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Thin film models for an active gel

2017, Kitavtsev, Georgy, Münch, Andreas, Wagner, Barbara

In this study we present a free-boundary problem for an active liquid crystal based on the Beris-Edwards theory that uses a tensorial order parameter and includes active contributions to the stress tensor to analyse the rich defect structure observed in applications such as the Adenosinetriphosphate (ATP) driven motion of a thin film of an actin filament network. The small aspect ratio of the film geometry allows for an asymptotic approximation of the free-boundary problem in the limit of weak elasticity of the network and strong active terms. The new thin film model captures the defect dynamics in the bulk as well as wall defects and thus presents a significant extension of previous models based on the Leslie-Erickson-Parodi theory. Analytic expressions are derived that reveal the interplay of anchoring conditions, film thickness and active terms and their control of transitions of flow structure.

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Gradient flow perspective of thin-film bilayer flows

2013, Huth, Robert, Jachalski, Sebastian, Kitavtsev, Georgy, Peschka, Dirk

We study gradient flow formulations of thin-film bilayer flows with triple-junctions between liquid/liquid/air. First we highlight the gradient structure in the Stokes free-boundary flow and identify its solutions with the well-known PDE with boundary conditions. Next we propose a similar gradient formulation for the corresponding thin-film model and formally identify solutions with those of the corresponding free-boundary problem. A robust numerical algorithm for the thin-film gradient flow structure is then provided. Using this algorithm we compare the sharp triple-junction model with precursor models. For their stationary solutions a rigorous connection is established using [Gamma]-convergence. For time-dependentsolutions the comparison of numerical solutions shows a good agreement for small and moderate times. Finally we study spreading in the zero-contact angle case, where we compare numerical solutions with asymptotically exact source-type solutions.

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Coarsening dynamics of slipping droplets

2008, Kitavtsev, Georgy, Wagner, Barbara

This paper studies the late phase dewetting process of nanoscopic thin polymer films on hydrophobized substrates using some recently derived lubrication models that take account of large slippage at the polymer-substrate interface. The late phase of this process is characterized by the slow-time coarsening dynamics of arrays of droplets that remain after rupture and the initial dewetting phases. For this situation a reduced system of ordinary differential equations is derived from the lubrication model for large slippage using asymptotic analysis. This extends known results for the no-slip case. On the basis of the reduced model, the role of the slippage as a control parameter for droplet migration is analysed and several new qualitative effects for the coarsening process are identified.

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Center manifold reduction approach for the lubrication equation

2010, Kitavtsev, Georgy, Recke, Lutz, Wagner, Barbara

The goal of this study is the reduction of the lubrication equation, modelling thin film dynamics, onto an approximate invariant manifold. The reduction is derived for the physical situation of the late phase evolution of a dewetting thin liquid film, where arrays of droplets connected by an ultrathin film of thickness eps undergo a slow-time coarsening dynamics. With this situation in mind, we construct an asymptotic approximation of the corresponding invariant manifold, that is parametrized by a family of droplet pressures and positions, in the limit when $epsto 0$. The approach is inspired by the paper by Mielke and Zelik [Mem. Amer. Math. Soc., Vol. 198, 2009], where the center manifold reduction was carried out for a class of semilinear systems. In this study this approach is considered for quasilinear degenerate parabolic PDE's such as lubrication equations. While it has previously been shown by Glasner and Witelski [Phys. Rev. E, Vol. 67, 2003], that the system of ODEs governing the coarsening dynamics, can be obtained via formal asymptotic methods, the center manifold reduction approach presented here, pursues the rigorous justification of this asymptotic limit.

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Stationary solutions for two-layer lubrication equations

2011, Jachalski, Sebastian, Huth, Robert, Kitavtsev, Georgy, Peschka, Dirk, Wagner, Barbara

We investigate stationary solutions of flows of thin liquid bilayers in an energetic formulation which is motivated by the gradient flow structure of its lubrication approximation. The corresponding energy favors the liquid substrate to be only partially covered by the upper liquid. This is expressed by a negative spreading coefficient which arises from an intermolecular potential combining attractive and repulsive forces and leads to an ultra-thin layer of thickness e. For the corresponding lubrication models existence of stationary solutions is proven. In the limit e to 0 matched asymptotic analysis is applied to derive sharp-interface models and the corresponding contact angles, i.e. the Neumann triangle. In addition we use G-convergence and derive the equivalent sharp-interface models rigorously in this limit. For the resulting model existence and uniqueness of energetic minimizers are proven. The minimizers agree with solutions obtained by matched asymptotics.

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Weak solutions to lubrication systems describing the evolution of bilayer thin films

2012, Jachalski, Sebastian, Kitavtsev, Georgy, Taranets, Roman

The existence of global nonnegative weak solutions is proved for coupled one-dimensional lubrication systems that describe the evolution of nanoscopic bilayer thin polymer films that take account of Navier-slip or no-slip conditions at both liquid-liquid and liquidsolid interfaces. In addition, in the presence of attractive van der Waals and repulsive Born intermolecular interactions existence of positive smooth solutions is shown.

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Asymptotics for the spectrum of a thin film equation in a singular limit

2010, Kitavtsev, Georgy, Recke, Lutz, Wagner, Barbara

In this paper the linear stability properties of the steady states of a no-slip lubrication equation are studied. The steady states are configurations of droplets and arise during the late-phase dewetting process under the influence of both destabilizing van der Waals and stabilizing Born intermolecular forces, which in turn give rise to the minimum thickness eps of the remaining film connecting the droplets. The goal of this paper is to give an asymptotic description of the eigenvalues and eigenfunctions of the problem, linearized about the one-droplet solutions, as epsto 0. For this purpose, corresponding asymptotic eigenvalue problems with piecewise constant coefficients are constructed, such that their eigenvalue asymptotics can be determined analytically. A comparison with numerically computed eigenvalues and eigenfunctions shows good agreement with the asymptotic results and the existence of a spectrum gap to a single exponentially small eigenvalue for sufficiently small eps.