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- ItemCADEX and beyond: Installation of a new PollyXT site in Dushanbe(Les Ulis : EDP Sciences, 2019) Engelmann, Ronny; Hofer, Julian; Makhmudov, Abduvosit N.; Baars, Holger; Hanbuch, Karsten; Ansmann, Albert; Abdullaev, Sabur F.; Macke, Andreas; Althausen, DietrichDuring the 18-month Central Asian Dust Experiment we conducted continuous lidar measurements at the Physical Technical Institute of the Academy of Sciences of Tajikistan in Dushanbe between 2015 and 2016. Mineral dust plumes from various source regions have been observed and characterized in terms of their occurrence, and their optical and microphysical properties with the Raman lidar PollyXT. Currently a new container-based lidar system is constructed which will be installed for continuous long-term measurements in Dushanbe. © 2019 The Authors, published by EDP Sciences.
- ItemVariations of the aerosol chemical composition during Asian dust storm at Dushanbe, Tajikistan(Les Ulis : EDP Sciences, 2019) Fomba, Khanneh Wadinga; Müller, Konrad; Hofer, Julian; Makhmudov, Abduvosit N.; Althausen, Dietrich; Nazarov, Bahron I.; Abdullaev, Sabur F.; Herrmann, HartmutAerosol chemical composition was characterized during the Central Asian Dust Experiment (CADEX) at Dushanbe (Tajikistan). Aerosol samples were collected during a period of 2 months from March to May 2015 using a high volume DIGITEL DHA-80 sampler on quartz fiber filters. The filters were analyzed for their ionic, trace metals as well as organic and elemental carbon (OC/EC) content. The aerosol mass showed strong variation with mass concentration ranging from 18 μg/m3 to 110 μg/m3. The mineral dust concentrations varied between 0.9 μg/m3 and 88 μg/m3. Days of high aerosol mass loadings were dominated by mineral dust, which made up to about 80% of the aerosol mass while organic matter and inorganic ions made up about 70% of the aerosol mass during days of low aerosol mass loadings. The mineral dust composition showed different trace metal signatures in comparison to Saharan dust with higher Ca content and Ca/Fe ratios twice as high as that observed in Saharan dust. Strong influence of anthropogenic activities was observed in the trace metal concentrations with Zn and Pb concentrations ranging from 7 to 197 ng/m3 and 2 to 20 ng/m3, respectively. Mineral dust and anthropogenic activities relating to traffic, combustion as well as metallurgical industrial emissions are identified as the sources of the aerosol during this period. © 2019 The Authors, published by EDP Sciences.
- ItemAerosol layer heights above Tajikistan during the CADEX campaign(Les Ulis : EDP Sciences, 2019) Hofer, Julian; Althausen, Dietrich; Abdullaev, Sabur F.; Nazarov, Bakhron I.; Makhmudov, Abduvosit N.; Baars, Holger; Engelmann, Ronny; Ansmann, AlbertMineral dust influences climate and weather by direct and indirect effects. Surrounded by dust sources, Central Asian countries are affected by atmospheric mineral dust on a regular basis. Climate change effects like glacier retreat and desertification are prevalent in Central Asia as well. Therefore, the role of dust in the climate system in Central Asia needs to be clarified and quantified. During the Central Asian Dust EXperiment (CADEX) first lidar observations in Tajikistan were conducted. Long-term vertically resolved aerosol measurements were performed with the multiwavelength polarization Raman lidar PollyXT from March 2015 to August 2016 in Dushanbe, Tajikistan. In this contribution, a climatology of the aerosol layer heights is presented, which was retrieved from the 18-month lidar measurements. Automatic detection based on backscatter coefficient thresholds were used to retrieve the aerosol layer heights and yield similar layer heights as manual layer height determination. The significant aerosol layer height has a maximum in summer and a minimum in winter. The highest layers occurred in spring, but in summer uppermost layer heights above 6 km AGL are frequent, too. © 2019 The Authors, published by EDP Sciences.
- ItemEstimation of dust related ice nucleating particles in the atmosphere: Comparison of profiling and in-situ measurements(Les Ulis : EDP Sciences, 2019) Haarig, Moritz; Ansmann, Albert; Walser, Adrian; Baars, Holger; Urbanneck, Claudia; Weinzierl, Bernadett; Schöberl, Manuel; Dollner, Maximilian; Mamouri, Rodanthi; Althausen, DietrichVertical profiles of number concentrations of dust particles relevant for ice nucleation in clouds are derived from lidar measurements. The results are compared to coincidental airborne in-situ measurements of particle number and surface area concentrations in the dust layer. The observations were performed in long-range transported Saharan dust at Barbados and Asian dust at Cyprus. The Asian dust data analysis is ongoing. A comparison of Asian and Saharan dust will be given at the conference. Concentrations of ice nucleating particles in the order of 10 to 1000 per cm-3 in the dust layer are derived for a temperature of-25°C at Barbados. The method can be used to continuously monitor the concentration of ice nucleating dust particles vertically resolved from lidar measurements. © 2019 The Authors, published by EDP Sciences.
- ItemDust impacts on radiative effects of black carbon aerosol in Central Asia(Les Ulis : EDP Sciences, 2019) Tegen, Ina; Heinold, BerndThe radiative effect of mineral dust and black carbon aerosol are investigated with aerosolclimate model simulations with fixed sea surface temperatures as boundary condition. The semi-direct effects of the absorbing aerosol are assessed as the residual between the total direct radiative effect and the instantaneous direct radiative effect of the aerosol species. For Central Asia the presence of mineral dust aerosol below a black carbon aerosol layer enhances the positive radiative effect of the black carbon aerosol. © 2019 The Authors, published by EDP Sciences.
- ItemAn Overview on the Role of Relative Humidity in Airborne Transmission of SARS-CoV-2 in Indoor Environments(Taoyuan City : Taiwan Association for Aerosol Research (TAAR), 2020) Ahlawat, Ajit; Wiedensohler, Alfred; Mishra, Sumit KumarCOVID-19 disease is caused by severe acute respiratory syndrome coronavirus 2 (SARS-CoV-2), which originated in Wuhan, China and spread with an astonishing rate across the world. The transmission routes of SARS-CoV-2 are still debated, but recent evidence strongly suggests that COVID-19 could be transmitted via air in poorly ventilated places. Some studies also suggest the higher surface stability of SARS-CoV-2 as compared to SARS-CoV-1. It is also possible that small viral particles may enter into indoor environments from the various emission sources aided by environmental factors such as relative humidity, wind speed, temperature, thus representing a type of an aerosol transmission. Here, we explore the role of relative humidity in airborne transmission of SARS-CoV-2 virus in indoor environments based on recent studies around the world. Humidity affects both the evaporation kinematics and particle growth. In dry indoor places i.e., less humidity (< 40% RH), the chances of airborne transmission of SARS-CoV-2 are higher than that of humid places (i.e., > 90% RH). Based on earlier studies, a relative humidity of 40–60% was found to be optimal for human health in indoor places. Thus, it is extremely important to set a minimum relative humidity standard for indoor environments such as hospitals, offices and public transports for minimization of airborne spread of SARS-CoV-2. © The Author(s).
- ItemNo Evidence for a Significant Impact of Heterogeneous Chemistry on Radical Concentrations in the North China Plain in Summer 2014(Columbus, Ohio : American Chemical Society, 2020) Tan, Zhaofeng; Hofzumahaus, Andreas; Lu, Keding; Brown, Steven S.; Holland, Frank; Huey, Lewis Gregory; Kiendler-Scharr, Astrid; Li, Xin; Liu, Xiaoxi; Ma, Nan; Min, Kyung-Eun; Rohrer, Franz; Shao, Min; Wahner, Andreas; Wang, Yuhang; Wiedensohler, Alfred; Wu, Yusheng; Wu, Zhijun; Zeng, Limin; Zhang, Yuanhang; Fuchs, HendrikThe oxidation of nitric oxide to nitrogen dioxide by hydroperoxy (HO2) and organic peroxy radicals (RO2) is responsible for the chemical net ozone production in the troposphere and for the regeneration of hydroxyl radicals, the most important oxidant in the atmosphere. In Summer 2014, a field campaign was conducted in the North China Plain, where increasingly severe ozone pollution has been experienced in the last years. Chemical conditions in the campaign were representative for this area. Radical and trace gas concentrations were measured, allowing for calculating the turnover rates of gas-phase radical reactions. Therefore, the importance of heterogeneous HO2 uptake on aerosol could be experimentally determined. HO2 uptake could have suppressed ozone formation at that time because of the competition with gas-phase reactions that produce ozone. The successful reduction of the aerosol load in the North China Plain in the last years could have led to a significant decrease of HO2 loss on particles, so that ozone-forming reactions could have gained importance in the last years. However, the analysis of the measured radical budget in this campaign shows that HO2 aerosol uptake did not impact radical chemistry for chemical conditions in 2014. Therefore, reduced HO2 uptake on aerosol since then is likely not the reason for the increasing number of ozone pollution events in the North China Plain, contradicting conclusions made from model calculations reported in the literature. © 2020 American Chemical Society.
- ItemVertical profiles of dust and other aerosol types above a coastal site(Les Ulis : EDP Sciences, 2019) Althausen, Dietrich; Mewes, Silke; Heese, Birgit; Hofer, Julian; Schechner, Yoav; Aides, Amit; Holodovsky, VadimMonthly mean vertical profiles of aerosol type occurrences are determined from multiwavelength Raman and polarization lidar measurements above Haifa, Israel, in 2017. This contribution presents the applied methods and threshold values. The results are discussed for one example, May 2017. This month shows more often large, non-spherical particles in lofted layers than within the planetary boundary layer. Small particles are observed at higher altitudes only when they are observed in lower altitudes, too. © 2019 The Authors, published by EDP Sciences.
- ItemThe regime of Aerosol Optical Depth and Ångström exponent over Central and South Asia(Les Ulis : EDP Sciences, 2019) Floutsi, Athina Avgousta; Korras Carraca, Marios Bruno; Matsoukas, Christos; Hatzianastassiou, Nikos; Biskos, GeorgeCentral and South Asia are regions of particular interest for studying atmospheric aerosols, being among the largest sources of desert dust aerosols globally. In this study we use the newest collection (C061) of MODIS-Aqua aerosol optical depth (AOD) at 550 nm and Ångström exponent (a) at 412/470 nm over the 15-year period between 2002 and 2017, providing the longest analyzed dataset for this region. According to our results, during spring and summer, high aerosol load (AOD up to 1.2) consisting of coarse desert dust particles, as indicated by a values as low as 0.15, is observed over the Taklamakan, Thar and Registan deserts and the region between the Aral and Caspian seas. The dust load is much lower during winter and autumn (lower AOD and higher a values compared to the other seasons). The interannual variation of AOD and a suggests that the dust load exhibits large decreasing trends (AOD slopes down to-0.22, a slopes up to 0.47 decade-1) over the Thar desert and large increasing trends between the Aral and Caspian seas (AOD and a slopes up to 0.23 decade-1 and down to-0.61 decade-1, respectively.) The AOD data are evaluated against AERONET surface-based measurements. Generally, MODIS and AERONET data are in good agreement with a correlation coefficient (R) equal to 0.835. © 2019 The Authors, published by EDP Sciences.
- ItemModelling mineral dust in the Central Asian region(Les Ulis : EDP Sciences, 2019) Heinold, Bernd; Tegen, InaIn Central Asia, climate and air quality are largely affected by local and long-travelled mineral dust. For the last century, the area has experienced severe land-use changes and water exploitation producing new dust sources. Today global warming causes rapid shrinking of mountain glaciers with yet unknow consequences for dust and its climate effects. Despite the importance for a growing population, only little is known about sources, transport pathways and properties of Central Asian dust. A transport study with a global aerosol-climate model is undertaken to investigate the life cycle of mineral dust in Central Asia for the period of a remote-sensing campaign in Tajikistan in 2015-2016. An initial evaluation with sun photometer measurements shows reasonable agreement for the average amount of dust, but a significant weakness of the model in reproducing the seasonality of local dust with maximum activity in summer. Source apportionment reveals a major contribution from Arabia throughout the year in accordance with observations. In the model, local sources mainly contribute in spring and autumn while summer-time dust production is underestimated. The results underline the importance of considering long-range transport and, locally, a detailed representation of atmospheric dynamics and surface characteristics for modelling dust in Central Asia. © 2019 The Authors, published by EDP Sciences.