, Markus; Weigelt, Andreas; Kapustin, Vladimir; Anderson, Bruce; Thornhill, Kenneth; Van Velthoven, Peter; Zahn, Andreas; Brenninkmeijer, CarlThis study extrapolates aerosol data of the CARIBIC project from 1997 until June 2008 in along trajectories to compose large-scale maps and vertical profiles of submicrometre particle concentrations in the upper troposphere and lowermost stratosphere (UT/LMS). The extrapolation was validated by comparing extrapolated values with CARIBIC data measured near the respective trajectory position and by comparing extrapolated CARIBIC data to measurements by other experiments near the respective trajectory positions. Best agreement between extrapolated and measured data is achieved with particle lifetimes longer than the maximum length of used trajectories. The derived maps reveal regions of strong and frequent new particle formation, namely the Tropical Central and Western Africa with the adjacent Atlantic, South America, the Caribbean and Southeast Asia. These regions of particle formation coincide with those of frequent deep convective clouds. Vertical particle concentration profiles for the troposphere and the stratosphere confirm statistically previous results indicating frequent new particle formation in the tropopause region. There was no statistically significant increase in Aitken mode particle concentration between the first period of CARIBIC operation, 1997–2002, and the second period, 2004–2009. However, a significant increase in concentration occurred within the latter period when considering it in isolation.