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- ItemElectronic structure and aspects of unconventional superconductivity in NaxCoO2.yH2O(São Carlos : Universidade Federal de São Carlos, 2003) Rosner, H.; Drechsler, S.-L.; Fuchs, G.; Handstein, A.; Wälte, A.; Müller, K.-H.We examine the electronic structure of NaxCoO2.yH2O within the local density approximation. The parametrization of the band which forms the largest hole-Fermi surface centered at G shows significant deviations from what is frequently assumed in recent sophisticated theoretical studies. In particular, the commonly used nearest neighbor approaches in the framework of single band pictures are found to be unrealistic. The special role of H2O in screening the disorder in the charge reservoir is briefly discussed and compared with the case of Y1–xCaxCu3O6+d.
- ItemOrbital and spin effects for the upper critical field in As-deficient disordered Fe pnictide superconductors(Milton Park : Taylor & Francis, 2009) Fuchs, G.; Drechsler, S.-L.; Kozlova, N.; Bartkowiak, M.; Hamann-Borrero, J.E.; Behr, G.; Nenkov, K.; Klauss, H.-H.; Maeter, H.; Amato, A.; Luetkens, H.; Kwadrin, A.; Khasanov, R.; Freudenberger, J.; Köhler, A.; Knupfer, M.; Arushanov, E.; Rosner, H.; Büchner, B.; Schultz, L.We report upper critical field Bc2(T) data for LaO0.9F0.1FeAs1- δ in a wide temperature and field range up to 60 T. The large slope of Bc2≈- 5.4 to -6.6 T K-1 near an improved Tc≈28.5 K of the in-plane Bc2(T) contrasts with a flattening starting near 23 K above 30 T we regard as the onset of Pauli-limited behaviour (PLB) with Bc2(0)≈63–68 T. We interpret a similar hitherto unexplained flattening of the Bc2(T) curves reported for at least three other disordered closely related systems, Co-doped BaFe2As2, (Ba,K) Fe2As2 and NdO0.7F0.3FeAs (all single crystals), for applied fields H∥(a,b), also as a manifestation of PLB. Their Maki parameters have been estimated by analysing their Bc2(T) data within the Werthamer–Helfand–Hohenberg approach. The pronounced PLB of (Ba, K)Fe2As2 single crystals obtained from an Sn flux is attributed also to a significant As deficiency detected by wavelength dispersive x-ray spectroscopy as reported by Ni et al (2008 Phys. Rev. B 78 014507). Consequences of our results are discussed in terms of disorder effects within conventional superconductivity (CSC) and unconventional superconductivity (USC). USC scenarios with nodes on individual Fermi surface sheets (FSS), e.g. p- and d-wave SC, can be discarded for our samples. The increase of dBc2/dT|Tc by sizeable disorder provides evidence for an important intraband (intra-FSS) contribution to the orbital upper critical field. We suggest that it can be ascribed either to an impurity-driven transition from s± USC to CSC of an extended s++-wave state or to a stabilized s±-state provided As-vacancies cause predominantly strong intraband scattering in the unitary limit. We compare our results with Bc2 data from the literature, which often show no PLB for fields below 60–70 T probed so far. A novel disorder-related scenario of a complex interplay of SC with two different competing magnetic instabilities is suggested.
- ItemCoexistence of superconductivity and ferromagnetism in Sr0.5Ce0.5FBiS2-xSex (x = 0.5 and 1.0), a non-U material with Tc < TFM(London : Nature Publishing Group, 2016) Thakur, Gohil S.; Fuchs, G.; Nenkov, K.; Haque, Zeba; Gupta, L.C.; Ganguli, A.K.We have carried out detailed magnetic and transport studies of the new Sr0.5Ce0.5FBiS2-xSex (0.0 ≤ x ≤ 1.0) superconductors derived by doping Se in Sr0.5Ce0.5FBiS2. Se–doping produces several effects: it suppresses semiconducting–like behavior observed in the undoped Sr0.5Ce0.5FBiS2, the ferromagnetic ordering temperature, TFM, decreases considerably from 7.5 K (in Sr0.5Ce0.5FBiS2) to 3.5 K and the superconducting transition temperature, Tc, gets enhanced slightly to 2.9–3.3 K. Thus in these Se–doped materials, TFM is marginally higher than Tc. Magnetization studies provide evidence of bulk superconductivity in Sr0.5Ce0.5FBiS2-xSex at x ≥ 0.5 in contrast to the undoped Sr0.5Ce0.5FBiS2 (x = 0) where magnetization measurements indicate a small superconducting volume fraction. Quite remarkably, as compared with the effective paramagnetic Ce–moment (~2.2 μB), the ferromagnetically ordered Ce–moment in the superconducting state is rather small (~0.1 μB) suggesting itinerant ferromagnetism. To the best of our knowledge, Sr0.5Ce0.5FBiS2-x Sex (x = 0.5 and 1.0) are distinctive Ce–based bulk superconducting itinerant ferromagnetic materials with Tc < TFM. Furthermore, a novel feature of these materials is that they exhibit a dual and quite unusual hysteresis loop corresponding to both the ferromagnetism and the coexisting bulk superconductivity.