Plasmon-driven sequential chemical reactions in an aqueous environment

dc.bibliographicCitation.firstPage5407eng
dc.bibliographicCitation.journalTitleScientific Reportseng
dc.bibliographicCitation.lastPage1067eng
dc.bibliographicCitation.volume4eng
dc.contributor.authorZhang, X.
dc.contributor.authorWang, P.
dc.contributor.authorZhang, Z.
dc.contributor.authorFang, Y.
dc.contributor.authorSun, M.
dc.date.accessioned2020-11-20T17:21:10Z
dc.date.available2020-11-20T17:21:10Z
dc.date.issued2014
dc.description.abstractPlasmon-driven sequential chemical reactions were successfully realized in an aqueous environment. In an electrochemical environment, sequential chemical reactions were driven by an applied potential and laser irradiation. Furthermore, the rate of the chemical reaction was controlled via pH, which provides indirect evidence that the hot electrons generated from plasmon decay play an important role in plasmon-driven chemical reactions. In acidic conditions, the hot electrons were captured by the abundant H + in the aqueous environment, which prevented the chemical reaction. The developed plasmon-driven chemical reactions in an aqueous environment will significantly expand the applications of plasmon chemistry and may provide a promising avenue for green chemistry using plasmon catalysis in aqueous environments under irradiation by sunlight.eng
dc.description.versionpublishedVersioneng
dc.identifier.urihttps://doi.org/10.34657/4595
dc.identifier.urihttps://oa.tib.eu/renate/handle/123456789/5966
dc.language.isoengeng
dc.publisherLondon : Nature Publishing Groupeng
dc.relation.doihttps://doi.org/10.1038/srep05407
dc.relation.issn2045-2322
dc.rights.licenseCC BY-NC-SA 4.0 Unportedeng
dc.rights.urihttps://creativecommons.org/licenses/by-nc-sa/4.0/eng
dc.subject.ddc620eng
dc.subject.otherelectrochemical environmenteng
dc.subject.otherchemical reactioneng
dc.subject.otheraqueous environmenteng
dc.titlePlasmon-driven sequential chemical reactions in an aqueous environmenteng
dc.typeArticleeng
dc.typeTexteng
tib.accessRightsopenAccesseng
wgl.contributorIPHTeng
wgl.subjectIngenieurwissenschafteneng
wgl.typeZeitschriftenartikeleng
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