Extended high-harmonic spectra through a cascade resonance in confined quantum systems

Abstract

The study of high-harmonic generation in confined quantum systems is vital to establishing a complete physical picture of harmonic generation from atoms and molecules to bulk solids. Based on a multilevel approach, we demonstrate how intraband resonances significantly influence the harmonic spectra via charge pumping to the higher subbands and thus redefine the cutoff laws. As a proof of principle, we consider the interaction of graphene nanoribbons, with zigzag as well as armchair terminations, and resonant fields polarized along the cross-ribbon direction. Here, this effect is particularly prominent due to many nearly equiseparated energy levels. In such a scenario, a cascade resonance effect can take place in high-harmonic generation when the field strength is above a critical threshold, which is completely different from the harmonic generation mechanism of atoms, molecules, and bulk solids. We further discuss the implications not only for other systems in a nanoribbon geometry, but also systems where only a few subbands (energy levels) meet this frequency-matching condition by considering a generalized multilevel Hamiltonian. Our study highlights that cascade resonance has a fundamentally distinct influence on the laws of harmonic generation, specifically the cutoff laws based on laser duration, field strength, and wavelength, thus unraveling additional insights in solid-state high-harmonic generation.