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End date: 2020 × Subject: phase transition ×

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Now showing 1 - 10 of 24
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    Tuning the interplay between nematicity and spin fluctuations in Na1-x Li x FeAs superconductors
    (London : Nature Publishing Group, 2018) Baek, S.-H.; Bhoi, D.; Nam, W.; Lee, B.; Efremov, D.V.; Büchner, B.; Kim, K.H.
    Strong interplay of spin and charge/orbital degrees of freedom is the fundamental characteristic of the iron-based superconductors (FeSCs), which leads to the emergence of a nematic state as a rule in the vicinity of the antiferromagnetic state. Despite intense debate for many years, however, whether nematicity is driven by spin or orbital fluctuations remains unsettled. Here, by use of transport, magnetization, and 75As nuclear magnetic resonance (NMR) measurements, we show a striking transformation of the relationship between nematicity and spin fluctuations (SFs) in Na1-x Li x FeAs; For x ≤ 0.02, the nematic transition promotes SFs. In contrast, for x ≥ 0.03, the system undergoes a non-magnetic phase transition at a temperature T 0 into a distinct nematic state that suppresses SFs. Such a drastic change of the spin fluctuation spectrum associated with nematicity by small doping is highly unusual, and provides insights into the origin and nature of nematicity in FeSCs.
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    Two types of magnetic shape-memory effects from twinned microstructure and magneto-structural coupling in Fe1 +yTe
    (Washington : National Academy of Sciences, 2019) Rößler, S.; Koz, C.; Wang, Z.; Skourski, Y.; Doerr, M.; Kasinathan, D.; Rosner, H.; Schmidt, M.; Schwarz, U.; Rößler, U.K.; Wirth, S.
    A detailed experimental investigation of Fe1+yTe (y = 0.11, 0.12) using pulsed magnetic fields up to 60 T confirms remarkable magnetic shape-memory (MSM) effects. These effects result from magnetoelastic transformation processes in the low-temperature antiferromagnetic state of these materials. The observation of modulated and finely twinned microstructure at the nanoscale through scanning tunneling microscopy establishes a behavior similar to that of thermoelastic martensite. We identified the observed, elegant hierarchical twinning pattern of monoclinic crystallographic domains as an ideal realization of crossing twin bands. The antiferromagnetism of the monoclinic ground state allows for a magnetic-field–induced reorientation of these twin variants by the motion of one type of twin boundaries. At sufficiently high magnetic fields, we observed a second isothermal transformation process with large hysteresis for different directions of applied field. This gives rise to a second MSM effect caused by a phase transition back to the field-polarized tetragonal lattice state.
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    Collapse of layer dimerization in the photo-induced hidden state of 1T-TaS2
    ([London] : Nature Publishing Group UK, 2020) Stahl, Quirin; Kusch, Maximilian; Heinsch, Florian; Garbarino, Gaston; Kretzschmar, Norman; Hanff, Kerstin; Rossnagel, Kai; Geck, Jochen; Ritschel, Tobias
    Photo-induced switching between collective quantum states of matter is a fascinating rising field with exciting opportunities for novel technologies. Presently, very intensively studied examples in this regard are nanometer-thick single crystals of the layered material 1T-TaS2, where picosecond laser pulses can trigger a fully reversible insulator-to-metal transition (IMT). This IMT is believed to be connected to the switching between metastable collective quantum states, but the microscopic nature of this so-called hidden quantum state remained largely elusive up to now. Here, we characterize the hidden quantum state of 1T-TaS2 by means of state-of-the-art x-ray diffraction and show that the laser-driven IMT involves a marked rearrangement of the charge and orbital order in the direction perpendicular to the TaS2-layers. More specifically, we identify the collapse of interlayer molecular orbital dimers as a key mechanism for this non-thermal collective transition between two truly long-range ordered electronic crystals.
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    Hybrid soliton dynamics in liquid-core fibres
    (Berlin : Nature Pulishing, 2017) Chemnitz, Mario; Gebhardt, Martin; Gaida, Christian; Stutzki, Fabian; Kobelke, Jens; Limpert, Jens; Tünnermann, Andreas; Schmidt, Markus A.
    The discovery of optical solitons being understood as temporally and spectrally stationary optical states has enabled numerous innovations among which, most notably, supercontinuum light sources have become widely used in both fundamental and applied sciences. Here, we report on experimental evidence for dynamics of hybrid solitons—a new type of solitary wave, which emerges as a result of a strong non-instantaneous nonlinear response in CS2-filled liquid-core optical fibres. Octave-spanning supercontinua in the mid-infrared region are observed when pumping the hybrid waveguide with a 460 fs laser (1.95 μm) in the anomalous dispersion regime at nanojoule-level pulse energies. A detailed numerical analysis well correlated with the experiment uncovers clear indicators of emerging hybrid solitons, revealing their impact on the bandwidth, onset energy and noise characteristics of the supercontinua. Our study highlights liquid-core fibres as a promising platform for fundamental optics and applications towards novel coherent and reconfigurable light sources.
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    Phase transition observations and discrimination of small cloud particles by light polarization in expansion chamber experiments
    (München : European Geopyhsical Union, 2016) Nichman, Leonid; Fuchs, Claudia; Järvinen, Emma; Ignatius, Karoliina; Höppel, Niko Florian; Dias, Antonio; Heinritzi, Martin; Simon, Mario; Tröstl, Jasmin; Wagner, Andrea Christine; Wagner, Robert; Williamson, Christina; Yan, Chao; Connolly, Paul James; Dorsey, James Robert; Duplissy, Jonathan; Ehrhart, Sebastian; Frege, Carla; Gordon, Hamish; Hoyle, Christopher Robert; Kristensen, Thomas Bjerring; Steiner, Gerhard; McPherson Donahue, Neil; Flagan, Richard; Gallagher, Martin William; Kirkby, Jasper; Möhler, Ottmar; Saathoff, Harald; Schnaiter, Martin; Stratmann, Frank; Tomé, António
    Cloud microphysical processes involving the ice phase in tropospheric clouds are among the major uncertainties in cloud formation, weather, and general circulation models. The detection of aerosol particles, liquid droplets, and ice crystals, especially in the small cloud particle-size range below 50 μm, remains challenging in mixed phase, often unstable environments. The Cloud Aerosol Spectrometer with Polarization (CASPOL) is an airborne instrument that has the ability to detect such small cloud particles and measure the variability in polarization state of their backscattered light. Here we operate the versatile Cosmics Leaving OUtdoor Droplets (CLOUD) chamber facility at the European Organization for Nuclear Research (CERN) to produce controlled mixed phase and other clouds by adiabatic expansions in an ultraclean environment, and use the CASPOL to discriminate between different aerosols, water, and ice particles. In this paper, optical property measurements of mixed-phase clouds and viscous secondary organic aerosol (SOA) are presented. We report observations of significant liquid–viscous SOA particle polarization transitions under dry conditions using CASPOL. Cluster analysis techniques were subsequently used to classify different types of particles according to their polarization ratios during phase transition. A classification map is presented for water droplets, organic aerosol (e.g., SOA and oxalic acid), crystalline substances such as ammonium sulfate, and volcanic ash. Finally, we discuss the benefits and limitations of this classification approach for atmospherically relevant concentrations and mixtures with respect to the CLOUD 8–9 campaigns and its potential contribution to tropical troposphere layer analysis.
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    Weak solutions and weak-strong uniqueness for a thermodynamically consistent phase-field model
    (Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2019) Lasarzik, Robert; Rocca, Elisabetta; Schimperna, Giulio
    In this paper we prove the existence of weak solutions for a thermodynamically consistent phase-field model introduced in [26] in two and three dimensions of space. We use a notion of solution inspired by [18], where the pointwise internal energy balance is replaced by the total energy inequality complemented with a weak form of the entropy inequality. Moreover, we prove existence of local-in-time strong solutions and, finally, we show weak-strong uniqueness of solutions, meaning that every weak solution coincides with a local strong solution emanating from the same initial data, as long as the latter exists.
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    On the clustering property of the random intersection graphs
    (Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2008) Yao, Xin; Chen, Jinwen; Zhang, Changshui; Li, Yanda
    A random intersection graph mtlmcalG_V,W,p is induced from a random bipartite graph mtlmcalG^*_V,W,p with vertices classes mtlV, mtlW and the edges incident between mtlv in V and mtlw in W with probability mtlp. Two vertices in mtlV are considered to be connected with each other if both of them connect with some common vertices in mtlW. The clustering properties of the random intersection graph are investigated completely in this article. Suppose that the vertices number be mtlN = mabsV and mtlM=mabsW and mtlM = N^alpha, p=N^-beta, where mtlalpha > 0,, beta > 0, we derive the exact expressions of the clustering coefficient mtlC_v of vertex mtlv in mtlmcalG_V,W,p. The results show that if mtlalpha < 2beta and mtlalpha neq beta, mtlC_v decreases with the increasing of the graph size; if mtlalpha = beta or mtlalpha geq 2beta, the graph has the constant clustering coefficients, in addition, if mtlalpha > 2beta, the graph connecChangshui Zhangts almost completely. Therefore, we illustrate the phase transition for the clustering property in the random intersection graphs and give the condition that mtlriG being high clustering graph.
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    Shape optimization for a sharp interface model of distortion compensation
    (Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2013) Sturm, Kevin; Hintermüller, Michael; Hömberg, Dietmar
    We study a mechanical equilibrium problem for a material consisting of two components with different densities, which allows to change the outer shape by changing the interface between the subdomains. We formulate the shape design problem of compensating unwanted workpiece changes by controlling the interface, employ regularity results for transmission problems for a rigorous derivation of optimality conditions based on the speed method, and conclude with some numerical results based on a spline approximation of the interface.
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    Analysis of a thermodynamically consistent Navier--Stokes--Cahn--Hilliard model
    (Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2020) Lasarzik, Robert
    In this paper, existence of generalized solutions to a thermodynamically consistent Navier--Stokes--Cahn--Hilliard model introduced in [19] is proven in any space dimension. The generalized solvability concepts are measure-valued and dissipative solutions. The measure-valued formulation incorporates an entropy inequality and an energy inequality instead of an energy balance in a nowadays standard way, the Gradient flow of the internal variable is fulfilled in a weak and the momentum balance in a measure-valued sense. In the dissipative formulation, the distributional relations of the momentum balance and the energy as well as entropy inequality are replaced by a relative energy inequality. Additionally, we prove the weak-strong uniqueness of the proposed solution concepts and that all generalized solutions with additional regularity are indeed strong solutions.
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    Low Mach asymptotic preserving scheme for the Euler-Korteweg model
    (Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2013) Giesselmann, Jan
    We present an all speed scheme for the Euler-Korteweg model.We study a semi-implicit time-discretisation which treats the terms, which are stiff for low Mach numbers, implicitly and thereby avoids a dependence of the timestep restriction on the Mach number. Based on this we present a fully discrete finite difference scheme. In particular, the scheme is asymptotic preserving, i.e., it converges to a stable discretisation of the incompressible limit of the Euler-Korteweg model when the Mach number tends to zero.