Earth-abundant photocatalytic systems for the visible-light-driven reduction of CO2 to CO

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dc.bibliographicCitation.firstPage2356
dc.bibliographicCitation.issue10
dc.bibliographicCitation.lastPage2360
dc.bibliographicCitation.volume19
dc.contributor.authorRosas-Hernández, Alonso
dc.contributor.authorSteinlechner, Christoph
dc.contributor.authorJunge, Henrik
dc.contributor.authorBeller, Matthias
dc.date.accessioned2023-03-01T05:37:47Z
dc.date.available2023-03-01T05:37:47Z
dc.date.issued2017
dc.description.abstractHerein, we report a highly selective photocatalytic system, based on an in situ copper photosensitizer and an iron catalyst, for the reduction of CO2 to CO. Turnover numbers (TON) up to 487 (5 h) with selectivities up to 99% and ΦCO = 13.3% were observed. Stern-Volmer analysis allowed us to establish a reductive quenching mechanism between the Cu PS and electron donor.eng
dc.description.versionpublishedVersioneng
dc.identifier.urihttps://oa.tib.eu/renate/handle/123456789/11574
dc.identifier.urihttp://dx.doi.org/10.34657/10607
dc.language.isoeng
dc.publisherCambridge : RSC
dc.relation.doihttps://doi.org/10.1039/c6gc03527b
dc.relation.essn1463-9270
dc.relation.ispartofseriesGreen chemistry : GC 19 (2017), Nr. 10
dc.relation.issn1463-9262
dc.rights.licenseCC BY-NC 3.0 Unported
dc.rights.urihttps://creativecommons.org/licenses/by-nc/3.0
dc.subjectcopper-based photosensitizerseng
dc.subjectcarbon-dioxideeng
dc.subjectphotochemical reductioneng
dc.subjecthydrogen-productioneng
dc.subjecthighly efficienteng
dc.subjectwater reductioneng
dc.subjectcatalysteng
dc.subjectironeng
dc.subjectphotophysicseng
dc.subjectcomplexeseng
dc.subject.ddc540
dc.titleEarth-abundant photocatalytic systems for the visible-light-driven reduction of CO2 to COeng
dc.typearticle
dc.typeText
dcterms.bibliographicCitation.journalTitleGreen chemistry : GC
tib.accessRightsopenAccess
wgl.contributorLIKAT
wgl.subjectChemieger
wgl.typeZeitschriftenartikelger
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