2012, Zherebtsov, S., Süßmann, F., Peltz, C., Plenge, J., Betsch, K.J., Znakovskaya, I., Alnaser, A.S., Johnson, N.G., Kübel, M., Horn, A., Mondes, V., Graf, C., Trushin, S.A., Azzeer, A., Vrakking, M.J.J., Paulus, G.G., Krausz, F., Rühl, E., Fennel, T., Kling, M.F.

Waveform-controlled light fields offer the possibility of manipulating ultrafast electronic processes on sub-cycle timescales. The optical lightwave control of the collective electron motion in nanostructured materials is key to the design of electronic devices operating at up to petahertz frequencies. We have studied the directional control of the electron emission from 95 nm diameter SiO 2 nanoparticles in few-cycle laser fields with a well-defined waveform. Projections of the three-dimensional (3D) electron momentum distributions were obtained via single-shot velocity-map imaging (VMI), where phase tagging allowed retrieving the laser waveform for each laser shot. The application of this technique allowed us to efficiently suppress background contributions in the data and to obtain very accurate information on the amplitude and phase of the waveform-dependent electron emission. The experimental data that are obtained for 4 fs pulses centered at 720 nm at different intensities in the range (1-4)×10 13Wcm -2 are compared to quasi-classical mean-field Monte-Carlo simulations. The model calculations identify electron backscattering from the nanoparticle surface in highly dynamical localized fields as the main process responsible for the energetic electron emission from the nanoparticles. The local field sensitivity of the electron emission observed in our studies can serve as a foundation for future research on propagation effects for larger particles and field-induced material changes at higher intensities.

2012, Kelkensberg, F., Koenderink, A.F., Vrakking, M.J.J.

A theoretical study of the application of attosecond streaking spectroscopy to time-resolved studies of the plasmonic fields surrounding isolated, resonantly excited spherical nanoparticles is presented. A classification of the different regimes in attosecond streaking is proposed and identified in our results that are derived from Mie calculations of plasmon fields, coupled to classical electron trajectory simulations. It is shown that in an attosecond streaking experiment, the electrons are almost exclusively sensitive to the component of the field parallel to the direction in which they are detected. This allows one to probe the different components of the field individually by resolving the angle of emission of the electrons. Finally, simulations based on fields calculated by finite-difference time-domain (FDTD) are compared with the results obtained using Mie fields. The two are found to be in good agreement with each other, supporting the notion that FDTD methods can be used to reliably investigate non-spherical structures.

2014, Bowlan, P., Martinez-Moreno, E., Reimann, K., Woerner, M., Elsaesser, T.

The nonlinear interaction between intense terahertz (THz) pulses and epitaxial multilayer graphene is studied by field-resolved THz pump-probe spectroscopy. THz excitation results in a transient induced absorption with decay times of a few picoseconds, much faster than carrier recombination in single graphene layers. The decay times increase with decreasing temperature and increasing amplitude of the excitation. This behaviour originates from the predominant coupling of electrons to the electromagnetic field via the very strong interband dipole moment while scattering processes with phonons and impurities play a minor role. The nonlinear response at field amplitudes above 1 kV cm-1 is in the carrier-wave Rabi flopping regime with a pronounced coupling of the graphene layers via the radiation field. Theoretical calculations account for the experimental results.

2013, Martens, C., Longo, P., Busch, K.

We discuss the transport properties of a single photon in a one-dimensional waveguide with an embedded three-level atom and utilize both stationary plane-wave solutions and time-dependent transport calculations to investigate the interaction of a photon with driven and undriven V- and Λ-systems. Specifically, for the case of an undriven V-system, we analyze the phenomenon of long-time occupation of the upper atomic levels in conjunction with almost dark states. For the undriven Λ-system, we find non-stationary dark states and we explain how the photon's transmittance can be controlled by an initial phase difference between the energetically lower-lying atomic states. With regard to the driven three-level systems, we discuss electromagnetically induced transparency in terms of the pulse propagation of a single photon through a Λ-type atom. In addition, we demonstrate how a driven V-type atom can be utilized to control the momentum distribution of the scattered photon.

2011, Gademann, G., Kelkensberg, F., Siu, W.K., Johnsson, P., Gaarde, M.B., Schafer, K.J., Vrakking, M.J.J.

We show that high harmonic generation driven by an intense nearinfrared (IR) laser can be temporally controlled when an attosecond pulse train (APT) is used to ionize the generation medium, thereby replacing tunnel ionization as the first step in the well-known three-step model. New harmonics are formed when the ionization occurs at a well-defined time within the optical cycle of the IR field. The use of APT-created electron wave packets affords new avenues for the study and application of harmonic generation. In the present experiment, this makes it possible to study harmonic generation at IR intensities where tunnel ionization does not give a measurable signal.

2012, Korneev, Ph.A., Popruzhenko, S.V., Goreslavski, S.P., Becker, W., Paulus, G.G., Fetić, B., Milošević, D.B.

Laser-induced electron detachment or ionization of atoms and negative ions is considered. In the context of the saddle-point evaluation of the strong-field approximation (SFA), the velocity maps of the direct electrons (those that do not undergo rescattering) exhibit a characteristic structure due to the constructive and destructive interference of electrons liberated from their parent atoms/ions within certain windows of time. This structure is defined by the above-threshold ionization rings at fixed electron energy and by two sets of curves in momentum space on which destructive interference occurs. The spectra obtained with the SFA are compared with those obtained by numerical solution of the time-dependent Schrödinger equation. For detachment, the agreement is excellent. For ionization, the effect of the Coulomb field is most pronounced for electrons emitted in a direction close to laser polarization, while for nearperpendicular emission the qualitative appearance of the spectrum is unaffected.

2014, Leitenstorfer, A., Nelson, K.A., Reimann, K., Tanaka, K.

Resulting from the availability of improved sources, research in the terahertz (THz) spectral range has increased dramatically over the last decade, leading essentially to the disappearance of the so-called 'THz gap'. While most work to date has been carried out with THz radiation of low field amplitude, a growing number of experiments are using THz radiation with large electric and magnetic fields that induce nonlinearities in the system under study. This 'focus on' collection contains a number of articles, both experimental and theoretical, in the new subfield of THz nonlinear optics and spectroscopy on various systems, among them molecular gases, superconductors, semiconductors, antiferromagnets and graphene.

2012, Passig, J., Irsig, R., Truong, N.X., Fennel, T., Tiggesbäumker, J., Meiwes-Broer, K.H.

The nanoplasmonic field enhancement effects in the energetic electron emission from few-nm-sized silver clusters exposed to intense femtosecond dual pulses are investigated by high-resolution double differential electron spectroscopy. For moderate laser intensities of 10 14Wcm -2, the delaydependent and angular-resolved electron spectra show laser-aligned emission of electrons up to keV kinetic energies, exceeding the ponderomotive potential by two orders of magnitude. The importance of the nanoplasmonic field enhancement due to resonant Mie-plasmon excitation observed for optimal pulse delays is investigated by a direct comparison with molecular dynamics results. The excellent agreement of the key signatures in the delay-dependent and angular-resolved spectra with simulation results allows for a quantitative analysis of the laser and plasmonic contributions to the acceleration process. The extracted field enhancement at resonance verifies the dominance of surfaceplasmon-assisted re-scattering.

2013, Woerner, M., Kuehn, W., Bowlan, P., Reimann, K., Elsaesser, T.

Recent experimental progress has allowed for the implementation of nonlinear two-dimensional (2D) terahertz (THz) spectroscopy in the ultrafast time domain. We discuss the principles of this technique based on multiple phase-locked electric field transients interacting in a collinear geometry with a solid and the phase-resolved detection of the THz fields after interaction with the sample. To illustrate the potential of this new method, 2D correlation spectra of coupled intersubband-longitudinal optical phonon excitations in a double quantum well system and a study of ultrafast carrier dynamics in graphene are presented.

2013, Richter, M., Patchkovskii, S., Morales, F., Smirnova, O., Ivanov, M.

We discuss the connection between strong-field ionization, saturation of the Kerr response and the formation of the Kramers-Henneberger (KH) atom and long-living excitations in intense infrared (IR) external fields. We present a generalized model for the intensity-dependent response of atoms in strong IR laser fields, describing deviations in the nonlinear response at the frequency of the driving field from the standard model. We show that shaping the driving laser pulse allows one to reveal signatures of the excited KH states in the Kerr response of an individual atom.