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    SESAM mode-locked Tm:Y2O3 ceramic laser
    (Washington, DC : Soc., 2022) Zhang, Ning; Liu, Shande; Wang, Zhanxin; Liu, Jian; Xu, Xiaodong; Xu, Jun; Wang, Jun; Liu, Peng; Ma, Jie; Shen, Deyuan; Tang, Dingyuan; Lin, Hui; Zhang, Jian; Chen, Weidong; Zhao, Yongguang; Griebner, Uwe; Petrov, Valentin
    We demonstrate a widely tunable and passively mode-locked Tm:Y2O3 ceramic laser in-band pumped by a 1627-nm Raman fiber laser. A tuning range of 318 nm, from 1833 to 2151 nm, is obtained in the continuous-wave regime. The SESAM mode-locked laser produces Fourier-transform-limited pulses as short as 75 fs at ∼ 2.06 µm with an average output power of 0.26 W at 86.3 MHz. For longer pulse durations of 178 fs, an average power of 0.59 W is achieved with a laser efficiency of 29%. This is, to the best of our knowledge, the first mode-locked Tm:Y2O3 laser in the femtosecond regime. The spectroscopic properties and laser performance confirm that Tm:Y2O3 transparent ceramics are a promising gain material for ultrafast lasers at 2 µm.
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    Spectroscopy of solid-solution transparent sesquioxide laser ceramic Tm:LuYO3
    (Washington, DC : OSA, 2022) Eremeev, Kirill; Loiko, Pavel; Braud, Alain; Camy, Patrice; Zhang, Jian; Xu, Xiaodong; Zhao, Yongguang; Liu, Peng; Balabanov, Stanislav; Dunina, Elena; Kornienko, Alexey; Fomicheva, Liudmila; Mateos, Xavier; Griebner, Uwe; Petrov, Valentin; Wang, Li; Chen, Weidong
    We report on a detailed spectroscopic study of a Tm3+-doped transparent sesquioxide ceramic based on a solid-solution (lutetia – yttria, LuYO3) composition. The ceramic was fabricated using commercial oxide powders by hot isostatic pressing at 1600°C for 3 h at 190 MPa argon pressure. The most intense Raman peak in Tm:LuYO3 at 385.4 cm−1 takes an intermediate position between those for the parent compounds and is notably broadened (linewidth: 12.8 cm−1). The transition intensities of Tm3+ ions were calculated using the Judd-Ofelt theory; the intensity parameters are W2 = 2.537, W4 = 1.156 and W6 = 0.939 [1020 cm2]. For the 3F4 → 3H6 transition, the stimulated-emission cross-section amounts to 0.27 × 10−20 cm2 at 2059nm and the reabsorption-free luminescence lifetime is 3.47 ms (the 3F4 radiative lifetime is 3.85 ± 0.1 ms). The Tm3+ ions in the ceramic exhibit long-wave multiphonon-assisted emission extending up to at least 2.35 µm; a phonon sideband at 2.23 µm is observed and explained by coupling between electronic transitions and the dominant Raman mode of the sesquioxides. Low temperature (12 K) spectroscopy reveals a significant inhomogeneous spectral broadening confirming formation of a substitutional solid-solution. The mixed ceramic is promising for ultrashort pulse generation at >2 µm.