Co-generation of Ammonia and H2 from H2O Vapor and N2 Using a Membrane Electrode Assembly
dc.bibliographicCitation.firstPage | 62 | eng |
dc.bibliographicCitation.issue | 44228 | eng |
dc.bibliographicCitation.journalTitle | Chemie-Ingenieur-Technik | eng |
dc.bibliographicCitation.lastPage | 69 | eng |
dc.bibliographicCitation.volume | 92 | eng |
dc.contributor.author | Kugler, Kurt | |
dc.contributor.author | Kriescher, Stefanie M.A. | |
dc.contributor.author | Giela, Martin | |
dc.contributor.author | Hosseiny, Schwan | |
dc.contributor.author | Thimm, Kristof | |
dc.contributor.author | Wessling, Matthias | |
dc.date.accessioned | 2021-07-29T13:26:13Z | |
dc.date.available | 2021-07-29T13:26:13Z | |
dc.date.issued | 2020 | |
dc.description.abstract | The direct electrochemical synthesis of NH3 from nitrogen and water vapor without the use of a fossil carbon source is highly desired. This synthesis is a viable option to store energy and produce fertilizer precursors. Here, a new Pt-free membrane electrode assembly is presented. An electrochemical membrane reactor demonstrates the feasibility of co-generating NH3 and H2 directly from nitrogen and water vapor at ambient conditions. An unprecedented high NH3-specific current efficiency of up to 27.5% using Ti as cathodic catalyst is reported. The co-generation can be tuned by the balance of process parameters. © 2019 The Authors. Published by WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim | eng |
dc.description.version | publishedVersion | eng |
dc.identifier.uri | https://oa.tib.eu/renate/handle/123456789/6419 | |
dc.identifier.uri | https://doi.org/10.34657/5466 | |
dc.language.iso | eng | eng |
dc.publisher | Weinheim : Wiley-VCH | eng |
dc.relation.doi | https://doi.org/10.1002/cite.201900090 | |
dc.relation.essn | 1522-2640 | |
dc.relation.issn | 0009-286X | |
dc.rights.license | CC BY-NC-ND 4.0 Unported | eng |
dc.rights.uri | https://creativecommons.org/licenses/by-nc-nd/4.0/ | eng |
dc.subject.ddc | 540 | eng |
dc.subject.ddc | 660 | eng |
dc.subject.other | Ammonia | eng |
dc.subject.other | Electrochemical nitrogen reduction | eng |
dc.subject.other | Haber process | eng |
dc.subject.other | Membrane electrode assembly | eng |
dc.title | Co-generation of Ammonia and H2 from H2O Vapor and N2 Using a Membrane Electrode Assembly | eng |
dc.type | Article | eng |
dc.type | Text | eng |
tib.accessRights | openAccess | eng |
wgl.contributor | DWI | eng |
wgl.subject | Chemie | eng |
wgl.type | Zeitschriftenartikel | eng |
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